Polyolefin-ROMP Composite Bonding for Consistent Adhesion

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Solution Overview

Problem

Existing methods for preparing articles with a polyolefin component and a polymer made by ring-opening metathesis polymerization of cyclic olefin monomers lack reliable and consistent adhesion, which is crucial for industrial applications.

Innovation Solution

A method involving pre-treating the polyolefin surface and applying a ring-opening metathesis polymerizable mixture with a catalyst, ensuring a viscosity of 1000 mPa·s at 30°C for more than 9 seconds, followed by curing, to achieve strong and consistent adhesion between the components, preferably through injection molding for high-quality results.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If a ring-opening metathesis polymerisable mixture is applied to bond a polyolefin component with a polymer component, then adhesion between the components is achieved, but the adhesion level is inconsistent and insufficient for industrial applications

Engineering Contradiction:
Improveadhesion consistencyVSAvoidadhesion strength
Core Design Contradiction:
ReliabilityVSStrength

Solution Approach 1:

The patent applies parameter changes by carefully controlling the viscosity of the ring-opening metathesis polymerisable mixture (maintaining >9 seconds at 1000 mPa·s at 30°C) and optimizing the catalyst system (molybdenum or tungsten-based) to achieve consistent and reliable adhesion between polyolefin and polymer components, transforming the unreliable bonding process into a controlled and predictable industrial operation

Inventive Principle:
Principle #35Parameter changes

2Strength

If the viscosity of the ring-opening metathesis polymerisable mixture is increased to improve adhesion, then bonding strength increases, but the working time and ease of application decrease

Engineering Contradiction:
Improveadhesion strengthVSAvoidapplication ease
Core Design Contradiction:
StrengthVSEase of operation

Solution Approach 1:

The patent optimizes the viscosity parameter of the ring-opening metathesis polymerisable mixture to maintain a balance between adhesion strength and workability. By specifying a viscosity range (>9 seconds at 1000 mPa·s at 30°C), the invention ensures sufficient flow and application ease while maintaining high adhesion strength upon curing

Inventive Principle:
Principle #35Parameter changes

3Reliability

If pre-treatment of the polyolefin surface is applied to improve adhesion, then bonding reliability increases, but the manufacturing complexity and time increase

Engineering Contradiction:
Improveadhesion reliabilityVSAvoidprocess complexity
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The patent applies preliminary action by implementing surface pre-treatment of the polyolefin component before applying the ring-opening metathesis polymerisable mixture. This pre-treatment (such as corona treatment, plasma treatment, or chemical etching) activates the polyolefin surface to improve subsequent adhesion reliability, ensuring consistent bonding in industrial applications

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method provides a consistently higher level of adhesion between the polyolefin and the polymerized component, ensuring cohesive failure rather than adhesive failure, and enhances the article's ability to withstand high water pressures.

Implementation Method 1

a second component of a polymer made by ring-opening metathesis polymerisation of cyclic olefin monomers

Methodology Applied
Scientific EffectRing-opening metathesis polymerisation: Chemical Bonding

Implementation Method 2

applying a ring-opening metathesis polymerisable mixture of cyclic olefin monomers and a catalyst to the surface

Methodology Applied
Scientific EffectCatalysis: Catalysis

Data Source

PatentUS11155010B2Method for preparing a two-component article and article obtainable by the method
Publication Date: 2021.10.26 TELENE SAS

AI summary

A method for preparing an article includes at least a first component of a polyolefin in conjunction with a second component of a polymer made by ring-opening metathesis polymerisation of norbornene type monomers. The method includes pre-treating a surface of the first component, applying a ring-opening metathesis polymerisable mixture of norbornene type monomers and a catalyst to the surface, and curing the ring-opening metathesis polymerisable mixture in contact with the surface, wherein the ring-opening metathesis polymerisable mixture has a η1000 at 30° C. of more than 9 sec. Articles such as a pipe line field joint or a protective element for a concrete tunnel lining element can be made using the method.