Polymer Polyol Preparation via Seed Polymerization with Heel

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Solution Overview

Problem

Existing methods for producing polymer polyols struggle to achieve a balance between high solid content and low viscosity, which is essential for efficient handling and optimal properties in flexible polyurethane foams, often requiring complex combinations of continuous and semi-batch operations.

Innovation Solution

A batch or semi-batch process involving the use of a seed polymerized in a base polyol with a polymer polyol heel, along with additional ethylenically unsaturated monomers and a macromer, to achieve a broad particle size distribution and low viscosity at high solids content.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Quantity of substance

If high solid polymer content is achieved in polymer polyol, then the polymer content increases, but the viscosity increases making handling difficult

Engineering Contradiction:
Improvesolid polymer contentVSAvoidease of handling
Core Design Contradiction:
Quantity of substanceVSEase of operation

Solution Approach 1:

The patent changes the particle size distribution parameters of the polymer to achieve a broad distribution with specific mean particle sizes (0.1-10 micrometers). This parameter change allows high solid content while maintaining low viscosity because the broad distribution prevents excessive chain entanglement that would occur with narrow distributions at high concentrations.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite polymer polyol system combining polymer particles dispersed in a polyol base. The composite structure consists of solid polymer particles (0.1-10 micrometers) distributed within a liquid polyol matrix, achieving both high solid content and low viscosity through the specific composite architecture.

Inventive Principle:
Principle #40Composite materials

2Stability of the object's composition

If narrow particle size distribution is used, then the polymer polyol has uniform properties, but the cell opening is limited and crushing force increases

Engineering Contradiction:
Improveparticle size distribution uniformityVSAvoidcrushing force
Core Design Contradiction:
Stability of the object's compositionVSStrength

Solution Approach 1:

Instead of using a narrow particle size distribution (conventional approach), the patent inverts the approach by using a broad particle size distribution. This inversion leads to improved cell opening and reduced crushing force, as the broader distribution allows for better foam cell formation and weaker cell walls that crush more easily.

Inventive Principle:
Principle #13The other way round (Inversion)

3Productivity

If continuous process is used for polymer polyol preparation, then production efficiency increases, but equipment complexity increases requiring both continuous and semi-batch equipment

Engineering Contradiction:
Improveproduction efficiencyVSAvoidequipment complexity
Core Design Contradiction:
ProductivityVSDevice complexity

Solution Approach 1:

The patent segments the polymerization process into distinct stages: a seed polymerization stage followed by a main polymerization stage. This segmentation can be achieved in a single batch reactor or semi-batch reactor, eliminating the need for complex continuous processing equipment while maintaining high productivity through efficient process control.

Inventive Principle:
Principle #1Segmentation

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This process results in polymer polyols with improved cell opening and reduced crushing force, facilitating the production of flexible polyurethane foams with enhanced properties.

Implementation Method 1

polymerizing in a base polyol at least one ethylenically unsaturated monomer in the presence of a polymerization initiator

Methodology Applied
Scientific EffectPolymerization: Photopolymerisation

Data Source

PatentUS8017664B2Process for preparing polymer polyols
Publication Date: 2011.09.13 SHELL USA INC

AI summary

The invention relates to a process for the batch or semi-batch preparation of a polymer polyol, which process involves (1) preparing a seed by polymerizing in a base polyol at least one ethylenically unsaturated monomer in the presence of a polymerization initiator and macromer, and in the presence of from 0.5 to 50% wt of polymer polyol heel, based on amount of polymer present in the heel compared with total amount of polymer formed, (2) adding additional ethylenically unsaturated monomer to the seed obtained in step (1) and optionally additional polyol, and (3) polymerizing the mixture obtained in step (2).