Protease Variants with Targeted Substitutions for Liquid Detergent Stability

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Solution Overview

Problem

Existing proteases used in detergents and cleaning agents often lack sufficient catalytic activity and storage stability, particularly in liquid surfactant-containing preparations, leading to suboptimal cleaning performance on protease-sensitive soils.

Innovation Solution

A protease with an amino acid sequence that has at least 80% sequence identity to a specific sequence, featuring targeted substitutions at positions 9, 271, and additional positions such as 29, 48, 101, 130, 131, 133, 144, 224, and 252, enhancing storage stability and catalytic activity.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If proteases are used in liquid surfactant-containing preparations, then cleaning performance on protease-sensitive soils can be achieved, but the proteases exhibit insufficient storage stability and catalytic activity

Engineering Contradiction:
Improvestorage stabilityVSAvoidcatalytic activity
Core Design Contradiction:
ReliabilityVSProductivity

Solution Approach 1:

The patent applies parameter changes by modifying the amino acid sequence of the protease through site-directed mutagenesis. Specific amino acid substitutions at positions 9, 271, and other positions (29, 48, 101, 130, 131, 133, 144, 224, 252) are introduced to alter the enzyme's physical and chemical properties, thereby improving both storage stability and catalytic activity in liquid surfactant-containing preparations.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent applies local quality by making targeted local modifications to the protease structure through specific amino acid substitutions at defined positions. Rather than global changes, the invention focuses on localized sequence modifications at critical residues to optimize performance in liquid detergent formulations while maintaining overall enzyme functionality.

Inventive Principle:
Principle #3Local quality

2Productivity

If standard proteases are used in detergents, then protein-containing soils can be degraded, but the proteases lack sufficient catalytic performance under washing conditions

Engineering Contradiction:
Improvecatalytic performanceVSAvoidstorage stability
Core Design Contradiction:
ProductivityVSReliability

Solution Approach 1:

The patent applies parameter changes by systematically modifying amino acid parameters at specific positions to enhance catalytic performance. The substitutions at positions 9 (e.g., P9T, P9H, P9S, P9A), 271 (Q271E), and other positions are designed to optimize the enzyme's catalytic efficiency, substrate binding, and stability under washing conditions while maintaining storage stability.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent applies self-service by engineering the protease to be self-stabilizing through intrinsic structural modifications. The amino acid substitutions create an enzyme variant that inherently maintains its catalytic activity and structural integrity in liquid surfactant environments without requiring external stabilizers or protective measures.

Inventive Principle:
Principle #25Self-service

3Duration of action of stationary object

If proteases are stored in liquid formulations, then they can be used in cleaning agents, but they lose activity over extended storage periods

Engineering Contradiction:
Improvestorage periodVSAvoidproteolytic activity
Core Design Contradiction:
Duration of action of stationary objectVSProductivity

Solution Approach 1:

The patent applies preliminary action by pre-modifying the protease amino acid sequence before storage to prevent activity loss. The site-directed mutagenesis creates a stabilized enzyme variant that is pre-adapted to resist denaturation and maintain catalytic activity during extended storage in liquid formulations, eliminating the need for post-storage optimization.

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The patent applies beforehand cushioning by introducing amino acid substitutions that act as protective measures against storage-induced degradation. The modifications at critical positions create structural resilience that cushions the enzyme against denaturation, aggregation, and activity loss during long-term storage in liquid detergent preparations.

Inventive Principle:
Principle #11Beforehand cushioning (Prior cushioning)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The modified protease exhibits improved storage stability and catalytic activity, maintaining effective cleaning performance on protease-sensitive soils even after extended storage periods and varying temperatures.

Implementation Method 1

They act as nonspecific endopeptidases and hydrolyze any acid amide bonds found within peptides or proteins

Methodology Applied
Scientific EffectHydrolysis: Hydrolysis

Implementation Method 2

Proteases are among the most technically important enzymes of all. They degrade protein-containing soils on the items being cleaned

Methodology Applied
Scientific EffectEnzyme catalysis: Enzyme

Data Source

PatentEP3679131B1Performance-enhanced protease variants ii
Publication Date: 2024.09.04 HENKEL KGAA

AI summary

The invention relates to proteases comprising an amino acid sequence which has at least 70% sequence identity to the amino acid sequence given in SEQ ID No.1 over its entire length, and (a) amino acid substitutions on the positions corresponding to the positions 9 and 271 relating in each case to the numbering according to SEQ ID No. 1, and (b) an amino acid substitution on at least one of the positions corresponding to the positions 29, 48, 101, 30, 131, 133, 144, 224 or 252, relating in each case to the numbering according to SEQ ID No.1. The invention also relates to the production and use thereof. Said type of proteases have a very good cleaning performance.