Contaminated Polymer Depolymerization with Trapping Agents

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Solution Overview

Problem

Existing depolymerization processes for recycling plastics, such as poly(methyl methacrylate) (PMMA), struggle to effectively reduce the concentration of contaminants like pigments, plasticizers, and degradation products, which can lead to contamination of the resulting monomers and pose environmental and health risks.

Innovation Solution

The introduction of one or more trapping agents during the depolymerization process, which interact with contaminants to immobilize or degrade them, allowing for their separation from the monomers. These trapping agents can include dolomite, diatomaceous earth, metal oxides, and supported peroxides.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If conventional depolymerization processes are used to recycle PMMA, then the process is simple and energy-efficient, but the concentration of contaminants (pigments, plasticizers, degradation products) in the resulting monomers remains high

Engineering Contradiction:
Improvepurity of recovered monomersVSAvoidcomplexity of depolymerization process
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The patent introduces trapping agents as intermediary substances that mediate between the contaminants and the depolymerization process. These agents (such as metal oxides, activated carbon, or molecular sieves) selectively capture contaminants like pigments, plasticizers, and degradation products, allowing the monomers to be recovered with high purity without requiring complex additional separation equipment

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent modifies the depolymerization process by changing parameters such as temperature profiles, residence time, and the addition of trapping agents. By optimizing these parameters, the process achieves both high monomer purity and reasonable process complexity, resolving the contradiction between manufacturing precision and device complexity

Inventive Principle:
Principle #35Parameter changes

2Productivity

If high temperature pyrolysis is used to depolymerize PMMA, then the depolymerization efficiency is high, but contaminants are released and contaminate the crude MMA

Engineering Contradiction:
Improvedepolymerization efficiencyVSAvoidcontaminant release
Core Design Contradiction:
ProductivityVSObject-generated harmful factors

Solution Approach 1:

The patent converts the harmful effect of high temperature (which releases contaminants) into a beneficial process by introducing trapping agents that capture these contaminants. The high temperature continues to provide efficient depolymerization, while the trapping agents transform the harmful contaminant release into a controlled capture mechanism, ultimately improving monomer purity

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Solution Approach 2:

Trapping agents serve as intermediaries between the high temperature pyrolysis process and the crude MMA product. These agents (such as metal oxides or activated carbon) intercept contaminants released during high-temperature depolymerization, preventing them from contaminating the monomer while allowing the efficient high-temperature process to continue

Inventive Principle:
Principle #24Intermediary (Mediator)

3Reliability

If polyethylene protection film is present with PMMA, then the plastic provides necessary protection, but polyethylene degrades at higher temperature and generates long chain oligomers that decrease the quality of recovered crude MMA

Engineering Contradiction:
Improveprotection function of plastic filmVSAvoidquality of recovered monomers
Core Design Contradiction:
ReliabilityVSManufacturing precision

Solution Approach 1:

The patent extracts or removes the harmful polyethylene degradation products from the system by using trapping agents that selectively capture long chain oligomers and waxes. This allows the polyethylene protection film to fulfill its protective function while its degradation products are removed before they can contaminate the recovered MMA monomers

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

Trapping agents act as intermediaries that selectively interact with polyethylene degradation products (long chain oligomers and waxes) without interfering with the PMMA depolymerization. This mediation allows the protection film to remain functional while its harmful degradation products are captured and removed from the monomer recovery stream

Inventive Principle:
Principle #24Intermediary (Mediator)

4Adaptability or versatility

If EVA copolymer is used as PVC replacement, then the plastic provides necessary functionality, but EVA decomposes into acetic acid and hydrocarbon oligomers that generate corrosion and decrease monomer quality

Engineering Contradiction:
Improvefunctional replacement capabilityVSAvoidcorrosion and oligomer contamination
Core Design Contradiction:
Adaptability or versatilityVSObject-generated harmful factors

Solution Approach 1:

The patent converts the harmful corrosion and contamination effects of EVA decomposition into a manageable process by using trapping agents to capture acetic acid and hydrocarbon oligomers. The EVA copolymer continues to provide its functional replacement capability, while its degradation products are transformed from harmful contaminants into captured substances that can be easily removed

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Solution Approach 2:

Trapping agents serve as intermediaries that selectively capture EVA degradation products (acetic acid and hydrocarbon oligomers) without interfering with the functional performance of the EVA copolymer during depolymerization. This mediation allows EVA to fulfill its replacement function while its harmful decomposition products are intercepted and removed

Inventive Principle:
Principle #24Intermediary (Mediator)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The use of trapping agents significantly reduces the concentration of contaminants in the resulting monomers, improving the quality of the recycled products, reducing environmental risks, and facilitating proper waste management.

Implementation Method 1

contacting at least one solid trapping agent with the contaminated polymers to be depolymerized... whereby the non-PET and non-PVC contaminants interact with the solid trapping agents

Methodology Applied
Scientific EffectAdsorption: Adsorption

Implementation Method 2

depolymerizing the polymers leading to corresponding monomers

Methodology Applied
Scientific EffectPyrolysis: Pyrolysis

Data Source

PatentUS20250075051A1Process for recycling contaminated polymers
Publication Date: 2025.03.06 ARKEMA FRANCE SA

AI summary

The present invention concerns an improved depolymerization process of contaminated polymers such as PMMA, comprising the separation of contaminants from the resulting monomers, by using appropriate agents for trapping the contaminants.