Polyether Carrier Fluid Stabilizes Catalyst Package

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Solution Overview

Problem

Two-part moisture cure organopolysiloxane compositions face issues with phase separation during storage, which affects the stability and usability of the catalyst package, leading to reduced productivity and safety concerns due to flammable catalysts, and fast curing rates that limit tooling time and adhesion development.

Innovation Solution

A two-part moisture curing silicone composition using a carrier fluid of linear or branched polyethers with specific terminal groups, combined with non-dipodal aminosilanes, tin-based catalysts, and fillers, to create a shelf-stable continuous phase that prevents phase separation and maintains adhesion and cure speed.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Stability of the object's composition

If conventional carrier fluids (trimethylsiloxy-terminated polydimethylsiloxane) are used in catalyst packages, then the catalyst package can be formulated, but phase separation occurs during storage reducing stability

Engineering Contradiction:
Improvestorage stabilityVSAvoidphase separation
Core Design Contradiction:
Stability of the object's compositionVSReliability

Solution Approach 1:

The patent changes the chemical parameters of the carrier fluid by using polyether carrier fluids with specific molecular weights (200-750,000 g/mol) and viscosity ranges (5-50,000 mPa·s) instead of conventional polydimethylsiloxane carrier fluids. This parameter change prevents phase separation while maintaining catalyst package stability during storage.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite catalyst package system by combining polyether carrier fluids with specific aminosilanes (non-dipodal structures), tin catalysts, and fillers. This composite formulation ensures compatibility between all components, preventing phase separation while maintaining functionality.

Inventive Principle:
Principle #40Composite materials

2Productivity

If tin catalyst and aminosilane levels are increased to achieve faster bulk durometer build, then substrates can be moved sooner, but tooling time and tack-free time are reduced

Engineering Contradiction:
Improvebulk durometer build speedVSAvoidtooling time
Core Design Contradiction:
ProductivityVSDuration of action of moving object

Solution Approach 1:

The patent optimizes the concentration parameters of catalysts and aminosilanes within specific ranges (0.01-3 wt% tin catalyst, 5-25 wt% aminosilane) rather than simply increasing them. This allows achieving fast bulk durometer build while maintaining adequate tooling time through precise parameter control.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The polyether carrier fluid acts as an intermediary that modulates the interaction between tin catalyst and aminosilane, enabling controlled cure kinetics. This intermediary effect allows the system to achieve fast bulk durometer build without excessively reducing tooling time.

Inventive Principle:
Principle #24Intermediary (Mediator)

3Reliability

If high concentrations of primary amine and tin catalyst are used in catalyst package, then adequate curing functionality is achieved, but random chain scission of carrier fluid occurs reducing viscosity and increasing particle settling

Engineering Contradiction:
Improvecuring functionalityVSAvoidcarrier fluid viscosity
Core Design Contradiction:
ReliabilityVSStability of the object's composition

Solution Approach 1:

The patent changes the chemical structure parameters of the carrier fluid from polydimethylsiloxane to polyether structures with specific molecular weights and viscosities. These parameter changes make the carrier fluid resistant to chain scission by high concentrations of catalysts and aminosilanes, maintaining viscosity stability.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent selects polyether carrier fluids that are inherently more resistant to degradation by catalysts compared to conventional carrier fluids. This selection criterion ensures the carrier fluid maintains its properties throughout the catalyst package shelf life without requiring additional protective measures.

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution provides improved storage stability, faster bulk durometer build, and maintained adhesion properties without sacrificing cure speed, reducing the need for additional catalysts or aminosilanes, thus enhancing productivity and safety.

Implementation Method 1

the catalyst package, despite comprising amino silane(s), alkoxy silane(s), tin catalyst(s) and optionally reinforcing filler(s) and/or extending filler(s) in a carrier fluid, undergoes minimal phase separation during storage, by utilizing a silane end-capped polyether as the carrier fluid, enabling the catalyst package to be stored and function as a shelf stable continuous phase

Methodology Applied
Scientific EffectPhase separation prevention:

Implementation Method 2

Condensation curable organosiloxane compositions, which cure to elastomeric solids

Methodology Applied
Scientific EffectCondensation cure: Condensation

Implementation Method 3

Two-part moisture cure organopolysiloxane compositions

Methodology Applied
Scientific EffectMoisture cure mechanism:

Implementation Method 4

a second part (catalyst or cure package) containing an alkyl-terminated diorganopolysiloxane, tin based catalyst, cross-linker and aminosilane

Methodology Applied
Scientific EffectCatalysis: Catalysis

Implementation Method 5

curing proceeds via a bulk cure mechanism wherein the composition will cure simultaneously throughout the material bulk

Methodology Applied
Scientific EffectBulk cure mechanism:

Data Source

PatentUS20240400830A1Moisture curable compositions
Publication Date: 2024.12.05 DOW SILICONES CORP

AI summary

A two-part moisture cure organopolysiloxane composition comprising a base part and a catalyst package part is provided. The catalyst package part undergoes minimal phase separation during storage despite comprising amino silane(s), alkoxy silane(s), and tin catalyst(s) and optionally reinforcing filler(s) and/or extending filler(s). This is given by the utilization of one or more linear or branched polyethers as a carrier fluid thereby enabling the catalyst package part to function as a shelf stable continuous phase.