Polyisocyanate Composition for Stable Polyurethane Foams

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Solution Overview

Problem

Existing polyurethane formulations for aerosol foams and adhesives face challenges with high viscosities and poor storage stability due to high monomeric isocyanate content, leading to usability issues and safety concerns from respirable isocyanates.

Innovation Solution

A process involving a mixture of diphenylmethane diisocyanate and polyphenylene polymethylene polyisocyanates with specific composition and purification to reduce uretonimine and monomeric isocyanate content, resulting in polyisocyanates with improved storage stability and processing properties.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Object-affected harmful factors

If monomeric isocyanates are removed by distillation to reduce respirable isocyanates, then safety is improved, but storage stability deteriorates

Engineering Contradiction:
Improverespirable isocyanate contentVSAvoidstorage stability
Core Design Contradiction:
Object-affected harmful factorsVSReliability

Solution Approach 1:

The patent changes the chemical composition parameters by controlling the core structure distribution (2-core MDI ≤2%, 3-core MDI 25-65%, 4-core MDI 5-45%, >5-core MDI 1-40%) and functionality (2.2-5.2) of polyphenylene polymethylene polyisocyanates. This parameter optimization achieves both low monomeric isocyanate content (<0.5% by weight) and improved storage stability, resolving the contradiction between safety and reliability

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent uses composite polyisocyanate formulations combining different core structures (2-core, 3-core, 4-core, and >5-core MDI) in specific proportions. This composite approach creates a synergistic effect where the mixture maintains stability while reducing harmful monomeric isocyanates, addressing both safety and storage stability requirements

Inventive Principle:
Principle #40Composite materials

2Object-affected harmful factors

If polyisocyanates with reduced monomer content are used, then safety is improved, but viscosity increases

Engineering Contradiction:
Improvemonomeric isocyanate contentVSAvoidviscosity
Core Design Contradiction:
Object-affected harmful factorsVSEase of operation

Solution Approach 1:

The patent optimizes the functionality parameter (average functionality 2.2-5.2) and core structure distribution of polyisocyanates to achieve the right balance. By controlling these parameters, the formulation reduces monomeric isocyanate content while maintaining viscosity at acceptable levels for processing, resolving the contradiction between safety and ease of operation

Inventive Principle:
Principle #35Parameter changes

3Productivity

If polyisocyanates with high functionality are used, then productivity is improved, but manufacturing complexity increases

Engineering Contradiction:
Improvecrosslinking efficiencyVSAvoidpolyisocyanate composition complexity
Core Design Contradiction:
ProductivityVSDevice complexity

Solution Approach 1:

The patent defines specific parameter ranges for functionality (2.2-5.2) and core structure distribution to optimize crosslinking efficiency. By establishing these parameter specifications, the patent achieves high productivity through efficient crosslinking while managing manufacturing complexity through clear compositional guidelines

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process produces polyisocyanates with reduced viscosity and enhanced storage stability, ensuring safer and more effective use in one- and two-component polyurethane systems, including aerosol foams and rigid foams, with improved processing and storage characteristics.

Implementation Method 1

reacting polyisocyanates a) with compounds having at least two hydrogen atoms reactive with isocyanate groups b)

Methodology Applied
Scientific EffectIsocyanate-hydrogen reaction: Chemical Bonding

Implementation Method 2

removing the unreacted monomeric isocyanates after the reaction, for example by distillation

Methodology Applied
Scientific EffectDistillation: Distillation

Data Source

PatentEP2013258B1Process for preparing polyurethanes
Publication Date: 2010.08.25 BASF SE

AI summary

The invention provides a process for preparing polyurethanes by reacting polyisocyanates a) with compounds having at least two hydrogen atoms reactive with isocyanate groups b), characterized in that the polyisocyanate a) used is at least one polyisocyanate ai) with a mean functionality of greater than 2, a content of diisocyanates of not more than 2% by weight and a content of uretonimines of not more than 4% by weight, based in each case on the weight of the polyisocyanate ai).