Polymer Complex with Surface-Fibrillated Microcellulose Fibers

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Solution Overview

Problem

The production of nanocellulose fibers is complicated and costly, and they tend to aggregate, limiting their dispersion and reinforcing effect in polymer complexes, which affects the mechanical properties of the resulting materials.

Innovation Solution

A polymer complex is developed using microcellulose fibers with nanofibrils and fine particles, where the microcellulose fibers are fibrillated by growing fine particles without nano-sizing, and then complexed with a polymer matrix, enhancing mechanical properties and dispersibility.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Strength

If nanocellulose fibers are produced through traditional nanosizing processes, then reinforcing effect is improved, but production complexity and cost increase

Engineering Contradiction:
Improvereinforcing effectVSAvoidproduction complexity
Core Design Contradiction:
StrengthVSDevice complexity

Solution Approach 1:

The invention segments the cellulose fiber structure into microcellulose fibers with surface-raised nanofibrils, achieving nanoscale reinforcing effects without requiring complete nanosizing of the entire fiber structure. This segmentation allows retention of microfiber integrity while incorporating nanoscale elements for reinforcement.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The invention performs preliminary fibrillation action during the microcellulose fiber formation stage, raising nanofibrils on the fiber surface before final fiber assembly. This preliminary action eliminates the need for subsequent complex nanosizing processes.

Inventive Principle:
Principle #10Preliminary action

2Strength

If nanocellulose fibers are used as reinforcing material, then mechanical properties are improved, but dispersibility deteriorates due to aggregation

Engineering Contradiction:
Improvemechanical propertiesVSAvoiddispersibility
Core Design Contradiction:
StrengthVSStability of the object's composition

Solution Approach 1:

The invention applies local quality by concentrating nanofibrils only on the surface of microcellulose fibers rather than requiring complete nanosizing throughout. This localized nanofibril formation improves dispersibility while maintaining reinforcing capabilities at the fiber-matrix interface.

Inventive Principle:
Principle #3Local quality

Solution Approach 2:

The invention creates a composite structure combining microcellulose fibers with surface-raised nanofibrils, achieving a hierarchical composite that combines the dispersibility advantages of microfibers with the reinforcing advantages of nanofibrils.

Inventive Principle:
Principle #40Composite materials

3Stability of the object's composition

If cellulose fibers are complexed with polymers at high temperature, then complexation is improved, but fiber deterioration increases

Engineering Contradiction:
ImprovecomplexationVSAvoidfiber deterioration
Core Design Contradiction:
Stability of the object's compositionVSObject-affected harmful factors

Solution Approach 1:

The invention changes the temperature parameter during complexation by utilizing the high surface area and reactivity of surface-raised nanofibrils, which enable effective polymer complexation at lower temperatures, thereby preventing fiber deterioration while achieving sufficient complexation.

Inventive Principle:
Principle #35Parameter changes

Data Source

PatentEP4011955B1Polymer complex
Publication Date: 2025.08.20 LG CHEM LTD
  • EP4011955B1 patent drawingFigure 1(a)~1(d)
  • EP4011955B1 patent drawingFigure 2~3
  • EP4011955B1 patent drawingFigure 4

AI summary

The present disclosure relates to a polymer complex. According to the present disclosure, there is provided a polymer complex capable of exhibiting excellent mechanical properties while being environmentally friendly by including cellulose fibers as a reinforcing material.