Polypropylene Solvent Recycling With Supercritical Purification

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Solution Overview

Problem

Existing recycling methods for polypropylene plastics are inefficient in removing impurities such as additives, colorants, and metals, leading to limited economic upgrading and high energy consumption.

Innovation Solution

A process involving dissolution of polypropylene plastics in a light hydrocarbon solvent at specific temperatures and pressures, followed by purification steps including insoluble matter separation, washing, extraction, and adsorption, culminating in a supercritical separation to obtain purified polypropylene with minimal impurities.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If mechanical recycling is used to sort and reuse plastic waste, then the purity of the polymer stream is improved, but the impurities trapped in the polymer matrix (additives, colorants, metals) are not sufficiently removed

Engineering Contradiction:
Improvepurity of polymer streamVSAvoidimpurities in polymer matrix
Core Design Contradiction:
Manufacturing precisionVSObject-generated harmful factors

Solution Approach 1:

The patent extracts impurities from the polymer matrix by dissolving the polymer in a solvent system, allowing impurities to be separated from the polymer solution through filtration and extraction steps, thereby removing trapped additives, colorants, and metals that mechanical sorting cannot eliminate

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The patent introduces a solvent system as an intermediary medium to facilitate the removal of impurities. The solvent dissolves the polymer while allowing impurities to be separated through various treatment steps, acting as a mediator between the polymer and impurities for effective removal

Inventive Principle:
Principle #24Intermediary (Mediator)

2Adaptability or versatility

If chemical recycling via pyrolysis is used to reform monomers, then the plastic waste can be converted into useful chemicals, but the energy consumption is high due to high temperature treatments

Engineering Contradiction:
Improveconversion of plastic waste to chemicalsVSAvoidenergy consumption
Core Design Contradiction:
Adaptability or versatilityVSUse of energy by moving object

Solution Approach 1:

The patent changes the operational parameters from high-temperature pyrolysis to lower-temperature dissolution conditions (around 25-50°C), fundamentally altering the energy requirements while achieving effective polymer degradation and impurity removal through solvent-based processes

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent replaces the thermal-mechanical pyrolysis process with a chemical dissolution approach using solvent systems, substituting high-temperature thermal energy with chemical interactions that occur at much lower temperatures, thereby reducing energy consumption

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

3Object-generated harmful factors

If dissolution and purification methods are used to treat plastic waste, then impurities can be removed from the polymer, but the process complexity and cost increase

Engineering Contradiction:
Improveimpurity removalVSAvoidprocess complexity
Core Design Contradiction:
Object-generated harmful factorsVSDevice complexity

Solution Approach 1:

The patent segments the purification process into distinct functional steps: dissolution, filtration of insoluble matter, extraction of soluble impurities, and solvent recovery. This segmentation allows each step to be optimized independently and facilitates easier implementation compared to single-step complex processes

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The patent implements solvent recovery and reuse mechanisms, discarding only the minimal amount of solvent needed for each cycle while recovering and reusing the bulk solvent. This reduces waste, lowers costs, and simplifies the overall process by eliminating the need for complete solvent disposal and replacement

Inventive Principle:
Principle #34Discarding and recovering

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process effectively recovers purified polypropylene with low impurity content, suitable for reuse in new plastic products, while reducing energy consumption and solvent use, thus enhancing economic viability and resource conservation.

Implementation Method 1

a dissolution step involving placing the plastic feedstock in contact with a dissolution solvent, comprising at least one hydrocarbon-based compound having a boiling point of between −15 and 100° C., at a dissolution temperature of between 150° C. and 250° C. and a dissolution pressure of between 1.0 and 18.0 MPa absolute, to obtain at least one crude polymer solution

Methodology Applied
Scientific EffectDissolution: Solvation

Implementation Method 2

c) a solvent-polymer separation step, using at least one supercritical separation section operated at a temperature of between 160 and 300° C. and at a pressure (Psupercritical) of between 2.7 and 10.0 MPa absolute, followed by at least one solvent recovery section

Methodology Applied
Scientific EffectSupercritical fluid extraction: Supercritical Fluid Extraction

Data Source

PatentUS20250367858A1Process for recycling used plastics based on polypropylene using a light hydrocarbon solvent
Publication Date: 2025.12.04 IFP ENERGIES NOUVELLES

AI summary

The present invention relates to a process for purifying a plastic feedstock comprising polypropylene, involving:a) dissolving the plastic feedstock in a dissolution solvent comprising a hydrocarbon-based compound having a boiling point of between −15° C. and 100° C., at a dissolution temperature of between 150° C. and 250° C., a dissolution pressure of between 1.0 and 18.0 MPa absolute, to obtain a crude polymer solution;b) purifying the crude polymer solution, comprising:b1) separation of the insoluble matter;b2) washing, with a dense solution;b3) extraction, with an extraction solvent; and/orb4) adsorption of the impurities; and thenc) solvent-polymer separation, using a supercritical separation section, at a temperature of between 160 and 300° C. and a pressure of between 2.7 and 10.0 MPa absolute, followed by at least one solvent recovery section, to obtain purified polypropylene.