Post-CMP Cleaning Liquid for CuO Removal and Re-Oxidation Control

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Solution Overview

Problem

Conventional cleaning solutions for semiconductor chips after chemical mechanical polishing (CMP) are inadequate in removing copper oxide (CuO) and prone to re-oxidation, leading to secondary contamination, reduced reliability of gate oxide layers, and increased circuit impedance due to CuO film formation during waiting times.

Innovation Solution

A post-CMP cleaning solution comprising 5-20 parts of a strong base, 5-30 parts of a weak base, 0.5-3 parts of a cellulose derivative, and 0.5-2 parts of a chitin derivative, which forms a monomolecular adsorbent layer to prevent re-oxidation and remove CuO, using renewable biomass derivatives to avoid petroleum-based additives.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If acidic cleaning solution is used to remove CuO, then cleaning effectiveness is improved, but copper substrate corrosion increases

Engineering Contradiction:
Improvecleaning effectivenessVSAvoidcopper substrate corrosion
Core Design Contradiction:
Manufacturing precisionVSObject-affected harmful factors

Solution Approach 1:

The patent changes the chemical parameters of the cleaning solution by using alkaline environment (pH 10-13) instead of acidic, and specifically controls the oxidation-reduction potential and composition ratios of different bases to achieve effective CuO removal while protecting copper substrate from corrosion

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The cleaning solution uses a composite formulation containing multiple components including strong base (5-20 parts), weak base (5-30 parts), cellulose derivative (0.5-3 parts), and chitin derivative (0.5-2 parts), where each component contributes different functions to achieve synergistic cleaning effect without substrate damage

Inventive Principle:
Principle #40Composite materials

2Loss of time

If wafer is left in O2-containing environment during waiting time, then process scheduling flexibility is improved, but re-oxidation of Cu2O occurs

Engineering Contradiction:
Improveprocess scheduling flexibilityVSAvoidre-oxidation resistance
Core Design Contradiction:
Loss of timeVSReliability

Solution Approach 1:

The cleaning solution applies preliminary protective action by forming a passivation layer on the copper surface during cleaning, which prevents or slows down subsequent re-oxidation of Cu2O to CuO during the waiting period, thereby extending the safe waiting time window

Inventive Principle:
Principle #9Preliminary anti-action

Solution Approach 2:

The cleaning solution creates a chemically inert environment on the copper surface through the formed protective layer, which acts as a barrier against oxygen diffusion and prevents re-oxidation reactions during the waiting time between CMP and deposition processes

Inventive Principle:
Principle #39Inert atmosphere (Inert environment)

3Device complexity

If conventional cleaning solution is used, then cleaning process simplicity is maintained, but secondary contamination occurs

Engineering Contradiction:
Improvecleaning process simplicityVSAvoidsecondary contamination
Core Design Contradiction:
Device complexityVSObject-generated harmful factors

Solution Approach 1:

The patent uses biodegradable natural polymers (cellulose and chitin derivatives) that break down easily and do not leave harmful residues, replacing conventional petroleum-based surfactants and cleaning agents that cause secondary contamination

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution effectively removes CuO, inhibits re-oxidation, and enhances the reliability of semiconductor devices by extending the process window, reducing circuit impedance, and improving electrostatic repulsion of contaminants.

Implementation Method 1

Acidic post-CMP cleaning solutions can dissolve CuO and Cu 2 O on the copper surface, and alkaline post-CMP cleaning solutions for semiconductor chips can selectively dissolve CuO

Methodology Applied
Scientific EffectChemical dissolution: Redox Reactions

Implementation Method 2

the chitin derivative generates a monomolecular adsorbent layer on the Cu surface, thereby effectively suppressing re-oxidation of the Cu surface within the waiting time

Methodology Applied
Scientific EffectAdsorption: Adsorption

Implementation Method 3

The cleaning solution provides an alkaline environment, which can improve electrostatic repulsion between particle contaminants and substrates

Methodology Applied
Scientific EffectElectrostatic repulsion: Electrostatics

Data Source

PatentEP4585673A1Cleaning liquid after chemical mechanical polishing for semiconductor chip, and preparation method for cleaning liquid and use of cleaning liquid
Publication Date: 2025.07.16 ZHEJIANG AUFIRST MATERIAL TECH CO LTD
  • EP4585673A1 patent drawingFigure 1~2
  • EP4585673A1 patent drawingFigure 3~4
  • EP4585673A1 patent drawingFigure 5

AI summary

A post-chemical mechanical polishing cleaning solution of semiconductor chips, a preparation method and use thereof are provided. The post-chemical mechanical polishing cleaning solution of semiconductor chips includes, parts by mass: 5-20 parts of a strong base; 5-30 parts of a weak base; 0.5-3 parts of a cellulose derivative; 0.5-2 parts of a chitin derivative; 70-95 parts of ultrapure water. The cellulose derivative is one or more of 2,5-furandicarboxylic acid, levulinic acid, and 5-aminolevulinic acid. The chitin derivative is one or more of chitosan oligosaccharide, carboxymethyl chitosan, N-acetyl glucose, glucosamine, and carboxymethyl glucosamine.