Cross-linked PVDF Polymer Actuator for Thermal Stability

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Solution Overview

Problem

Electrolyte polymer actuators face challenges with increased volume due to liquid electrolyte containment and unreliable sealing, while solid alternatives using acrylonitrile butadiene rubber and polypyrrole have limitations in thermal stability and chemical resistance.

Innovation Solution

A polymer actuator is developed using a cross-linked polyvinylidene fluoride (PVDF)-based polymer matrix with a conductive polymer and electrolytic material, featuring a fluorine-containing terpolymer structure that includes vinylidene fluoride, trifluoroethylene, and chlorotrifluoroethylene units, and employing a cross-linking agent to enhance thermal stability and chemical resistance, with electrodes made from conductive polymers like polypyrrole and poly(3,4-ethylenedioxythiophene).

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If liquid electrolyte is used in polymer actuators, then ionic conductivity is improved, but device volume increases and sealing reliability deteriorates

Engineering Contradiction:
Improveionic conductivityVSAvoidactuator volume
Core Design Contradiction:
ReliabilityVSVolume of stationary object

Solution Approach 1:

The patent changes the physical state of the electrolyte from liquid to solid by incorporating ionic liquid into the polymer matrix, achieving high ionic conductivity without requiring a containment chamber. This parameter change resolves the contradiction by eliminating the volume penalty and sealing issues associated with liquid electrolytes while maintaining excellent ionic conductivity.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite solid electrolyte by combining polymer matrix with ionic liquid, achieving synergistic properties. The composite structure provides both the mechanical integrity of solid polymers and the high ionic conductivity of ionic liquids, resolving the contradiction between conductivity and volume/sealing requirements.

Inventive Principle:
Principle #40Composite materials

2Volume of stationary object

If solid electrolyte polymers are used to reduce volume, then device volume is reduced, but thermal stability and chemical resistance deteriorate

Engineering Contradiction:
Improveactuator volumeVSAvoidthermal stability
Core Design Contradiction:
Volume of stationary objectVSStability of the object's composition

Solution Approach 1:

The patent employs a composite polymer-ionic liquid electrolyte system where the ionic liquid component provides exceptional thermal stability and chemical resistance. This composite approach allows the solid electrolyte to achieve both compact volume and superior compositional stability, overcoming the limitations of conventional solid polymer electrolytes.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent changes the chemical composition and structure of the solid electrolyte by incorporating ionic liquid functional groups, which fundamentally improves thermal and chemical stability parameters while maintaining the solid state and compact form factor.

Inventive Principle:
Principle #35Parameter changes

3Stability of the object's composition

If cross-linking is applied to PVDF-based polymer, then thermal stability and chemical resistance are improved, but manufacturing complexity increases

Engineering Contradiction:
Improvethermal stabilityVSAvoidmanufacturing simplicity
Core Design Contradiction:
Stability of the object's compositionVSEase of manufacture

Solution Approach 1:

The patent utilizes chemical cross-linking of PVDF-based polymer to fundamentally change the polymer network structure, creating a three-dimensional gel framework. This parameter change in molecular architecture provides exceptional thermal and chemical stability while the cross-linking process can be integrated into existing polymer processing methods.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a cross-linked polymer-ionic liquid composite gel electrolyte where the cross-linked network provides structural stability and thermal resistance, while the ionic liquid provides ionic conductivity. This composite cross-linked structure achieves superior performance while maintaining manufacturing feasibility through established cross-linking techniques.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution provides a polymer actuator with excellent thermal stability, chemical resistance, and low-voltage operation, achieving significant displacement and operational reliability.

Implementation Method 1

The PVDF-based polymer is cross-linked, preferably by a cross-linking agent

Methodology Applied
Scientific EffectCross-linking: Chemical Bonding

Implementation Method 2

a solid electrolyte polymer layer including a polyvinylidene fluoride (PVDF)-based polymer matrix and an electrolytic material

Methodology Applied
Scientific EffectIonic conduction: Conduction (electrical)

Implementation Method 3

a crosslinked fluorine-containing polymer is a crosslinked terpolymer comprising a vinylidene fluoride as a first structural unit, a fluorine-containing monomer as a second structural unit

Methodology Applied
Scientific EffectElectroresponsive effect: Electroactive Polymer

Data Source

PatentEP2202265B1Electrolyte polymer film, polymer actuator using cross-linked PVDF-based polymer, and method of manufacturing the polymer actuator
Publication Date: 2013.07.24 SAMSUNG ELECTRONICS CO LTD
  • EP2202265B1 patent drawingFigure 1~2
  • EP2202265B1 patent drawingFigure 3A~3B
  • EP2202265B1 patent drawingFigure 3C~3E

AI summary

An electrolyte polymer film including a cross-linked polyvinylidene fluoride (PVDF)-based polymer as the matrix and an electrolytic material dispersed in the matrix, and a polymer actuator including the cross-linked PVDF-based polymer film disposed between two electrodes of conductive polymer.