Method and system for polymer production

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Solution Overview

Problem

Existing methods struggle to produce polyolefin copolymers with high molecular weights in high concentrations while effectively reducing solvent levels, especially for elastomeric polymers with low bulk melting temperatures, and face challenges from stringent environmental regulations regarding volatile organic compound emissions.

Innovation Solution

A solution polymerization system utilizing a series of reactors, including continuous stirred tank reactors and loop reactors, combined with multiple devolatilization vessels and heat exchangers, to achieve high polymer concentrations and low solvent levels, using adiabatic flashing and sequential devolatilization to maintain the polymer in a single phase and reduce volatile content below 400 ppm.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Quantity of substance

If conventional solution polymerization is used to produce polyolefin copolymers, then polymer production capacity is achieved, but solvent levels remain high and polymer concentration is limited

Engineering Contradiction:
Improvepolymer concentrationVSAvoidsolvent content
Core Design Contradiction:
Quantity of substanceVSLoss of substance

Solution Approach 1:

The devolatilization process is divided into multiple sequential stages with progressively decreasing pressures. The first stage operates at higher pressure to remove bulk solvent, followed by second and third stages at progressively lower pressures to achieve ultra-low solvent levels (<400 ppm). This segmented approach enables efficient solvent removal while maintaining high polymer concentration throughout the process.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The system dynamically changes operating parameters, specifically pressure and temperature, across different devolatilization stages. Pressure is reduced sequentially from stage one to stage three, while temperature is adjusted to optimize solvent vaporization. These parameter changes enable the system to achieve both high polymer concentration and ultra-low solvent content.

Inventive Principle:
Principle #35Parameter changes

2Use of energy by moving object

If adiabatic flashing is used to reduce solvent levels, then energy consumption is reduced, but temperature control becomes challenging

Engineering Contradiction:
Improveenergy consumptionVSAvoidtemperature control
Core Design Contradiction:
Use of energy by moving objectVSTemperature

Solution Approach 1:

The system incorporates temperature monitoring and control mechanisms in each devolatilization stage to manage the temperature drops caused by adiabatic flashing. By providing feedback on actual temperature conditions, the system can adjust operating parameters to maintain optimal conditions for solvent removal while preventing excessive cooling that would affect polymer quality.

Inventive Principle:
Principle #23Feedback

Solution Approach 2:

The polymer solution is preheated before entering each devolatilization stage to compensate for the temperature drop that will occur during adiabatic flashing. This preliminary heating action ensures that the polymer maintains appropriate temperature and viscosity characteristics throughout the solvent removal process, enabling efficient operation without excessive energy input.

Inventive Principle:
Principle #10Preliminary action

3Manufacturing precision

If multiple devolatilization stages are implemented to achieve low solvent levels, then polymer purity is improved, but system complexity increases

Engineering Contradiction:
Improvepolymer purityVSAvoidsystem complexity
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

Multiple devolatilization stages are combined into a single integrated system with shared infrastructure. Common elements such as heat exchangers, pressure control systems, and polymer transfer mechanisms are consolidated across all three stages, reducing overall system complexity while maintaining the purity benefits of multi-stage processing.

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

Each devolatilization stage is designed with multi-functional capabilities, serving both as a solvent removal unit and as a polymer concentration unit. The system simultaneously achieves multiple objectives - solvent elimination, polymer concentration, and temperature management - within each stage, reducing the need for separate dedicated equipment and simplifying the overall process design.

Inventive Principle:
Principle #6Universality (Multi-functionality)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The system efficiently produces polyolefin copolymers with high molecular weights and low solvent content, meeting product quality and environmental regulation standards by maintaining the polymer in a single phase and effectively removing volatile components.

Implementation Method 1

using adiabatic flashing and sequential devolatilization to maintain the polymer in a single phase and reduce volatile content below 400 ppm

Methodology Applied
Scientific EffectAdiabatic flashing: Adiabatic Cooling

Implementation Method 2

A solution polymerization system utilizing a series of reactors, including continuous stirred tank reactors and loop reactors, combined with multiple devolatilization vessels and heat exchangers

Methodology Applied
Scientific EffectHeat exchange: Heat Exchanger

Implementation Method 3

using adiabatic flashing and sequential devolatilization to maintain the polymer in a single phase

Methodology Applied
Scientific EffectPhase change: Phase Change

Data Source

PatentEP3801875B1Method and system for polymer production
Publication Date: 2026.03.18 DOW GLOBAL TECHNOLOGIES LLC
  • EP3801875B1 patent drawingFigure 1
  • EP3801875B1 patent drawingFigure 2
  • EP3801875B1 patent drawingFigure 3A~3B

AI summary

Disclosed herein is a system for solution polymerization comprising a reactor system that is operative to receive a monomer and to react the monomer to form a polymer; a plurality of devolatilization vessels located downstream of the reactor system, where each devolatilization vessel operates at a lower pressure than the preceding devolatilization vessel; and a heat exchanger disposed between two devolatilization vessels and in fluid communication with them, where the heat exchanger has an inlet port temperature of 100°C to 230°C, an outlet port temperature of 200°C to 300°C, an inlet port pressure of 35 to 250 kgf/cm2 and an outlet port pressure of 20 to 200 kgf/cm2; and wherein the polymer solution remains in a single phase during its residence in the heat exchanger.