Polyolefin Composition for 3D Printing Shrinkage Control

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Solution Overview

Problem

Conventional polyolefins used in additive manufacturing exhibit significant physical distortions such as shrinkage, warpage, and curling during the layer deposition process, limiting their application in 3D printing.

Innovation Solution

Development of a heterophasic copolymer composition with a propylene-based matrix phase and an ethylene-based dispersed phase, featuring rapid crystallization kinetics and a distinct composition, which reduces unidimensional shrinkage and warpage, achieving isotropic shrinkage ratios between 0.8 to 1.2.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of manufacture

If conventional polyolefins are used in additive manufacturing, then material availability and ease of processing are improved, but physical distortions such as shrinkage, warpage, and curling increase

Engineering Contradiction:
Improveease of processingVSAvoiddimensional accuracy
Core Design Contradiction:
Ease of manufactureVSManufacturing precision

Solution Approach 1:

The patent modifies the crystallization parameters of polyolefin polymers by controlling crystallization temperature and time to achieve a crystallization half-time of less than 60 minutes. This parameter change reduces the degree of crystallinity and minimizes shrinkage and warpage during additive manufacturing, while maintaining ease of processing with conventional polyolefin materials

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite polymer system by blending polyolefin polymers with specific additives including nucleating agents and processing aids. This composite material approach modifies the crystallization behavior to reduce dimensional distortions while maintaining the base polyolefin's processability and material availability

Inventive Principle:
Principle #40Composite materials

2Manufacturing precision

If rapid crystallization is achieved in polyolefins, then manufacturing precision and dimensional stability are improved, but crystallization time increases

Engineering Contradiction:
Improvedimensional stabilityVSAvoidcrystallization time
Core Design Contradiction:
Manufacturing precisionVSLoss of time

Solution Approach 1:

The patent optimizes crystallization parameters by controlling temperature profiles and adding nucleating agents to achieve rapid crystallization with a half-time of less than 60 minutes. This creates an optimal balance where sufficient crystallization occurs to minimize shrinkage and warpage, while the process remains efficient for additive manufacturing applications

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The polymer composition significantly reduces physical distortions in 3D printed articles, achieving unidimensional shrinkage of less than 1.8% and low warpage, enhancing the reliability and accuracy of additive manufacturing processes.

Implementation Method 1

the matrix phase has a crystallization half-time of less than 60 minutes

Methodology Applied
Scientific EffectCrystallization: Crystallisation

Implementation Method 2

a heterophasic copolymer composition including: a matrix phase being a propylene-based polymer or copolymer; and a dispersed phase in the matrix phase

Methodology Applied
Scientific EffectPhase separation:

Data Source

PatentUS11680158B2Polyolefins having improved dimensional stability in three-dimensional printing, articles formed therefrom, and methods thereof
Publication Date: 2023.06.20 BRASKEM SA

AI summary

A polymer composition suitable for manufacturing of isotropic three-dimensional printed articles, the composition including: a matrix phase including a propylene-based polymer or copolymer; and a dispersed phase in the matrix phase, the dispersed phase including an ethylene-based copolymer having a C3-C12 comonomer, wherein the dispersed phase has a different composition than the matrix phase, wherein the matrix phase has a crystallization half-time of less than 60 minutes.