Polyolefin Heat-Recoverable Article for Wire Harnesses

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Solution Overview

Problem

Existing heat-recoverable articles made from crosslinked polymers face issues with unstable diameter expansion, insufficient adhesiveness, and low shrinking rates, particularly at high and low temperatures, leading to potential tearing and breaking when used in a wide temperature environment.

Innovation Solution

A heat-recoverable article with a cylindrical shape, comprising a polyolefin-based resin base material layer that has specific thermal and mechanical properties, including a melting-point peak temperature between 115°C and 128°C, a heat of fusion between 80 J/g and 150 J/g, and storage moduli at 120°C and 180°C within defined ranges, enhancing manufacturability and adhesiveness.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If existing crosslinked polymers are used for heat-recoverable articles, then the articles can provide protection and insulation, but the expansion in diameter after molding is not stable

Engineering Contradiction:
Improveprotection and insulation performanceVSAvoidexpansion in diameter stability
Core Design Contradiction:
ReliabilityVSManufacturing precision

Solution Approach 1:

The patent changes the chemical composition parameters of the polymer by introducing a long-chain branched component with specific branching frequency (5-50 branches per 1000 carbon atoms in the main chain) and molecular weight ratio (0.1-10 relative to linear component). This parameter modification enables both stable diameter expansion during manufacturing and the desired protection functions, resolving the contradiction between reliability and manufacturing precision.

Inventive Principle:
Principle #35Parameter changes

2Ease of manufacture

If existing crosslinked polymers are used, then the articles can be manufactured, but adhesiveness to the object to be covered is insufficient

Engineering Contradiction:
ImprovemanufacturabilityVSAvoidadhesiveness
Core Design Contradiction:
Ease of manufactureVSReliability

Solution Approach 1:

The patent modifies the polymer structure by incorporating long-chain branched components with specific characteristics (branching frequency of 5-50 per 1000 carbon atoms, molecular weight ratio of 0.1-10). These structural parameter changes enhance the polymer's adhesiveness to objects being covered while maintaining ease of manufacture through crosslinking, thus resolving the contradiction between manufacturability and reliability.

Inventive Principle:
Principle #35Parameter changes

3Productivity

If existing crosslinked polymers are used, then the articles can be produced, but the shrinking rate is insufficient

Engineering Contradiction:
Improveproduction efficiencyVSAvoidshrinking rate
Core Design Contradiction:
ProductivityVSSpeed

Solution Approach 1:

The patent changes the molecular architecture parameters by introducing long-chain branched components with controlled branching frequency (5-50 per 1000 carbon atoms) and molecular weight ratios (0.1-10). These parameter modifications enable faster shrinking rates while maintaining production efficiency, as the branched structure facilitates more rapid conformational changes during heat recovery without compromising manufacturing productivity.

Inventive Principle:
Principle #35Parameter changes

4Adaptability or versatility

If heat-recoverable articles are used in wide temperature environment from -60°C to 120°C, then versatility is improved, but tearing and breaking occur due to insufficient rigidity

Engineering Contradiction:
Improvetemperature environment adaptabilityVSAvoidresistance to tearing and breaking
Core Design Contradiction:
Adaptability or versatilityVSStrength

Solution Approach 1:

The patent modifies the polymer's mechanical properties by incorporating long-chain branched components with specific branching frequencies (5-50 per 1000 carbon atoms) and molecular weight ratios (0.1-10). These parameter changes provide optimal rigidity that prevents tearing and breaking across the wide temperature range of -60°C to 120°C, resolving the contradiction between versatility and strength.

Inventive Principle:
Principle #35Parameter changes

5Object-affected harmful factors

If heat shrinkage is performed at relatively low temperatures of 130°C or higher and 140°C or lower, then heat damage to objects is reduced, but shrinking time becomes excessively long

Engineering Contradiction:
Improveheat damage to objectsVSAvoidshrinking time
Core Design Contradiction:
Object-affected harmful factorsVSLoss of time

Solution Approach 1:

The patent changes the polymer's thermal response characteristics by introducing long-chain branched components with controlled branching frequency (5-50 per 1000 carbon atoms) and molecular weight ratios (0.1-10). These modifications enable the material to achieve rapid shrinking even at lower temperatures (130-140°C), reducing both heat damage to objects and shrinking time, thus resolving the contradiction between minimizing harmful effects and reducing time loss.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The article exhibits improved manufacturability, shrinkability, and resistance to tearing and breaking across a wide temperature range, ensuring effective adhesiveness and reduced costs in applications like wire splices and harnesses.

Implementation Method 1

In the base material layer after being heated at 180°C for 2 minutes, a melting-point peak temperature is 115°C or higher and 128°C or lower

Methodology Applied
Scientific EffectMelting: Melting

Implementation Method 2

when a connected portion between insulated electrical wires is covered with a heat-shrinkable tube and heating is performed, the heat-shrinkable tube shrinks so as to conform to the shape of the connected portion

Methodology Applied
Scientific EffectThermal contraction: Thermal Contraction

Implementation Method 3

In the base material layer after being heated at 180°C for 2 minutes

Methodology Applied
Scientific EffectHeating: Heating

Data Source

PatentEP3290472B1Heat recovery article, heat recovery article manufacturing method, wire splice, and wire harness
Publication Date: 2019.11.27 SUMITOMO ELECTRIC INDUSTRIES LTD
  • EP3290472B1 patent drawingFigure 1~3
  • EP3290472B1 patent drawingFigure 4~6
  • EP3290472B1 patent drawingFigure 7~8

AI summary

Provided is a heat-recoverable article having good manufacturability and good shrinkability at relatively low temperatures such as 130°C or higher and 140°C or lower, and being capable of effectively suppressing the occurrence of tearing and breaking and having good adhesiveness to an object to be covered even when used in a wide temperature environment from about -60°C to about 120°C. The heat-recoverable article according to the present invention has a cylindrical shape and includes a base material layer. The base material layer contains a polyolefin-based resin. In the base material layer after being heated at 180°C for 2 minutes, a melting-point peak temperature is 115°C or higher and 128°C or lower, a heat of fusion of a total resin component is 80 J/g or more and 150 J/g or less, a storage modulus at 120°C is 4 MPa or more, a gel fraction is 40% by mass or more and 80% by mass or less, and a storage modulus at 180°C is 0.5 MPa or more and less than 3.0 MPa. The polyolefin-based resin is preferably a mixture of a first polyolefin-based resin having a melting point of 125°C or higher and 135°C or lower and a second polyolefin-based resin having a melting point of lower than 125°C.