Polyester Resin Low-Temperature Solubility via Isosorbide and Trihydric Alcohol Units

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Solution Overview

Problem

Polyester resins with biomass-derived monomers, such as those described in Patent Literature 1, lack sufficient solubility in generic solvents, especially at low temperatures, requiring heating or use in warm conditions, which limits their application in cold regions.

Innovation Solution

A polyester resin formulation that includes specific ratios of isosorbide-derived and trihydric or higher alcohol-derived structural units relative to polycarboxylic acid-derived units, along with structural units from dihydric alcohols with alicyclic skeletons, enhances solubility at temperatures below 0°C, achieving improved storage stability and moisture resistance.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Adaptability or versatility

If polyester resin is made from biomass-derived monomers (isosorbide), then environmental sustainability is improved, but solubility in generic solvents at low temperatures deteriorates

Engineering Contradiction:
Improveenvironmental sustainabilityVSAvoidsolubility at low temperature
Core Design Contradiction:
Adaptability or versatilityVSReliability

Solution Approach 1:

The patent creates a composite polyester resin structure combining isosorbide-derived units (for sustainability) with trihydric or higher alcohol-derived units (for solubility enhancement). This composite approach allows the resin to maintain both environmental benefits and improved low-temperature solubility through the synergistic effect of different structural units working together

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent changes the compositional parameters of the polyester resin by controlling the molar ratios of different structural units. Specifically, it optimizes the content of isosorbide-derived units (0.1-0.5 mol) and trihydric or higher alcohol-derived units (0.03-0.3 mol) relative to polycarboxylic acid units to achieve the desired balance between sustainability and solubility performance

Inventive Principle:
Principle #35Parameter changes

2Adaptability or versatility

If polyester resin contains isosorbide-derived structural units, then biomass utilization is improved, but solubility in generic solvents deteriorates

Engineering Contradiction:
Improvebiomass utilizationVSAvoidsolubility in generic solvents
Core Design Contradiction:
Adaptability or versatilityVSEase of operation

Solution Approach 1:

The patent combines isosorbide-derived structural units with trihydric or higher alcohol-derived structural units in a specific composite structure. This composite design allows the resin to maintain high biomass utilization from isosorbide while the trihydric alcohol units provide enhanced solubility in generic solvents, resolving the contradiction between biomass content and solubility

Inventive Principle:
Principle #40Composite materials

3Adaptability or versatility

If polyester resin is formulated for cold region use, then application range is improved, but heating requirements are eliminated only if solubility is enhanced

Engineering Contradiction:
Improveapplication rangeVSAvoidheating requirement
Core Design Contradiction:
Adaptability or versatilityVSEase of manufacture

Solution Approach 1:

The patent changes the chemical composition parameters of the polyester resin by incorporating trihydric or higher alcohol-derived units in controlled amounts (0.03-0.3 mol relative to polycarboxylic acid units). This compositional change reduces the glass transition temperature and enhances chain flexibility, allowing the resin to maintain solubility at low temperatures without requiring heating during application

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The improved solubility of the polyester resin at low temperatures facilitates the preparation of paints and coating materials, ensuring they remain usable and effective in cold conditions without the need for heating, thereby expanding their application range.

Implementation Method 1

exhibits excellent solubility under low-temperature conditions, especially at or lower than 0° C.

Methodology Applied
Scientific EffectSolvation: Solvation

Data Source

PatentUS10093771B2Polyester resin, method for manufacturing polyester resin, and coating composition containing polyester resin
Publication Date: 2018.10.09 MITSUBISHI CHEM CORP

AI summary

The present invention relates to a polyester resin with excellent solubility in generic solvents, especially with excellent solubility at a temperature of 0° C. or lower. According to the present invention, by using the polyester resin with excellent solubility in generic solvents, solubility at a lower temperature, especially the solubility at a temperature of 0° C. or lower, is enhanced, making it easier to prepare paints, coatings and the like. The polyester resin related to the present invention contains 0.05 to 0.5 mol of an isosorbide-derived structural unit and 0.015 to 0.4 mol of a trihydric or higher alcohol-derived structural unit relative to 1 mol of a polycarboxylic acid-derived structural unit.