Polyester Particle Dispersion for Toner Fusing

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Solution Overview

Problem

Existing toner production methods for electrophotography fail to achieve a homogeneous dispersion of crystalline and amorphous polyester particles, leading to insufficient low-temperature fusing and anti-hot offset properties, particularly when using trivalent or higher-valent carboxylic acids and requiring large amounts of organic solvents.

Innovation Solution

A process involving the emulsification of mixed polyester containing trivalent or higher-valent carboxylic acid units in an aqueous medium or with an organic solvent, allowing for the homogeneous dispersion of crystalline and amorphous polyester particles without excessive organic solvent use, followed by aggregation and coalescence to produce toners with enhanced low-temperature fusing and anti-hot offset properties.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Stability of the object's composition

If a large amount of organic solvent is used to emulsify mixed polyester containing trivalent or higher-valent carboxylic acid, then homogeneous dispersion is achieved, but solvent usage increases and production cost rises

Engineering Contradiction:
Improvehomogeneous dispersionVSAvoidsolvent usage
Core Design Contradiction:
Stability of the object's compositionVSQuantity of substance

Solution Approach 1:

The invention changes the chemical composition parameters of the amorphous polyester by incorporating trivalent or higher-valent carboxylic acid units (trimellitic anhydride, pyromellitic anhydride, or tricyclodecanetricarboxylic acid) in specific amounts (0.1-10 mol% based on total amorphous polyester). This compositional parameter change enables the polyester to form stable homogeneous dispersions without requiring large amounts of organic solvent, thus resolving the contradiction between dispersion quality and solvent usage.

Inventive Principle:
Principle #35Parameter changes

2Reliability

If trivalent or higher-valent carboxylic acid component is used in large amounts to improve anti-hot offset property, then anti-hot offset property is enhanced, but homogeneous dispersion becomes difficult to achieve

Engineering Contradiction:
Improveanti-hot offset propertyVSAvoidhomogeneous dispersion
Core Design Contradiction:
ReliabilityVSStability of the object's composition

Solution Approach 1:

The invention optimizes the concentration parameter of trivalent or higher-valent carboxylic acid units within a specific range (0.1-10 mol% based on total amorphous polyester). This parameter optimization ensures sufficient anti-hot offset property while maintaining the ability to form homogeneous dispersions, thus resolving the contradiction between functional performance and compositional stability.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention creates a composite polyester system combining crystalline polyester and amorphous polyester with trivalent or higher-valent carboxylic acid units in controlled proportions. This composite material approach allows the system to simultaneously achieve homogeneous dispersion and enhanced anti-hot offset property by balancing the contributions of different polyester components.

Inventive Principle:
Principle #40Composite materials

3Ease of manufacture

If divalent acid only is used in amorphous polyester to simplify production, then production process is simplified, but anti-hot offset property becomes insufficient

Engineering Contradiction:
Improveproduction process simplicityVSAvoidanti-hot offset property
Core Design Contradiction:
Ease of manufactureVSReliability

Solution Approach 1:

The invention modifies the chemical composition parameter of the amorphous polyester by introducing trivalent or higher-valent carboxylic acid units (changing from divalent acid only to include higher-valent acids). This parameter change directly enhances the anti-hot offset property of the toner while maintaining production feasibility, thus resolving the contradiction between manufacturing simplicity and product performance.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process enables the production of toners with improved low-temperature fusing and anti-hot offset properties by ensuring homogeneous dispersion and aggregation of polyester particles, reducing solvent usage and maintaining performance.

Implementation Method 1

emulsifying mixed polyester containing (1) an amorphous polyester containing a constitutional unit derived from a trivalent or higher-valent carboxylic acid in an amount of from 2.0 to 12.0 mol % and (2) a crystalline polyester, in an aqueous medium in a single vessel, or mixing the mixed polyester with an organic solvent and then adding an aqueous medium to the resulting mixture to emulsify the mixed polyester in a single vessel

Methodology Applied
Scientific EffectEmulsification: Emulsion

Implementation Method 2

a toner which is produced at least by conducting a step of aggregating and coalescing the above dispersion of polyester particles

Methodology Applied
Scientific EffectAggregation: Coagulation

Implementation Method 3

a step of aggregating and coalescing the above dispersion of polyester particles

Methodology Applied
Scientific EffectCoalescence:

Data Source

PatentUS8652746B2Manufacturing method for polyester particle dispersion liquid
Publication Date: 2014.02.18 KAO CORP

AI summary

The present invention relates to a process for producing a dispersion of polyester particles which includes the step of emulsifying mixed polyester containing (1) an amorphous polyester containing a constitutional unit derived from a trivalent or higher-valent carboxylic acid in an amount of from 2.0 to 12.0 mol % on the basis of whole constitutional units of the whole amorphous polyester and (2) a crystalline polyester, in an aqueous medium in a single vessel, or the step of mixing the mixed polyester with an organic solvent and then adding the aqueous medium to the resulting mixture to emulsify the mixed polyester in a single vessel. The present invention also relates to a dispersion of polyester particles produced by the above production process, as well as a toner for electrophotography which is produced by subjecting the dispersion of the polyester particles to aggregation and coalescence and is excellent in both of a low-temperature fusing property and an anti-hot offset property, and a process for producing the toner.