Quantum Absorption Spectroscopy Using Entangled-Photon Interference

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Solution Overview

Problem

Existing spectroscopy systems struggle to achieve spectroscopy in a wide wavelength range, particularly when utilizing quantum entangled photon pairs, as they often require wavelength scanning and spectral dispersion, which can be time-consuming and costly.

Innovation Solution

A quantum absorption spectroscopy system and method that utilizes a quantum optical system with a nonlinear optical element to generate a quantum entangled photon pair, performs quantum interference, and calculates absorption spectroscopy characteristics through Fourier transforms without wavelength sweep, using a silicon-based photodetector and a phase converter to measure a wide wavelength range.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Measurement precision

If conventional spectroscopic measurement methods are used, then the system structure is relatively simple, but the measurement precision is insufficient for detecting low-concentration substances

Engineering Contradiction:
Improvedetection sensitivityVSAvoidsystem structure
Core Design Contradiction:
Measurement precisionVSDevice complexity

Solution Approach 1:

The system divides the measurement process into distinct functional modules: a quantum cascade laser source for generating mid-infrared radiation, an absorption cell for sample interaction, and a detector for signal measurement. This modular segmentation enables high detection sensitivity while maintaining manageable system complexity through standardized interfaces and independent optimization of each module.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The patent introduces a mid-infrared laser as an intermediary radiation source that bridges the gap between conventional light sources and the absorption characteristics of target molecules. This intermediary enables selective excitation of molecular vibrations in the fingerprint region, dramatically improving detection sensitivity for low-concentration substances without requiring complex sample preparation or measurement procedures.

Inventive Principle:
Principle #24Intermediary (Mediator)

2Productivity

If conventional spectroscopic methods are used, then the device complexity is low, but the productivity is insufficient due to long measurement times

Engineering Contradiction:
Improvemeasurement speedVSAvoidmeasurement time
Core Design Contradiction:
ProductivityVSLoss of time

Solution Approach 1:

The system employs periodic modulation of the laser source and synchronized detection to rapidly acquire spectral data. By using pulsed or modulated mid-infrared radiation and lock-in detection techniques, the system achieves high measurement speeds with improved signal-to-noise ratios, enabling rapid detection of low-concentration substances without requiring prolonged integration times.

Inventive Principle:
Principle #19Periodic action

3Measurement precision

If conventional light sources are used, then the energy consumption is moderate, but the measurement precision for low-concentration detection is insufficient

Engineering Contradiction:
Improvedetection limitVSAvoidlight source energy
Core Design Contradiction:
Measurement precisionVSUse of energy by moving object

Solution Approach 1:

The patent changes the fundamental parameter of the light source by transitioning from broadband thermal sources to quantum cascade lasers operating in the mid-infrared region. This parameter change enables resonant excitation of molecular vibrations, dramatically improving detection limits for low-concentration substances. The laser's coherent radiation and narrow linewidth provide high spectral resolution with efficient energy coupling to molecular transitions, achieving superior detection sensitivity with moderate energy consumption.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

Enables spectroscopy across a wide wavelength range from ultraviolet to far-infrared without the need for wavelength scanning, enhancing efficiency and reducing measurement time.

Implementation Method 1

a light source that is a quantum cascade laser

Methodology Applied
Scientific EffectQuantum cascade laser emission:

Implementation Method 2

Quantum absorption spectroscopy system and quantum absorption spectroscopy method

Methodology Applied
Scientific EffectAbsorption spectroscopy: Absorption Spectroscopy

Implementation Method 3

an optical filter; and a detector that detects light having passed through the optical filter

Methodology Applied
Scientific EffectOptical absorption filtering: Absorption (EM radiation)

Data Source

PatentEP4075110B1Quantum absorption spectroscopy system and quantum absorption spectroscopy method
Publication Date: 2026.05.06 KYOTO UNIV
  • EP4075110B1 patent drawingFigure 1
  • EP4075110B1 patent drawingFigure 2
  • EP4075110B1 patent drawingFigure 3

AI summary

A quantum absorption spectroscopy system (100) includes a laser light source (1), a quantum optical system (201), a photodetector (31), and a controller (4). The laser light source (1) emits pump light. The quantum optical system (201) includes a nonlinear optical crystal (23) that generates a quantum entangled photon pair of a signal photon and an idler photon by irradiation with pump light, and a moving mirror (25) that changes a phase of the idler photon, and causes quantum interference between a plurality of physical processes in which the quantum entangled photon pair is generated. The photodetector (31) detects the signal photon when the phase of the idler photon is changed by the nonlinear optical crystal (23) in a state where a sample is disposed on an optical path of the idler photon, and outputs a quantum interference signal corresponding to the detected number of photons. The controller (4) calculates an absorption spectroscopy characteristic of the sample by performing Fourier transform on the quantum interference signal.