Flexible Polyurethane Gel Coats for Epoxy Resins

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Solution Overview

Problem

Existing polyurethane gel coats for composite materials face issues such as short lamination times, poor adhesion to epoxy and vinyl ester resins, surface defects like sink marks, and limited weathering resistance, which restrict their use in high-temperature curing processes and applications requiring long-term stability.

Innovation Solution

A two-component composition comprising a polyol component with low and higher molecular weight polyols and light-resistant aromatic amines, combined with a polyisocyanate component, to produce flexible polyurethane gel coats that offer extended lamination times, improved adhesion, and enhanced weathering resistance, while maintaining mechanical stability and preventing surface defects.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Duration of action of moving object

If conventional polyurethane gel coats are used, then the gel coat provides a surface coating for composite materials, but the lamination time is too short to ensure adequate adhesion between synthetic resin and gel coat

Engineering Contradiction:
Improvelamination timeVSAvoidadhesion between synthetic resin and gel coat
Core Design Contradiction:
Duration of action of moving objectVSReliability

Solution Approach 1:

The patent changes the chemical parameters of the polyol component by selecting specific molecular weights (160-600 g/mol) and hydroxyl group concentrations (5 to less than 20 mol/kg), which optimizes the reaction kinetics to extend lamination time while maintaining adhesion reliability

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite gel coat system combining polyol component (A) with specific polyisocyanate component (B), where the synergistic interaction between components extends the working time while preserving bonding capability through controlled crosslinking density

Inventive Principle:
Principle #40Composite materials

2Ease of manufacture

If polyurethane gel coats are used for composite materials, then the gel coat can be applied as a surface coating, but adhesion to epoxy and vinyl ester resins is poor

Engineering Contradiction:
Improvesurface coating applicationVSAvoidadhesion to epoxy and vinyl ester resins
Core Design Contradiction:
Ease of manufactureVSReliability

Solution Approach 1:

The patent optimizes the hydroxyl group concentration parameter (5 to less than 20 mol/kg) and molecular weight parameters of the polyol to achieve balanced reactivity that ensures both ease of application and strong adhesion to epoxy and vinyl ester resins

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates different local properties within the gel coat system: the polyol component provides adhesion to the composite material substrate, while the polyisocyanate component provides crosslinking for surface durability, with each component optimized for its specific function

Inventive Principle:
Principle #3Local quality

3Shape

If gel coats are applied to composite material surfaces, then the surface appearance is improved, but surface defects like sink marks occur during high-temperature curing

Engineering Contradiction:
Improvesurface appearanceVSAvoidsurface defects
Core Design Contradiction:
ShapeVSManufacturing precision

Solution Approach 1:

The patent selects polyols with specific molecular weights (160-600 g/mol) and hydroxyl concentrations that provide optimal viscosity and reactivity balance, preventing sink marks during high-temperature curing while maintaining smooth surface appearance

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent formulates the gel coat with extended lamination time that allows the gel coat to fully adhere to the composite material before curing begins, cushioning against the development of surface defects like sink marks during subsequent high-temperature processing

Inventive Principle:
Principle #11Beforehand cushioning (Prior cushioning)

4Ease of manufacture

If conventional gel coats are used, then the gel coat provides surface coating functionality, but weathering resistance and long-term stability are limited

Engineering Contradiction:
Improvesurface coatingVSAvoidweathering resistance
Core Design Contradiction:
Ease of manufactureVSReliability

Solution Approach 1:

The patent creates a composite polyurethane system combining specific polyol and polyisocyanate components that work synergistically to provide both ease of application and superior weathering resistance through enhanced crosslinking density and chemical stability

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent optimizes the molecular weight and hydroxyl group concentration parameters to achieve a crosslinking density that provides long-term weathering stability and chemical resistance while maintaining the desired surface coating properties

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution provides gel coats with Shore D hardness greater than 65, elongation at break greater than 3%, and excellent adhesion to epoxy and vinyl ester resins, ensuring cohesive fracture within the synthetic resin laminate, and exhibits superior weathering and chemical resistance without reactive diluents or plasticizers, allowing for smooth surfaces and extended use temperatures.

Implementation Method 1

a two-component composition, which comprises a polyol component and a polyisocyanate component, for the production of flexible polyurethane gel coats

Methodology Applied
Scientific EffectPolymerization reaction: Chemical Bonding

Implementation Method 2

The layer obtained after gelling is sufficiently mechanically stable not to be damaged during the application of the synthetic resin

Methodology Applied
Scientific EffectCuring reaction: Chemical Bonding

Implementation Method 3

A3) one or more light-resistant aromatic amines

Methodology Applied
Scientific EffectUV absorption: Absorption (EM radiation)

Implementation Method 4

excellent adhesion to epoxy and vinyl ester resins, ensuring cohesive fracture within the synthetic resin laminate

Methodology Applied
Scientific EffectAdhesion: Adhesive

Data Source

PatentUS9067341B2Two-component composition for producing flexible polyurethane gel coats
Publication Date: 2015.06.30 MANKIEWICZ GEBR & CO GMBH & CO KG

AI summary

The invention relates to the use of a two-component composition comprising a polyol component and a polyisocyanate component, for producing flexible polyurethane gel coats for epoxy-resin and vinyl-ester resin composite materials.