Pressure-Sensitive Adhesive Layer Surface Treatment for Bond Strength

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Solution Overview

Problem

Highly crosslinked polyacrylate adhesives used in self-adhesive tapes face challenges in achieving adequate adhesion and shear strength, particularly in viscoelastic unsupported tapes, where cohesion and adhesion properties often lead to compromises, and existing methods for enhancing bond strength are complex and prone to delamination issues.

Innovation Solution

A method involving physical treatment, such as plasma or corona discharge, is applied to both surfaces of the pressure-sensitive adhesive (PSA) layer, with the substrate also being pretreated, to create unequal bond strengths and enhance adhesive strength without additional lamination, allowing for cohesive failure instead of adhesive failure during peel tests.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Strength

If highly cross-linked polyacrylate adhesives are used to achieve high shear strength and cohesion, then adhesive strength is improved, but adhesion to substrate deteriorates due to insufficient flowability and wetting

Engineering Contradiction:
Improveshear strengthVSAvoidadhesion to substrate
Core Design Contradiction:
StrengthVSEase of manufacture

Solution Approach 1:

The patent applies different cross-linking densities to different regions of the adhesive layer. The layer is designed with a gradient structure where the cross-linking density varies from the substrate interface to the surface, allowing optimal properties at each location. This resolves the contradiction by providing high cohesion where needed while maintaining adequate flowability and wetting at the substrate interface.

Inventive Principle:
Principle #3Local quality

Solution Approach 2:

The adhesive layer is segmented into multiple sub-layers with different cross-linking degrees. This segmentation allows each sub-layer to perform its specific function: lower cross-linked regions provide wetting and adhesion at the substrate interface, while higher cross-linked regions provide cohesion and shear strength in the bulk and surface regions.

Inventive Principle:
Principle #1Segmentation

2Duration of action of stationary object

If adhesive composition is optimized for high cohesion through cross-linking, then bond durability is improved, but initial tack and wetting ability deteriorate

Engineering Contradiction:
Improvebond durabilityVSAvoidinitial tack
Core Design Contradiction:
Duration of action of stationary objectVSEase of operation

Solution Approach 1:

The patent creates local quality differences within the adhesive layer by controlling cross-linking density spatially. Regions closer to the substrate have lower cross-linking to maintain initial tack and wetting ability, while regions farther from the substrate have higher cross-linking to provide durability and resistance to sustained loads.

Inventive Principle:
Principle #3Local quality

Solution Approach 2:

The adhesive layer is designed to exhibit dynamic behavior where the viscoelastic properties vary with depth. The gradient cross-linking structure allows the adhesive to display appropriate tackiness at the interface while maintaining elastic restoring forces in the bulk, resolving the contradiction between initial tack and long-term durability.

Inventive Principle:
Principle #15Dynamics

3Reliability

If adhesive layer is made thick to compensate for unevenness and provide durability, then bond reliability is improved, but transparency deteriorates

Engineering Contradiction:
Improvebond reliabilityVSAvoidtransparency
Core Design Contradiction:
ReliabilityVSIllumination intensity

Solution Approach 1:

The patent applies local quality variations through gradient cross-linking that extends through the entire thickness of the adhesive layer. This allows the layer to maintain adequate transparency while providing the necessary reliability through optimized cross-linking density at different depths, preventing the need for excessive thickness.

Inventive Principle:
Principle #3Local quality

Solution Approach 2:

The patent changes the cross-linking parameter continuously through the adhesive layer thickness. By controlling the cross-linking degree as a function of depth, the adhesive maintains transparency (avoiding excessive thickness) while achieving bond reliability through optimized cross-linking in the bulk region.

Inventive Principle:
Principle #35Parameter changes

4Strength

If physical treatment methods are applied to both surfaces to increase adhesive strength, then bond strength is improved, but process complexity increases

Engineering Contradiction:
Improveadhesive strengthVSAvoidprocess complexity
Core Design Contradiction:
StrengthVSDevice complexity

Solution Approach 1:

The patent combines the formation of the adhesive layer with the physical treatment process. The gradient cross-linking structure is created during the adhesive application and curing process itself, rather than requiring separate treatment steps. This merging of processes reduces overall process complexity while achieving the desired adhesive strength enhancement.

Inventive Principle:
Principle #5Merging (Combining)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach significantly increases bond strength by up to 58% on one side and 135% in ratio, achieving graded adhesive strengths without compromising shear strength, making it suitable for high-performance applications and reducing the need for additional lamination or primers.

Implementation Method 1

A method involving physical treatment, such as plasma or corona discharge, is applied to both surfaces of the pressure-sensitive adhesive (PSA) layer

Methodology Applied
Scientific EffectPlasma: Plasma

Implementation Method 2

A method involving physical treatment, such as plasma or corona discharge, is applied to both surfaces of the pressure-sensitive adhesive (PSA) layer

Methodology Applied
Scientific EffectCorona discharge: Corona Discharge

Implementation Method 3

the type of interaction is also important for adhesion, i.e., the specific interaction energy of the interfaces between the adhesive and the substrate

Methodology Applied
Scientific EffectSurface wetting: Wetting

Data Source

PatentEP2705102B1Method for increasing the adhesive properties of a pressure-sensitive adhesive layer having an upper and a lower surface
Publication Date: 2019.07.24 TESA SE

AI summary

Method for increasing the adhesive power of a pressure-sensitive adhesive layer having an upper and a lower surface, wherein at least one surface of the pressure-sensitive adhesive layer is subjected to a physical process, said physical process being selected from among the group comprising corona discharge, dielectric barrier discharge, preliminary flame treatment, or plasma treatment.