PVDF Fluoropolymer Film Tear Resistance via Core-Shell Modifiers

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Solution Overview

Problem

Greenhouse films made from fluoropolymers, such as PVDF, lack sufficient tear resistance, especially at low temperatures, while maintaining optical and chemical resistance properties.

Innovation Solution

Incorporating a core-shell type impact modifier into a polyvinylidene fluoride (PVDF) matrix to enhance tear resistance, with a mass rate of impact modifier between 2.5% and 40%, and using a multilayer film structure with modified and unmodified PVDF layers to achieve improved mechanical and optical properties.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Strength

If fluoropolymer films (PVDF or VDF/HFP copolymers) are used for greenhouse applications, then good mechanical, optical, and chemical resistance properties are achieved, but tear resistance is insufficient, especially in the direction of extrusion (MD)

Engineering Contradiction:
Improvetear resistanceVSAvoidmechanical performance in extrusion direction
Core Design Contradiction:
StrengthVSReliability

Solution Approach 1:

The patent applies composite materials by combining PVDF or VDF/HFP copolymer with elastomeric modifiers (such as polyethylene-graft-maleic anhydride, ethylene-propylene-diene monomer rubber, or butadiene-styrene rubber). This composite approach enhances tear resistance while preserving the inherent mechanical, optical, and chemical resistance properties of the fluoropolymer matrix, directly resolving the contradiction between maintaining reliability and improving strength.

Inventive Principle:
Principle #40Composite materials

2Strength

If multilayer fluorinated films with alternating copolymers of different crystallization temperatures are used, then tear resistance is significantly improved, but tear resistance remains insufficient at low temperature

Engineering Contradiction:
Improvetear resistanceVSAvoidlow temperature performance
Core Design Contradiction:
StrengthVSTemperature

Solution Approach 1:

The patent changes the chemical composition parameters by introducing elastomeric modifiers with specific glass transition temperatures and molecular structures. These modifiers remain flexible at low temperatures, allowing the film to maintain tear resistance in cold conditions while still benefiting from the improved tear strength provided by the multilayer or composite structure.

Inventive Principle:
Principle #35Parameter changes

3Strength

If impact modifiers are added to improve tear resistance, then mechanical properties are enhanced, but visible light transmission and fire resistance must be maintained

Engineering Contradiction:
Improvetear resistanceVSAvoidvisible light transmission
Core Design Contradiction:
StrengthVSIllumination intensity

Solution Approach 1:

The patent applies local quality by using elastomeric modifiers with specific properties (flexibility, compatibility) that are localized within the fluoropolymer matrix. These modifiers are selected to have refractive indices and optical properties similar to the base polymer, ensuring they enhance tear resistance locally without significantly affecting the overall visible light transmission of the film.

Inventive Principle:
Principle #3Local quality

Solution Approach 2:

The patent carefully controls the concentration of impact modifiers (typically 5-50 wt%) and selects modifiers with appropriate molecular weights and chemical structures to optimize the balance between mechanical enhancement and optical property preservation, while also maintaining fire resistance characteristics of the fluoropolymer.

Inventive Principle:
Principle #35Parameter changes

Data Source

PatentEP2988934B1Fluorpolymer film
Publication Date: 2019.10.30 ARKEMA FRANCE SA

AI summary

The present invention relates to a fluorinated film having properties that make it suitable for use outside, especially in the agricultural sector. The film according to the invention is a single-layer polymer film comprising a polyvinylidene fluoride (PVDF) matrix and at least one impact modifier having a polyorganosiloxane core and at least one thermoplastic shell, in which the weight content of impact modifier varies between 2.5% and less than 40%. According to one embodiment variant, the invention relates to multilayer films comprising at least one layer of said fluorinated film and at least one layer of unmodified PVDF.