Continuous Polymer Particle Synthesis via Microchannel Mixing

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Solution Overview

Problem

Current batch processes for manufacturing polymer particles are inefficient, resulting in polydisperse particles with inconsistent physical properties, leading to high production costs and decreased productivity due to the difficulty in achieving monodispersity and homogeneous cross-linking.

Innovation Solution

A continuous dispersion polymerization method using a microchannel mixer connected to a tubular reactor with an aspect ratio of 100,000 or more, allowing for controlled dispersion polymerization with a linear speed of 0.5 m/min or more, and an additional reactor for further reaction, enabling the production of monodisperse polymer particles with desired properties.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If batch process is used for polymer particle manufacturing, then flexibility in synthesis conditions is maintained, but production time increases and productivity decreases

Engineering Contradiction:
Improveproduction timeVSAvoidprocess complexity
Core Design Contradiction:
ProductivityVSDevice complexity

Solution Approach 1:

The feedstock is pre-mixed in a microchannel mixer before entering the tubular reactor, ensuring homogeneous distribution of monomers and initiators. This preliminary mixing action enables continuous processing while maintaining uniform particle formation throughout the reaction, thereby increasing productivity without sacrificing process control

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The invention implements continuous flow polymerization in a tubular reactor with aspect ratio of 100 or more, where feedstock continuously flows through the reactor at controlled linear velocities (0.5-10 m/s). This continuous operation eliminates batch cycling, significantly reducing production time and increasing throughput while maintaining consistent particle properties

Inventive Principle:
Principle #20Continuity of useful action

2Manufacturing precision

If conventional polymerization process is used, then manufacturing cost is reduced, but particle monodispersity deteriorates

Engineering Contradiction:
Improveparticle size uniformityVSAvoidproduction efficiency
Core Design Contradiction:
Manufacturing precisionVSProductivity

Solution Approach 1:

The invention changes critical process parameters by using a tubular reactor with aspect ratio of 100 or more and maintaining linear flow velocities of 0.5-10 m/s. These parameter changes ensure sufficient residence time for complete polymerization while preventing particle aggregation, achieving monodisperse particles with narrow size distribution (PDI < 0.1) and high production efficiency simultaneously

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The continuous flow system utilizes hydraulic principles to maintain laminar flow regime in the tubular reactor, ensuring uniform shear distribution and consistent particle formation. The controlled flow dynamics prevent particle aggregation and enable efficient heat and mass transfer, achieving both high precision particle synthesis and improved productivity

Inventive Principle:
Principle #29Pneumatics and hydraulics

3Manufacturing precision

If batch process with multiple steps is used, then particle properties can be adjusted, but manufacturing cost increases

Engineering Contradiction:
Improvecross-linking uniformityVSAvoidmanufacturing cost
Core Design Contradiction:
Manufacturing precisionVSEase of manufacture

Solution Approach 1:

The continuous process is segmented into distinct functional zones within the tubular reactor: mixing zone, polymerization zone, and cross-linking zone. This spatial segmentation allows different reactions to occur simultaneously under optimized conditions for each zone, achieving uniform cross-linking and desired particle properties in a single continuous operation, thereby reducing manufacturing cost compared to sequential batch steps

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The tubular reactor design serves multiple functions: it acts as a mixing chamber, polymerization reactor, and cross-linking vessel simultaneously. This multi-functionality eliminates the need for separate batch processing steps, reducing equipment requirements, labor costs, and manufacturing complexity while maintaining precise control over particle properties and cross-linking uniformity

Inventive Principle:
Principle #6Universality (Multi-functionality)

4Manufacturing precision

If separation and dispersion steps are added to achieve monodispersity, then particle quality improves, but productivity decreases and cost increases

Engineering Contradiction:
Improveparticle monodispersityVSAvoidoverall production rate
Core Design Contradiction:
Manufacturing precisionVSProductivity

Solution Approach 1:

The microchannel mixer performs preliminary homogenization of the feedstock before polymerization, ensuring uniform distribution of all components. This preliminary action prevents particle aggregation during the reaction, producing monodisperse particles directly from the continuous process without requiring subsequent separation or ultrasonification steps, thereby maintaining high productivity

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The continuous flow process maintains constant shear rates and residence times throughout the reactor, ensuring uniform particle formation and preventing aggregation. This continuous action produces particles with narrow size distribution directly, eliminating the need for post-processing separation steps and maintaining high overall production rates

Inventive Principle:
Principle #20Continuity of useful action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This method effectively produces polymer particles with excellent monodispersity, controlled particle diameter, and uniform cross-linking, allowing for reproducible and customizable polymer properties, such as core-shell structures, while reducing production time and costs.

Implementation Method 1

a feedstock mixing device that is a microchannel mixer

Methodology Applied
Scientific EffectTurbulence: Turbulence

Implementation Method 2

mixing the feedstock in said mixing device

Methodology Applied
Scientific EffectMass transfer: Diffusion

Implementation Method 3

carrying out the dispersion polymerization of a mixture fed from the mixing device

Methodology Applied
Scientific EffectPolymerization: Photopolymerisation

Implementation Method 4

dispersion polymerization method for manufacturing polymer particles

Methodology Applied
Scientific EffectFree radical reaction: Chemical Bonding

Implementation Method 5

a linear speed of the mixture is maintained at 0.5 m/min or more in said reactor

Methodology Applied
Scientific EffectLaminar flow: Laminar Flow

Implementation Method 6

a tubular reactor for the dispersion polymerization that has an aspect ratio of 100,000 or more

Methodology Applied
Scientific EffectResidence time:

Data Source

PatentEP2357036B1Method and apparatus for manufacturing polymer particle
Publication Date: 2017.09.27 LG CHEM LTD
  • EP2357036B1 patent drawingFigure 1
  • EP2357036B1 patent drawingFigure 2
  • EP2357036B1 patent drawingFigure 3

AI summary

[Summary] The present invention relates to an apparatus for manufacturing polymer particles and a method for manufacturing the same. The present invention provides an apparatus and a method, by which polymer particles having excellent monodispersity and homogeneous physical properties, such as homogeneous cross-linking degree and polymerization degree, may be efficiently prepared. In the present invention, particles having excellent monodispersity with the desired particle diameter, and also having a high cross-linking degree or a core-shell or core-double shell structure may also be effectively prepared. In addition, the processes for manufacturing said polymer particles are exceptionally reproducible in the present invention. Additionally, the present invention provides an apparatus which may effectively control particle diameter, shape, cross-linking degree, polymerization degree or structure, and the concentration of solid content in a polymer solution, and the like, depending on the intended purpose, and a method thereof.