Polymer Surface Plasma Treatment for Stable Adhesion at Line Speed

Resolve Bottlenecks,
Find Innovative Solutions
Generate Solutions

Solution Overview

Problem

Current surface treatment methods for polymer substrates, such as those used in packaging and insulation, face challenges including high energy consumption, equipment costs, limited compatibility with materials like thermosensitive films, and unsatisfactory surface energy and aging issues, particularly with polypropylene.

Innovation Solution

A surface treatment process using an electric discharge with a dielectric barrier in a gas mixture containing a carrier gas and a mono-unsaturated or poly-unsaturated hydrocarbon, with minimal oxygen content, allowing for efficient surface functionalization and adhesion without the need for glues, enabling higher processing speeds and broader material compatibility.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If low-pressure plasma surface treatment is used to introduce functional groups and improve adhesion, then surface properties are significantly improved, but the treatment cannot be performed in continuous mode and is incompatible with high production rates

Engineering Contradiction:
ImproveadhesionVSAvoidproduction rate
Core Design Contradiction:
ReliabilityVSProductivity

Solution Approach 1:

The invention changes the pressure parameter from reduced pressure to atmospheric pressure, enabling continuous processing while maintaining plasma treatment effectiveness. This allows the substrate to be treated in a single pass through the treatment zone without requiring vacuum conditions, thus achieving both good adhesion and high production rates.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention enables continuous treatment by eliminating the need for vacuum cycles. The substrate moves continuously through the atmospheric pressure plasma zone, receiving constant treatment without interruption, which matches the requirements of high-speed production lines.

Inventive Principle:
Principle #20Continuity of useful action

2Ease of operation

If corona treatment is used for surface treatment at atmospheric pressure, then processing is simplified, but surface energy values are too low and aging is unsatisfactory

Engineering Contradiction:
Improveprocessing simplicityVSAvoidsurface energy
Core Design Contradiction:
Ease of operationVSReliability

Solution Approach 1:

The invention introduces a dielectric barrier as an intermediary between the electrode and the substrate. This barrier modifies the discharge characteristics to produce a more effective plasma that can achieve high surface energy values while maintaining atmospheric pressure operation. The dielectric barrier prevents direct contact between the high-voltage electrode and substrate, enabling better control of the treatment process.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The invention changes the electrical parameters by using a dielectric barrier with specific properties (material, thickness) to modify the discharge mode. This transforms the simple corona discharge into a more complex but effective barrier discharge that produces higher surface energy and better resistance to aging.

Inventive Principle:
Principle #35Parameter changes

3Reliability

If electric discharge with dielectric barrier is used in atmosphere with silane and oxidizing gas, then excellent surface properties are achieved, but additional costs are incurred

Engineering Contradiction:
Improvesurface propertiesVSAvoidcost
Core Design Contradiction:
ReliabilityVSQuantity of substance

Solution Approach 1:

The invention extracts and eliminates the silane component from the gas mixture, retaining only the oxidizing gas (oxygen or air). The research demonstrates that silane is not essential for achieving good surface properties, and its removal significantly reduces costs while maintaining treatment effectiveness.

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The invention changes the chemical composition parameters of the treatment atmosphere by replacing the complex silane-oxidizing gas mixture with a simpler oxidizing gas atmosphere. This parameter change maintains the plasma's ability to introduce functional groups while eliminating the need for expensive silane additives.

Inventive Principle:
Principle #35Parameter changes

4Reliability

If high power is used to treat large surfaces at atmospheric pressure, then treatment effectiveness is improved, but heat-sensitive films are damaged

Engineering Contradiction:
Improvetreatment effectivenessVSAvoidthermal damage
Core Design Contradiction:
ReliabilityVSTemperature

Solution Approach 1:

The dielectric barrier performs a preliminary function of distributing and moderating the electrical energy before it reaches the substrate. This preliminary action prevents concentrated thermal spots and distributes the energy more evenly, reducing the risk of thermal damage to heat-sensitive materials while maintaining treatment effectiveness.

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The dielectric barrier acts as a thermal intermediary that decouples the electrical energy input from direct thermal transfer to the substrate. It allows the plasma to be generated at atmospheric pressure with high power while preventing excessive heat from being transferred to the substrate, thus protecting heat-sensitive films.

Inventive Principle:
Principle #24Intermediary (Mediator)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This process achieves stable surface energy levels suitable for wettability and adhesion, reduces energy consumption, and expands the range of treatable materials, including thermosensitive films, while minimizing equipment costs and thermal effects.

Implementation Method 1

the substrate is subjected to an electric discharge with a dielectric barrier, in a gaseous treatment mixture comprising at least one carrier gas and an active gas

Methodology Applied
Scientific EffectElectric discharge: Electric Arc

Implementation Method 2

electric discharge with a dielectric barrier in a gas mixture containing a carrier gas and a mono-unsaturated or poly-unsaturated hydrocarbon

Methodology Applied
Scientific EffectPlasma: Plasma

Implementation Method 3

surface functionalization and adhesion without the need for glues

Methodology Applied
Scientific EffectGrafting: Chemical Bonding

Implementation Method 4

enabling higher processing speeds and broader material compatibility... minimizing equipment costs and thermal effects

Methodology Applied
Scientific EffectThermal conduction: Conduction (thermal)

Data Source

PatentEP2111332B1Method for processing the surface of polymer substrates, substrates thus obtained and use thereof in the production of multilayered materials
Publication Date: 2013.07.10 LAIR LIQUIDE SA POUR LETUDE & LEXPLOITATION DES PROCEDES GEORGES CLAUDE
  • EP2111332B1 patent drawingFigure 1~2

AI summary

The invention relates to a method for processing the surface of polymer substrates, during which the substrate is subjected to a dielectric-barrier electric discharge of the filament type in a gaseous processing mixture containing at least a carrier gas and an active gas and under a pressure substantially equal to the atmospheric pressure, characterised in that the active gas is selected from the group including a mono-unsaturated or poly-unsaturated linear or branched hydrocarbon preferably containing 2 to 10 carbon atoms, more preferably 2 to 5 carbon atoms and even more preferably 2 or 3 carbon atoms, the residual oxygen content of the processing mixture being lower than 250 ppm, preferably lower than 100 ppm, and more preferably lower than 50 ppm.