Propionic Acid Separation from Acrylic Acid via Ion Exchange

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Solution Overview

Problem

Existing methods for producing acrylic acid from biobased or propane-based feedstocks often result in excessive propionic acid impurities, which are difficult and costly to remove, affecting the purity and yield of the final product.

Innovation Solution

A process combining chromatography and crystallization to separate and remove propionic acid from acrylic acid compositions, with optional hydrogenation or oxidative dehydrogenation of residual acrylic acid to enhance propionic acid production or purity.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If traditional distillation methods are used to separate propionic acid from acrylic acid, then separation can be achieved, but the process becomes costly and complex due to the similar boiling points of the two acids

Engineering Contradiction:
Improvepurity of acrylic acid productVSAvoidcomplexity of separation process
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The patent changes the separation parameter from thermal (distillation based on boiling point difference) to chemical (ion exchange based on acid strength differences). By using ion exchange resins that selectively bind propionic acid over acrylic acid, the process achieves effective separation without relying on the difficult-to-exploit boiling point difference between the two acids.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent introduces an ion exchange resin as an intermediary substance that mediates the separation process. The resin acts as a selective binder that temporarily holds propionic acid while allowing acrylic acid to pass through, enabling separation without direct thermal processing of the acid mixture.

Inventive Principle:
Principle #24Intermediary (Mediator)

2Productivity

If conventional oxidative processes are used to produce acrylic acid from propylene or propane, then production efficiency is maintained, but excessive propionic acid impurities are generated that are difficult and costly to remove

Engineering Contradiction:
Improveproduction efficiency of acrylic acidVSAvoidamount of propionic acid impurity
Core Design Contradiction:
ProductivityVSLoss of substance

Solution Approach 1:

The patent converts the harmful propionic acid impurity into a recoverable resource. By using ion exchange chromatography, propionic acid is selectively captured and can be desorbed in concentrated form for reuse or sale, transforming from a waste removal problem into a value recovery opportunity.

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Solution Approach 2:

The patent implements a recovery system where propionic acid is not simply discarded but captured by the ion exchange resin and then recovered through desorption. This allows the impurity to be separated, concentrated, and potentially reused in other processes or sold as a byproduct.

Inventive Principle:
Principle #34Discarding and recovering

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach effectively reduces propionic acid content in acrylic acid products, improving their purity and yield while minimizing the economic and environmental impacts associated with traditional separation methods.

Implementation Method 1

A process combining chromatography and crystallization to separate and remove propionic acid from acrylic acid compositions

Methodology Applied
Scientific EffectChromatography: Chromatography

Implementation Method 2

A process combining chromatography and crystallization to separate and remove propionic acid from acrylic acid compositions

Methodology Applied
Scientific EffectCrystallization: Crystallisation

Implementation Method 3

with optional hydrogenation or oxidative dehydrogenation of residual acrylic acid to enhance propionic acid production or purity

Methodology Applied
Scientific EffectHydrogenation: Hydrogenation

Implementation Method 4

with optional hydrogenation or oxidative dehydrogenation of residual acrylic acid to enhance propionic acid production or purity

Methodology Applied
Scientific EffectOxidation: Oxidation

Data Source

PatentEP3039006B1Separation of propionic acid from acrylic acid
Publication Date: 2018.10.24 ARCHER DANIELS MIDLAND CO
  • EP3039006B1 patent drawingFigure 1
  • EP3039006B1 patent drawingFigure 2~3
  • EP3039006B1 patent drawingFigure 4~5

AI summary

Methods are provided for producing a reduced propionic acid content acrylic acid product having a propionic acid content comparable to acrylic acid products from the conventional two stage oxidation of propylene, but wherein the acrylic acid has been produced by oxidation of propane, by dehydration of glycerol to an acrolein intermediate and oxidation of the acrolein intermediate to acrylic acid, by dehydration of lactic acid or one or more lactate esters or by any combination of these source processes and otherwise is characterized by having excess propionic acid compared to a glacial acrylic acid conventionally prepared from propylene.