Random Oligonucleotide Synthesis via Spatial Control and Enzymatic Processes

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Solution Overview

Problem

Current methods for synthesizing oligonucleotides require a known sequence, which is not efficient for generating large numbers of unique oligonucleotides with varying sequences, particularly for applications like molecular cryptography where exact sequences are not necessary.

Innovation Solution

The method involves synthesizing random oligonucleotides using phosphoramidite chemistry and enzymatic processes, with spatial control and microfluidic techniques to generate molecules of varying lengths, followed by sequence determination using real-time sequencing technologies, allowing for the production of unique, partially random oligonucleotides with desired characteristics.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If traditional precision synthesis methods are used to generate oligonucleotides, then sequence accuracy is improved, but the ability to generate large numbers of unique random sequences is limited

Engineering Contradiction:
Improvesequence accuracyVSAvoidnumber of unique oligonucleotides generated
Core Design Contradiction:
Manufacturing precisionVSProductivity

Solution Approach 1:

The synthesis process is divided into multiple cycles where oligonucleotides are grown to different lengths in separate reactions. Each cycle generates a population of oligos with controlled length distribution, allowing systematic exploration of sequence space while maintaining manufacturing precision through controlled enzymatic reactions

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The method dynamically adjusts reaction conditions including enzyme concentrations, nucleotide ratios, and incubation times to optimize both randomness and precision at different synthesis stages. The system adapts parameters based on desired oligonucleotide characteristics and production scale

Inventive Principle:
Principle #15Dynamics

2Loss of substance

If spatial control methods are used to minimize reagent use, then cost efficiency is improved, but process complexity increases

Engineering Contradiction:
Improvereagent consumptionVSAvoidspatial control system complexity
Core Design Contradiction:
Loss of substanceVSDevice complexity

Solution Approach 1:

The patent transitions from traditional bulk solution synthesis to spatially-resolved synthesis on solid supports or microfluidic arrays. This dimensional change enables precise localization of reagents to specific reaction sites, dramatically reducing overall reagent consumption while the modular nature of the spatial system manages complexity through standardization

Inventive Principle:
Principle #17Another dimension (Dimensionality change)

3Adaptability or versatility

If enzymatic processes are used to generate random sequences, then sequence randomness is improved, but control over exact sequence composition decreases

Engineering Contradiction:
Improvesequence randomnessVSAvoidsequence composition control
Core Design Contradiction:
Adaptability or versatilityVSManufacturing precision

Solution Approach 1:

The method incorporates feedback mechanisms where synthesis conditions are adjusted based on desired sequence properties. By controlling enzyme specificity, nucleotide availability, and reaction parameters, the system guides the stochastic enzymatic process to achieve both randomness and controlled composition characteristics

Inventive Principle:
Principle #23Feedback

Solution Approach 2:

The patent systematically varies key parameters including enzyme type and concentration, dNTP ratios, temperature, and pH to optimize the balance between randomness and compositional control. Different parameter sets are used for different synthesis objectives, allowing flexible adjustment of the randomness-control tradeoff

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach enables the cost-effective generation of unique, random oligonucleotides with varying sequences, suitable for applications like molecular cryptography, by minimizing reagent use and optimizing sequence randomness, while ensuring high accuracy and uniqueness.

Implementation Method 1

certain embodiments synthesize nucleotides using phosphoramidite chemistry

Methodology Applied
Scientific EffectPhosphoramidite chemistry: Chemical Bonding

Implementation Method 2

oligonucleotides are synthesized using an enzymatic processes, such as using a terminal deoxynucleotidyl transferase when generating random oligonucleotides

Methodology Applied
Scientific EffectEnzymatic process: Enzyme

Data Source

PatentEP3887385B1A method for generating random oligonucleotides and determining their sequence
Publication Date: 2024.03.20 GENEINFOSEC INC
  • EP3887385B1 patent drawingFigure 1
  • EP3887385B1 patent drawingFigure 2(a)~2(d)
  • EP3887385B1 patent drawingFigure 3A~3C

AI summary

Random oligonucleotides are generated with incomplete information about the sequence of the nucleic acid bases present in the newly generated molecules. The sequences of the oligonucleotides are subsequently determined and then these oligonucleotides can be processed for various potential uses.