Radialene OLED Charge Generation Layers for Voltage Stability

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Solution Overview

Problem

Existing organic electroluminescent devices face challenges in achieving improved operating voltage stability over time and current efficiency, particularly due to imbalances in hole and electron injection and transport.

Innovation Solution

Incorporating an intermediate layer with a radialene of formula (I) and a p-type charge generation layer containing a hole transport matrix compound, along with an n-type charge generation layer, to balance charge injection and transport, utilizing specific hole transport compounds like arylamine and triarylamine, and optimizing layer thickness and energy levels for enhanced performance.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If conventional organic electroluminescent devices are used, then basic light emission function is achieved, but operating voltage stability over time deteriorates

Engineering Contradiction:
Improveoperating voltage stabilityVSAvoidoperating time
Core Design Contradiction:
ReliabilityVSDuration of action of stationary object

Solution Approach 1:

The device is divided into multiple functional layers including n-type charge generation layer, intermediate layer, and p-type charge generation layer. Each layer performs specific functions to balance charge injection and transport, thereby stabilizing operating voltage over time while extending device operation duration.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

Different materials with specific properties are assigned to different layers. The n-type charge generation layer uses electron transport materials, the p-type charge generation layer uses hole transport materials, and the intermediate layer uses compounds with specific HOMO/LUMO levels. This local optimization of material properties balances charge injection and transport characteristics.

Inventive Principle:
Principle #3Local quality

2Productivity

If conventional charge injection and transport mechanisms are used, then device operation is achieved, but current efficiency deteriorates

Engineering Contradiction:
Improvecurrent efficiencyVSAvoidenergy loss
Core Design Contradiction:
ProductivityVSLoss of energy

Solution Approach 1:

The HOMO and LUMO energy levels of the intermediate layer are specifically optimized to be between the HOMO of the p-type charge generation layer and the LUMO of the n-type charge generation layer. This parameter optimization facilitates efficient charge transport and recombination, improving current efficiency while reducing energy loss.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The device employs composite material structures where the intermediate layer contains compounds with specific HOMO/LUMO levels, and the charge generation layers contain dopants. This composite approach enables balanced charge injection and transport, enhancing current efficiency.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution results in improved operating voltage stability and efficiency, surpassing the performance of conventional devices by stabilizing operating voltage over time and enhancing current efficiency.

Implementation Method 1

the at least one intermediate connecting region comprises an n-type charge generation layer, an intermediate layer, and a p-type charge generation layer

Methodology Applied
Scientific EffectCharge generation:

Implementation Method 2

holes injected from the anode move to the EML, via the HTL, and electrons injected from the cathode move to the EML, via the ETL

Methodology Applied
Scientific EffectCharge transport: Conduction (electrical)

Implementation Method 3

the p-type charge generation layer comprises a hole transport matrix compound and a radialene of formula (I)

Methodology Applied
Scientific EffectHole transport:

Implementation Method 4

The holes and electrons recombine in the EML to generate excitons. When the excitons drop from an excited state to a ground state, light is emitted

Methodology Applied
Scientific EffectElectroluminescence: Electroluminescence

Data Source

PatentEP4344390B1Organic electroluminescent device comprising a radialene of formula (i) and a compound of formula (II), and display device comprising the organic electroluminescent device
Publication Date: 2026.03.04 NOVALED GMBH
  • EP4344390B1 patent drawingFigure 1~2
  • EP4344390B1 patent drawingFigure 3
  • EP4344390B1 patent drawingFigure 4

AI summary

The present invention relates to an electroluminescent device comprising a radialene of formula (I) and a compound of formula (II), and a display device comprising the organic electroluminescent device.