PVC Adhesive Sheet Preventing Plasticizer Migration

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Solution Overview

Problem

Conventional adhesive sheets using polyvinyl chloride suffer from migration of plasticizer, leading to decreased chip-holding ability in dicing and poor chip-exfoliating ability in picking-up processes.

Innovation Solution

An adhesive sheet with a polyvinyl chloride substrate and a specific adhesive composition containing (meth)acrylate copolymers and a polyester-based plasticizer, where the copolymers have distinct weight-average molecular weights and functional group-containing monomer units, along with a controlled cross-linking agent content, to prevent plasticizer migration and maintain adhesive performance over time.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If polyvinyl chloride is used as the substrate material, then the substrate provides good mechanical properties and processing performance, but plasticizer migration occurs over time causing deterioration of chip-holding ability and chip-exfoliating ability

Engineering Contradiction:
Improvechip-holding ability and chip-exfoliating abilityVSAvoidplasticizer migration
Core Design Contradiction:
ReliabilityVSStability of the object's composition

Solution Approach 1:

A silane coupling agent is introduced as an intermediary substance between the polyvinyl chloride substrate and the adhesive layer. The silane coupling agent contains both inorganic characteristics (for bonding to substrate) and organic characteristics (for compatibility with adhesive), thereby preventing plasticizer migration from the substrate to the adhesive layer while maintaining both chip-holding and chip-exfoliating abilities

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The substrate is formulated as a composite material combining polyvinyl chloride with silane coupling agent. This composite structure provides both the mechanical properties of PVC and the migration-preventing properties of silane, resolving the contradiction between mechanical performance and compositional stability

Inventive Principle:
Principle #40Composite materials

2Strength

If adhesive force increases with time, then bonding strength is improved, but chip-exfoliating ability deteriorates

Engineering Contradiction:
Improveadhesive forceVSAvoidchip-exfoliating ability
Core Design Contradiction:
StrengthVSReliability

Solution Approach 1:

The glass transition temperature of the adhesive is precisely controlled within -50°C to 0°C through selection of specific polymer components and ratios. This parameter control allows the adhesive to maintain optimal bonding strength while preventing excessive strength increase over time, thereby preserving chip-exfoliating ability

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

Different regions of the adhesive layer exhibit different properties: near the substrate, the adhesive provides strong bonding through controlled Tg, while the overall composition maintains lower cross-linking density to allow for future exfoliation. This spatial differentiation of adhesive properties resolves the contradiction between bonding strength and exfoliating ability

Inventive Principle:
Principle #3Local quality

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The adhesive sheet maintains chip-holding and chip-exfoliating abilities without deterioration, ensuring reliable performance in dicing and picking-up processes.

Implementation Method 1

a silane coupling agent which has both inorganic and organic characteristics and forms a cross-linked structure

Methodology Applied
Scientific EffectSilane cross-linking: Chemical Bonding

Data Source

PatentUS9422462B2Adhesive sheet
Publication Date: 2016.08.23 DENKA CO LTD

AI summary

An adhesive sheet of the invention includes a substrate and an adhesive composition laminated thereon, the substrate including polyvinyl chloride and a polyester-based plasticizer, wherein the adhesive composition includes two different (meth)acrylate copolymer components (A) and (B) in a mass ratio ranging from 10:90 to 90:10, wherein a content of a cross-linking agent which reacts with functional groups of the component (A) and the component (B) is in a range of 0.5 to 20 mass parts with respect to 100 mass parts of a sum of the component (A) and the component (B), and wherein 10 to 95 mass % of the monomer unit composing the component (A) is 2-ethylhexyl acrylate, and 10 to 95 mass % of the monomer unit composing the component (B) is butyl acrylate.