Polymer Microparticles Narrow Particle Diameter Distribution

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Solution Overview

Problem

Conventional processes for producing polymer microparticles with high heat resistance, particularly crystalline polymers, face challenges such as high viscosity during emulsion formation and wider particle diameter distribution.

Innovation Solution

A process involving the formation of an emulsion at 100°C or higher, using a polymer (A) and polymer (B) with specific structural units, and a poor solvent, where the polymer (A) is precipitated at a temperature equal to or above its cooling crystallization temperature, ensuring phase separation and narrow particle diameter distribution.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If a highly heat-resistant polymer (crystalline polymer) is used to produce microparticles with high heat resistance, then the heat resistance of the microparticles is improved, but the viscosity of the system becomes high during emulsion formation and the particle diameter distribution becomes wider

Engineering Contradiction:
Improveheat resistance of microparticlesVSAvoidparticle diameter distribution
Core Design Contradiction:
ReliabilityVSManufacturing precision

Solution Approach 1:

The invention changes the temperature parameter during emulsion formation to 100°C or higher, which reduces the viscosity of the system and improves the particle diameter distribution. This temperature parameter change allows the highly heat-resistant polymer to be processed while maintaining narrow particle size distribution.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention utilizes phase separation between two polymer solutions with different solubility parameters. By controlling the phase separation process and using a poor solvent to precipitate polymer A, the system achieves narrow particle diameter distribution while maintaining the heat resistance of the crystalline polymer.

Inventive Principle:
Principle #36Phase transitions

2Reliability

If a highly heat-resistant polymer (crystalline polymer) is used to produce microparticles with high heat resistance, then the heat resistance of the microparticles is improved, but the viscosity of the system becomes high during emulsion formation

Engineering Contradiction:
Improveheat resistance of microparticlesVSAvoidemulsion formation process
Core Design Contradiction:
ReliabilityVSEase of manufacture

Solution Approach 1:

The invention changes the temperature parameter during emulsion formation to 100°C or higher, which significantly reduces the viscosity of the system and makes emulsion formation easier. This high-temperature processing enables the use of highly heat-resistant polymers while maintaining ease of manufacture.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention utilizes phase separation between two polymer solutions with different solubility parameters. By controlling the phase separation process and using a poor solvent to precipitate polymer A, the system achieves narrow particle diameter distribution while maintaining the heat resistance of the crystalline polymer.

Inventive Principle:
Principle #36Phase transitions

3Device complexity

If conventional emulsion formation process is used for highly heat-resistant polymer, then the process is simple, but the particle diameter distribution becomes wider

Engineering Contradiction:
Improveproduction process simplicityVSAvoidparticle diameter distribution
Core Design Contradiction:
Device complexityVSManufacturing precision

Solution Approach 1:

The invention changes the temperature parameter during emulsion formation to 100°C or higher, which reduces the viscosity of the system and improves the particle diameter distribution. This parameter change maintains process simplicity while achieving narrow particle size distribution.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention utilizes phase separation between two polymer solutions with different solubility parameters. By controlling the phase separation process and using a poor solvent to precipitate polymer A, the system achieves narrow particle diameter distribution while maintaining the heat resistance of the crystalline polymer.

Inventive Principle:
Principle #36Phase transitions

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This process stabilizes the production of high-quality polymer microparticles with a narrow particle diameter distribution, suitable for applications like thin liquid crystal displays, by controlling the emulsion formation and precipitation conditions.

Implementation Method 1

a system which comprises a polymer (A), a polymer (B) and an organic solvent and can cause phase separation into two phases of a solution phase mainly composed of the polymer (A) and a solution phase mainly composed of the polymer (B)

Methodology Applied
Scientific EffectPhase separation: Phase Change

Implementation Method 2

the polymer (A) is precipitated by bringing a poor solvent for the polymer (A) into contact with the emulsion

Methodology Applied
Scientific EffectPrecipitation: Precipitation

Implementation Method 3

forming of the emulsion is carried out at a temperature of 100 °C or higher

Methodology Applied
Scientific EffectHeating: Heating

Implementation Method 4

the temperature at which said poor solvent is brought into contact with said emulsion for precipitating said polymer (A) after said emulsion is formed, is a temperature of a cooling crystallization temperature of said polymer (A) or higher

Methodology Applied
Scientific EffectCrystallization: Crystallisation

Data Source

PatentEP2623542B1Polymer microparticles and process for production thereof
Publication Date: 2017.05.24 TORAY INDUSTRIES INC
  • EP2623542B1 patent drawingFigure 1
  • EP2623542B1 patent drawingFigure 2(A)~2(B)
  • EP2623542B1 patent drawing

AI summary

A process for producing polymer microparticles, characterized in that, in a system which comprises a polymer (A), a polyvinyl alcohol group and an organic solvent and can cause the phase separation into two phases of a solution phase mainly composed of the polymer (A) and a solution phase mainly composed of the polyvinyl alcohol when the polymer (A), the polyvinyl alcohol group and the organic solvent are dissolved and mixed together, the polymer (A) is precipitated by heating the system at 100°C or higher to form an emulsion and thereafter bringing a poor solvent for the polymer (A) into contact with the emulsion; and polymer microparticles produced by the process. It becomes possible to produce microparticles of various types of polymers including a highly heat-resistant polymer stably at a high quality, and it becomes possible to produce microparticles having a small particle diameter distribution stably in a simple manner. Particularly, the microparticles of the present invention can be used as a material suitable for the concavo-convex formation on a reflector that is used in a thin liquid crystal display.