PTFE-SWCNT Electrode Binder for Low-Resistance Dry Batteries

Resolve Bottlenecks,
Find Innovative Solutions
Generate Solutions

Solution Overview

Problem

Conventional binders for lithium ion batteries face challenges in reducing electrode resistance and achieving high strength, often requiring solvents that increase costs and introduce moisture, which can degrade battery performance.

Innovation Solution

A binder composed of a mixed powder of polytetrafluoroethylene (PTFE) and single-walled carbon nanotubes, with specific properties such as a standard specific gravity of 2.11 to 2.20 and a G/D ratio of 2 or more, is used to create a fibrillated structure that acts as a binder, reducing moisture content and improving dispersibility, thereby enhancing electrode performance.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Strength

If conventional binders are used for lithium ion batteries, then the electrode can be formed, but the electrode resistance is high and strength is insufficient

Engineering Contradiction:
Improveelectrode strengthVSAvoidelectrode resistance
Core Design Contradiction:
StrengthVSReliability

Solution Approach 1:

The patent uses a composite binder system combining PTFE (polytetrafluoroethylene) with conductive carbon materials. This composite approach allows the binder to simultaneously provide mechanical strength through PTFE's fibrous structure and electrical conductivity through the carbon component, resolving the contradiction between strength and resistance.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent optimizes specific parameters of the PTFE binder including standard specific gravity (2.11 to 2.20), G/D ratio (2 or more for single-walled carbon nanotubes), and fibril diameter (20 nm or more). These parameter changes enable the binder to achieve both high strength and low resistance properties.

Inventive Principle:
Principle #35Parameter changes

2Ease of manufacture

If solvents are used in binder preparation, then the binder can be applied, but moisture is introduced that degrades battery performance

Engineering Contradiction:
Improvebinder applicationVSAvoidmoisture content
Core Design Contradiction:
Ease of manufactureVSObject-affected harmful factors

Solution Approach 1:

The patent extracts and eliminates the harmful solvent component from the binder system. By using a solvent-free PTFE-based binder composition, the invention removes the source of moisture while maintaining ease of manufacture through direct mixing and application of the binder components.

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The PTFE (polytetrafluoroethylene) material inherently provides a chemically inert environment that resists moisture absorption and degradation. This inert characteristic protects the battery components from moisture-related damage while allowing for practical manufacturing and application.

Inventive Principle:
Principle #39Inert atmosphere (Inert environment)

3Reliability

If single-walled carbon nanotubes are used as conductive material, then electrical conductivity improves, but dispersibility and homogeneity are difficult to achieve

Engineering Contradiction:
Improveelectrical conductivityVSAvoiddispersibility and homogeneity
Core Design Contradiction:
ReliabilityVSStability of the object's composition

Solution Approach 1:

The PTFE acts as an intermediary material that facilitates the uniform dispersion of single-walled carbon nanotubes. The fibrillated PTFE structure provides a matrix that distributes the carbon nanotubes homogeneously throughout the binder, preventing aggregation and ensuring stable composition while maintaining high electrical conductivity.

Inventive Principle:
Principle #24Intermediary (Mediator)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The binder effectively reduces electrical resistance and increases the strength of the electrode, improving battery performance by minimizing moisture contact with active materials and ensuring homogeneous distribution of single-walled carbon nanotubes, leading to higher energy density and reduced production costs.

Implementation Method 1

studies have been made on the use of a single-walled carbon nanotube as an electrically conductive material in a negative electrode

Methodology Applied
Scientific EffectElectrical conduction: Conduction (electrical)

Implementation Method 2

The electrode preferably has a polytetrafluoroethylene resin having a fibrous structure with a fibril diameter (median value) of 20 nm or more

Methodology Applied
Scientific EffectFibrillation:

Implementation Method 3

a binder including a mixed powder, the mixed powder including a polytetrafluoroethylene resin and a single-walled carbon nanotube

Methodology Applied
Scientific EffectAdhesion: Adhesive

Implementation Method 4

The method for producing a binder, including homogeneously mixing a PTFE dispersion and a single-walled carbon nanotube dispersion by using water as a dispersion solvent, followed by drying to form a mixed powder. The method for the drying is preferably spray drying.

Methodology Applied
Scientific EffectSpray drying:

Implementation Method 5

The binder preferably has a moisture content of 1,000 ppm or less

Methodology Applied
Scientific EffectMoisture absorption: Absorption (physical)

Data Source

PatentUS20230378471A1Binder that is composite of single-walled carbon nanotube and PTFE, and composition for producing electrode and secondary battery using same
Publication Date: 2023.11.23 DAIKIN INDUSTRIES LTD

AI summary

A binder containing a mixed powder including a polytetrafluoroethylene resin and a single-walled carbon nanotube. A weight ratio of the polytetrafluoroethylene resin to the single-walled carbon nanotube is 99.9:0.1 to 80:20. Also disclosed is a composition for producing an electrode in a form of a powder including the binder and an electrode active material substantially free of a liquid medium; an electrode mixture including the composition for producing an electrode; an electrode using the electrode mixture; a secondary battery having the electrode; a method for producing the binder; and a method for producing the electrode.