Aqueous Polyurethane Dispersion with Durable Low Gloss

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Solution Overview

Problem

Existing polyurethane dispersions used for coatings tend to lose their matte aspect when exposed to heat and light, and the addition of matting particles can destabilize polymer compositions and pose health risks due to the use of silica particles.

Innovation Solution

Aqueous polyurethane dispersions are synthesized using polycarbonate diols with a limited amount of other diols, stabilized with an acrylic thickener and a surfactant having a specific HLB, and chain extended in water without organic solvents, achieving a durable low-gloss finish without external matting additives.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Illumination intensity

If matting particles (silica or polymer) are added to polyurethane dispersions to increase matt effect, then the gloss is reduced, but the composition becomes destabilized and the film becomes more brittle

Engineering Contradiction:
ImproveglossVSAvoidcomposition stability
Core Design Contradiction:
Illumination intensityVSStability of the object's composition

Solution Approach 1:

The invention extracts and eliminates the need for external matting particles by incorporating matting functionality directly into the polyurethane polymer structure itself through specific diol components, thereby removing the destabilizing element while maintaining the desired low gloss effect

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The invention merges the matting function with the polyurethane polymer structure by incorporating specific diol components (such as poly(tetramethylene glycol) or polyester diols) that inherently provide both structural integrity and matting properties, creating a unified material that achieves low gloss without external additives

Inventive Principle:
Principle #5Merging (Combining)

2Illumination intensity

If heterogeneous matting particles are added to achieve low gloss, then the matt effect is improved, but separation of materials occurs during application causing heterogeneity of optical effect

Engineering Contradiction:
ImproveglossVSAvoidhomogeneity
Core Design Contradiction:
Illumination intensityVSStability of the object's composition

Solution Approach 1:

The invention applies local quality by making the matting property an intrinsic characteristic of the polyurethane polymer chains themselves through specific diol incorporation, ensuring uniform distribution and consistent optical effect throughout the entire coating without localized variations

Inventive Principle:
Principle #3Local quality

Solution Approach 2:

The invention achieves homogeneity by integrating matting functionality into the polymer structure at the molecular level, ensuring that the low gloss effect is uniformly distributed throughout the entire coating composition rather than being present as separate heterogeneous particles

Inventive Principle:
Principle #33Homogeneity

3Illumination intensity

If amorphous or crystalline silica is used to increase matt effect, then the gloss is reduced, but health risks are created due to pulmonary disease risks from fine particle exposure

Engineering Contradiction:
ImproveglossVSAvoidhealth risk
Core Design Contradiction:
Illumination intensityVSObject-affected harmful factors

Solution Approach 1:

The invention extracts and removes hazardous silica particles from the formulation entirely, replacing them with safe polymeric matting agents that provide the same low gloss effect without any health risks associated with fine particle inhalation

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The invention converts the harmful silica particles into beneficial polymeric matting agents that provide the desired optical effect while eliminating health risks, effectively transforming a hazardous approach into a safe and effective solution

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

4Illumination intensity

If polyglycol ether polyurethanes are used to achieve low gloss and soft touch, then the initial matt aspect is obtained, but the matt aspect is lost when exposed to ambient heat and light

Engineering Contradiction:
ImproveglossVSAvoiddurability of matt aspect
Core Design Contradiction:
Illumination intensityVSDuration of action of stationary object

Solution Approach 1:

The invention changes the chemical parameters of the polyurethane structure by incorporating specific diol components (such as poly(tetramethylene glycol) or polyester diols) that provide heat and light stability, thereby maintaining the low gloss effect under prolonged environmental exposure

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention creates a composite polyurethane structure combining different diol components with specific properties that confer both matting capability and environmental stability, resulting in a durable low gloss coating that maintains its appearance under heat and light exposure

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process results in stable, low-gloss coatings that maintain their matte appearance under heat and light exposure, eliminating the need for hazardous silica particles and ensuring a homogeneous, re-dispersible dispersion.

Implementation Method 1

stabilizing the dispersion with an acrylic thickener and a surfactant having HLB between 10 and 20

Methodology Applied
Scientific EffectStabilization:

Implementation Method 2

stabilizing the dispersion with an acrylic thickener and a surfactant having HLB between 10 and 20

Methodology Applied
Scientific EffectSurfactant action: Surfactant

Implementation Method 3

by using polycarbonate diols in the synthesis of the polyurethane... that, without the addition of matt additives, is able to give films with durable low gloss (matt aspect)

Methodology Applied
Scientific EffectHeat resistance:

Implementation Method 4

The resistance of matt to light exposure is particularly desirable in the field of leather (artificial or natural) for automotive interiors

Methodology Applied
Scientific EffectLight resistance:

Implementation Method 5

the prepolymer is chain extended in water in the presence of from 0.1 to 2% by weight, preferably from 0.3% to 1% by weight of a surfactant having HLB from 10 to 20

Methodology Applied
Scientific EffectChain extension:

Data Source

PatentUS11220571B2Aqueous polyurethane dispersions
Publication Date: 2022.01.11 LAMBERTI SPA

AI summary

Process for the preparation of aqueous polyurethane dispersions, containing from 20 to 50% by weight of an anionic polyurethane having a mean particle size from 1 to 15 micron and providing films with durable low gloss aspect.