Polymer Latex Chain-Transfer Sequencing for Higher Strength

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Solution Overview

Problem

Existing polymer latexes used in paper and carpet backing applications lack sufficient mechanical properties, such as high elongation at break and tensile strength, which are essential for effective binding and resistance to moisture and ink splitting forces during printing processes.

Innovation Solution

A polymer latex is produced by combining hydroperoxide and sulfur-containing chain transfer agents during the polymerization of ethylenically unsaturated aromatic and conjugated diene monomers, where the sulfur-containing agent is added after a significant portion of the hydroperoxide has been introduced, resulting in a polymer with improved mechanical properties.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Strength

If conventional polymerization methods using single chain transfer agents are used, then the polymerization process is simple, but the mechanical properties (elongation at break and tensile strength) are insufficient

Engineering Contradiction:
Improvemechanical properties (elongation at break and tensile strength)VSAvoidpolymerization process complexity
Core Design Contradiction:
StrengthVSDevice complexity

Solution Approach 1:

The patent combines two different chain transfer agents (hydroperoxide and sulfur-containing compounds) in a single polymerization process. The hydroperoxide chain transfer agent is added first to initiate polymerization and control molecular weight, followed by the sulfur-containing chain transfer agent to further modify polymer structure and enhance mechanical properties. This merging of multiple agents achieves superior elongation at break and tensile strength that cannot be obtained with a single agent alone.

Inventive Principle:
Principle #5Merging (Combining)

2Strength

If polymer latex with high tensile strength is produced, then binding strength in paper coating is improved, but the flexibility for ease of installation may be reduced

Engineering Contradiction:
Improvetensile strength and binding strengthVSAvoidflexibility for ease of installation
Core Design Contradiction:
StrengthVSEase of operation

Solution Approach 1:

The patent optimizes the concentration ratios and addition sequences of hydroperoxide and sulfur-containing chain transfer agents to achieve the desired balance between strength and flexibility. By carefully controlling the amounts of each agent and their addition timing, the polymer latex attains high tensile strength for binding while maintaining sufficient flexibility for carpet installation and pattern matching.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The resulting polymer latex exhibits superior binding effects with high elongation and tensile strength, enhancing the performance in paper coatings, carpet backing, and fiber fabric pre-impregnation processes by providing better resistance to ink splitting and moisture retention.

Implementation Method 1

polymerizing one or more ethylenically unsaturated aromatic monomers and one or more conjugated diene monomers in the presence of hydroperoxide chain transfer agent and sulfur-containing chain transfer agent

Methodology Applied
Scientific EffectPolymerization: Photopolymerisation

Implementation Method 2

the combination of a hydroperoxide chain transfer agent and a sulfur-containing chain transfer agent allows the polymerization to provide a polymer latex with improved mechanical properties

Methodology Applied
Scientific EffectChain transfer:

Data Source

PatentEP2567985B1Polymer latex with improved mechanical properties and process for preparing said polymer latex
Publication Date: 2016.11.09 TRINSEO EURO GMBH
  • EP2567985B1 patent drawingFigure 1
  • EP2567985B1 patent drawing

AI summary

The present invention relates to a process for preparing a polymer latex comprising polymerizing one or more ethylenically unsaturated aromatic monomers and one or more conjugated diene monomers in the presence of hydroperoxide chain transfer agent and sulfur-containing chain transfer agent, wherein the sulfur-containing chain transfer agent is added after the hydroperoxide chain transfer agent. It further relates to the polymer latex thus obtained, to a composition comprising the polymer latex and to the use of the polymer latex or polymer latex composition in a carpet backing, paper coating, or fiber fabric pre-impregnation process.