Proanthocyanidin Extraction Using Aqueous Ethanol and Polymeric Resin

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Solution Overview

Problem

Existing methods for producing high-titre proanthocyanidin extracts are not easily scalable due to the use of toxic solvents, extreme temperatures, and complex equipment like supercritical fluids or ultrafiltration membranes, limiting industrial feasibility.

Innovation Solution

A process involving the use of aqueous ethanol for extraction and purification of proanthocyanidins from cranberry fruits or prepurified extracts, utilizing a macroreticular aliphatic crosslinked polymeric resin with mild conditions and non-toxic solvents, followed by concentration and drying, to achieve high proanthocyanidin content without the drawbacks of prior art.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Quantity of substance

If prior art processes are used to obtain high-titre proanthocyanidin extracts, then proanthocyanidin content can reach 80-90%, but the processes are not easily realisable on an industrial scale due to toxic solvents, extreme temperatures, and complex equipment

Engineering Contradiction:
Improveproanthocyanidin contentVSAvoidindustrial scalability
Core Design Contradiction:
Quantity of substanceVSEase of manufacture

Solution Approach 1:

The patent changes the extraction parameters by using aqueous ethanol at room temperature instead of extreme temperatures and toxic solvents. The ethanol concentration (50-80% v/v) and extraction time (10 min to 2 hours) are optimized to achieve high proanthocyanidin extraction efficiency under mild conditions, making the process industrially scalable

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent extracts proanthocyanidins from cranberry fruit or prepurified extracts using aqueous ethanol, then purifies the extract through filtration and concentration. This selective extraction approach achieves high proanthocyanidin content (over 10%, preferably over 15%) without requiring the complex multi-step processes of prior art

Inventive Principle:
Principle #2Taking out (Extraction)

2Productivity

If supercritical fluids or ultrafiltration membranes are used, then extraction efficiency improves, but device complexity and equipment requirements increase

Engineering Contradiction:
Improveextraction efficiencyVSAvoidequipment complexity
Core Design Contradiction:
ProductivityVSDevice complexity

Solution Approach 1:

The patent uses simple, inexpensive materials such as macroreticular polymeric resins for filtration and standard vacuum concentration equipment. These replace complex supercritical fluid systems and ultrafiltration membranes, achieving comparable extraction efficiency with much simpler, more industrially feasible equipment

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Solution Approach 2:

The patent replaces complex mechanical systems (supercritical fluid extraction equipment, ultrafiltration membranes) with simpler chemical extraction using aqueous ethanol followed by vacuum concentration. This substitution maintains extraction efficiency while dramatically reducing equipment complexity

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

3Manufacturing precision

If multiple extraction steps with various organic solvents are used, then proanthocyanidin purity increases, but process complexity and time consumption increase

Engineering Contradiction:
Improveextract purityVSAvoidprocess complexity
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The patent combines extraction and purification into a single integrated process using aqueous ethanol. The extract is filtered through macroreticular polymeric resin and concentrated under vacuum in one continuous operation, achieving high proanthocyanidin purity without requiring multiple separate extraction steps with different solvents

Inventive Principle:
Principle #5Merging (Combining)

4Quantity of substance

If extraction is carried out for long periods at extreme temperatures, then extraction completeness improves, but energy consumption and process time increase

Engineering Contradiction:
Improveextraction completenessVSAvoidenergy consumption
Core Design Contradiction:
Quantity of substanceVSUse of energy by moving object

Solution Approach 1:

The patent changes the extraction parameters to room temperature and short duration (10 min to 2 hours) by using aqueous ethanol as the extraction solvent. This achieves complete proanthocyanidin extraction without the energy-intensive extreme temperature conditions required by prior art methods

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This process achieves proanthocyanidin extracts with over 10% content, preferably exceeding 15% and up to 20%, under mild conditions, making high-titre extracts more industrially viable and safe.

Implementation Method 1

Treating the crushed fruit containing high amounts in proanthocyanidins or an already prepurified extract rich in proanthocyanidins with aqueous ethanol

Methodology Applied
Scientific EffectSolvation: Solvation

Implementation Method 2

loading the solution on a macroreticular aliphatic crosslinked polymeric resin

Methodology Applied
Scientific EffectAdsorption: Adsorption

Implementation Method 3

washing with water said resin

Methodology Applied
Scientific EffectFiltration: Filter (physical)

Implementation Method 4

eluting the polymeric macroreticular aliphatic crosslinked resin coming from step (h) with aqueous ethanol

Methodology Applied
Scientific EffectDesorption: Desorption

Implementation Method 5

concentrating the eluted solution coming from the previous step under vacuum

Methodology Applied
Scientific EffectEvaporation: Evaporation

Implementation Method 6

drying the concentrated product coming from step (j) under vacuum

Methodology Applied
Scientific EffectEvaporation: Evaporation

Data Source

PatentEP2033641B1Process of preparation of extracts rich in proanthocyanidins
Publication Date: 2011.12.21 FERLUX
  • EP2033641B1 patent drawingFigure 1
  • EP2033641B1 patent drawingFigure 2
  • EP2033641B1 patent drawing

AI summary

The present invention relates to a process of preparation of extracts containing high amounts of proanthocyanidins involving the use as starting reactants of crushed fruits, plants or already prepurified extracts rich in proanthocyanidins.