Polyolefin Laminate Adhesion via Low Density Polyethylene Blend

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Solution Overview

Problem

Propylene-α-olefin copolymers used in film applications suffer from low flexibility and stickiness at high temperatures, leading to processing issues such as wrinkles and poor optical quality during metallization, which are partially addressed by slip agents but result in reduced surface tension and organoleptic issues.

Innovation Solution

A polyolefin resin composition comprising a blend of 90-99.7wt% of a copolymer with 80-98wt% propylene and 2-20wt% α-olefin units, combined with 0.3-10wt% of polyethylene with a density of 870-920 kg/m³, adhered to a base layer, improving adhesion and film quality while maintaining surface tension for printing and metallization.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of operation

If slip agents are added to propylene-α-olefin copolymers to reduce stickiness during processing, then the risk of polymer sticking to rollers is reduced, but the surface tension of the film is reduced making printing or adhesion onto metallized surface much more difficult

Engineering Contradiction:
ImproveprocessabilityVSAvoidadhesion
Core Design Contradiction:
Ease of operationVSReliability

Solution Approach 1:

The invention changes the chemical composition parameters of the copolymer by controlling comonomer content (2-20wt% α-olefin) and propylene content (80-98wt%) to achieve the right balance between flexibility and surface tension retention, eliminating the need for slip agents

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention removes (extracts) the slip agents from the system entirely by designing a copolymer composition that inherently provides sufficient flexibility and processability without requiring external slip agents, thus preserving surface tension for good adhesion

Inventive Principle:
Principle #2Taking out (Extraction)

2Ease of operation

If high density polyethylene (density ≥ 940 kg/m³) is used in the blend to improve flexibility and reduce stickiness, then processing issues are reduced, but metal film adhesion and organoleptic properties deteriorate

Engineering Contradiction:
ImproveflexibilityVSAvoidmetal film adhesion
Core Design Contradiction:
Ease of operationVSReliability

Solution Approach 1:

The invention changes the density parameter of the polyethylene component from ≥940 kg/m³ (high density) to 870-920 kg/m³ (lower density), which provides better flexibility and metal film adhesion while maintaining processability

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention creates a composite resin composition blending propylene-α-olefin copolymer with lower density polyethylene (870-920 kg/m³) in specific ratios (90-99.7wt% copolymer, 0.3-10wt% polyethylene) to achieve synergistic effects of flexibility and adhesion

Inventive Principle:
Principle #40Composite materials

Data Source

PatentEP2694290B1Laminate comprising a polyolefin layer adhered to a base layer
Publication Date: 2016.07.20 INEOS EUROPE AG
  • EP2694290B1 patent drawingFigure 1
  • EP2694290B1 patent drawing

AI summary

A laminate is disclosed comprising a polyolefin layer of a composition comprising a blend of 90-99.7wt% of a copolymer of propylene and at least one a-olefin, and 0.3-10wt% of a polyethylene having a density of 940 kg/m3 or less, adhered to a base layer comprising a propylene homopolymer or a copolymer of propylene and up to 5wt% of C2-C10 alpha- olefin units other than propylene. The laminate may optionally be metallised.