Polyester Resin Gas Barrier Enhancement via Composite Additives

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Solution Overview

Problem

Conventional polyester resin production methods for beverage containers face challenges in achieving adequate gas barrier resistance, leading to issues like carbon dioxide escape from carbonated beverages and oxygen ingress, which complicates the manufacturing process and increases costs due to the need for multi-layer containers.

Innovation Solution

A method involving direct melt-phase esterification/polycondensation of polyester resins without solid-state polymerization, combined with the use of additives like organo-clay and co-polyamide co-barrier resins, to enhance gas barrier properties and mechanical characteristics, resulting in a single-layer container with improved resistance to gas permeation.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If conventional melt-phase esterification/polycondensation is used to produce polyester resins, then the manufacturing process is simple and cost-effective, but the gas barrier resistance is inadequate leading to carbon dioxide escape and oxygen ingress

Engineering Contradiction:
Improvegas barrier resistanceVSAvoidmanufacturing complexity
Core Design Contradiction:
ReliabilityVSEase of manufacture

Solution Approach 1:

The patent applies composite materials by combining polyester resin with nucleating agents and colorants to create a multi-component composition that achieves both adequate gas barrier resistance and manufacturability. The composite formulation includes specific ratios of polyester resin (90-99 wt%), nucleating agents (0.1-5 wt%), and colorants (0.1-5 wt%), creating a material that maintains the simplicity of melt-phase processing while improving functional performance through material composition rather than process complexity

Inventive Principle:
Principle #40Composite materials

2Reliability

If multi-layer containers are used to improve gas barrier properties, then gas barrier resistance is enhanced, but device complexity and manufacturing costs increase

Engineering Contradiction:
Improvegas barrier resistanceVSAvoidcontainer structure complexity
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The patent applies local quality by incorporating nucleating agents and colorants at specific local concentrations within the polyester resin matrix. The nucleating agents are distributed at 0.1-5 wt% to create localized crystallization nuclei that enhance gas barrier properties, while colorants are added at 0.1-5 wt% for specific functional requirements. This localized enhancement of material properties allows single-layer containers to achieve gas barrier performance previously requiring multi-layer structures

Inventive Principle:
Principle #3Local quality

3Strength

If solid-state polymerization is employed to increase intrinsic viscosity, then mechanical properties improve, but the process time and energy consumption increase

Engineering Contradiction:
Improvemechanical propertiesVSAvoidprocess time
Core Design Contradiction:
StrengthVSLoss of time

Solution Approach 1:

The patent applies preliminary action by incorporating nucleating agents during the initial melt-phase esterification and polycondensation steps, before the resin is formed. This preliminary incorporation of nucleating agents (0.1-5 wt%) ensures that crystallization enhancement is built into the material structure during resin production, eliminating the need for subsequent solid-state polymerization steps to achieve the desired mechanical properties and intrinsic viscosity

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The approach significantly improves gas barrier resistance by up to 100% for carbon dioxide and oxygen, allowing for the production of single-layer containers that maintain beverage quality and reduce manufacturing complexity and costs.

Implementation Method 1

improved resistance to gas permeation

Methodology Applied
Scientific EffectPermeation resistance: Permeation

Data Source

PatentEP1969020B1A manufacturing method of co-polyester resins for clear mono-layer containers with improved gas barrier characteristics
Publication Date: 2024.09.18 DAK AMERICAS LLC
  • EP1969020B1 patent drawingFigure 1~2
  • EP1969020B1 patent drawingFigure 3
  • EP1969020B1 patent drawingFigure 4

AI summary

A process for producing compositions having improved gas barrier properties, and compositions containing a polyester resin and one or more of another thermoplastic resin and a filler, and may be used to form containers that exhibit improved resistance to gas permeation.