Anionic Polymer-Treated Clay Liners for Chemical Resistance

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Solution Overview

Problem

Existing clayey barriers, such as compacted clay liners and geosynthetic clay liners, face challenges in long-term protection from chemical attacks by aggressive electrolyte solutions, leading to increased hydraulic conductivity and reduced effectiveness over time.

Innovation Solution

A method involving the use of anionic polymers, specifically sodium carboxymethyl cellulose, is applied to clay, where the clay is mixed with a polymer solution and then dehydrated to enhance adsorption, resulting in a dispersed structure with improved water adsorption capacity, swelling ability, and reduced hydraulic conductivity.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If clay is amended with organics (organobentonites) to resist pollutant transport, then sorption capacity for organic compounds increases 4-5 times, but hydraulic conductivity increases significantly

Engineering Contradiction:
Improveresistance to pollutant transportVSAvoidhydraulic conductivity
Core Design Contradiction:
ReliabilityVSQuantity of substance

Solution Approach 1:

The patent changes the chemical nature of the polymer amendment from organic (hydrophobic) to inorganic/polyelectrolyte (hydrophilic) type, fundamentally altering the interaction mechanism with clay and water to achieve both low hydraulic conductivity and pollutant resistance

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite material system combining clay with polyelectrolyte polymers, where the polymer-clay complex forms a new composite structure with properties distinct from either component alone, achieving simultaneous improvement in both hydraulic conductivity and pollutant resistance

Inventive Principle:
Principle #40Composite materials

2Reliability

If Multi-Swellable Bentonite (MSB) is used to activate osmotic swelling capacity, then swelling ability increases and hydraulic conductivity decreases one to two orders of magnitude, but after prolonged prehydration the hydraulic conductivity increases one order of magnitude due to release of PC

Engineering Contradiction:
Improveswelling ability and initial hydraulic conductivityVSAvoidlong-term hydraulic conductivity stability
Core Design Contradiction:
ReliabilityVSDuration of action of stationary object

Solution Approach 1:

The patent applies polyelectrolyte polymers to clay in advance to form a stable polymer-clay complex structure before exposure to aggressive solutions, preventing subsequent degradation and ensuring long-term performance stability

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The patent replaces the unstable Propylene Carbonate (PC) amendment with polyelectrolyte polymers that provide durable, long-lasting performance without the need for frequent replacement or reapplication

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

3Reliability

If clay is treated with anionic polymer and dehydrated to enhance adsorption, then water adsorption capacity and swelling ability improve, but the complexity of the treatment process increases

Engineering Contradiction:
Improvewater adsorption capacity and swelling abilityVSAvoidtreatment process complexity
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The patent utilizes the natural charge properties of anionic polymers and their affinity for clay surfaces, leveraging fundamental chemical interactions to achieve effective treatment through relatively simple processes without requiring complex equipment or multiple treatment stages

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The treated clay maintains low hydraulic conductivity and chemico-osmotic efficiency for an extended period, making it suitable for long-term use as a barrier, with hydraulic conductivity remaining low for at least 1000 days under laboratory conditions and potentially up to several thousand days in field applications.

Implementation Method 1

the clay is mixed with a polymer solution and then dehydrated to enhance adsorption

Methodology Applied
Scientific EffectAdsorption: Adsorption

Implementation Method 2

resulting in a dispersed structure with improved water adsorption capacity, swelling ability

Methodology Applied
Scientific EffectSwelling: Absorption (physical)

Implementation Method 3

The latter improved clays are surprisingly well, and for a long term, protected from chemical attack by aggressive electrolyte solutions present in, for example, sea water or waste liquids

Methodology Applied
Scientific EffectChemical resistance:

Data Source

PatentEP2608901B1Clayey barriers
Publication Date: 2020.06.03 UNIV GENT
  • EP2608901B1 patent drawingFigure 1~3
  • EP2608901B1 patent drawingFigure 4(a)~4(b)
  • EP2608901B1 patent drawingFigure 5~6

AI summary

The present invention relates to improved clayey barriers, such as compacted clay liners or geosynthetic clay liners, which can be used, among other uses, to isolate waste liquids from the environment. More in particular, the present invention relates to clay which is treated with an anionic polymer and is subsequently dehydrated before it is used as a barrier. The latter improved clays are surprisingly well, and for a long term, protected from chemical attack by aggressive electrolyte solutions present in, for example, sea water or waste liquids.