Reactive Polyurethane Dispersion pH Stability

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Solution Overview

Problem

Commercially available reactive polyurethane dispersions used in UV-curable inkjet inks are prone to pH instability under basic aqueous conditions, leading to hydrolysis and a significant drop in pH, which affects the ink's jetting performance and stability.

Innovation Solution

The development of reactive polyurethane dispersions with specific combinations of functional groups in the polymer backbone and capping units, including styrene-containing monoalcohols and ionic stabilizing groups, which are incorporated into the polymer strands to enhance pH stability and UV curability.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If conventional reactive polyurethane dispersions are used in UV-curable inkjet inks, then the ink can be cured to form a durable coating, but the dispersion is prone to pH instability under basic aqueous conditions leading to hydrolysis and pigment precipitation

Engineering Contradiction:
ImprovepH stabilityVSAvoidhydrolysis and pigment precipitation
Core Design Contradiction:
ReliabilityVSObject-generated harmful factors

Solution Approach 1:

The invention changes the chemical parameters of the polyurethane dispersion by incorporating specific functional groups (carboxylic acid groups with pKa 4-6 and ionic stabilizing groups) to modify the pH behavior and prevent hydrolysis under basic conditions

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention creates a composite polyurethane structure combining multiple functional groups (carboxylic acid groups, ionic stabilizing groups, and UV-curable groups) within the same polymer backbone to achieve simultaneous pH stability and curability

Inventive Principle:
Principle #40Composite materials

2Reliability

If ionic stabilizing groups are incorporated into the polymer strands, then pH stability is enhanced, but the complexity of the polymer structure increases

Engineering Contradiction:
ImprovepH stabilityVSAvoidpolymer structure complexity
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The invention merges multiple functions (pH stabilization, hydrolysis prevention, and UV curability) into a single polyurethane polymer structure, eliminating the need for separate stabilizing agents and simplifying the overall formulation

Inventive Principle:
Principle #5Merging (Combining)

3Strength

If the polyurethane dispersion is designed for UV curability, then a durable cross-linked coating is formed, but the presence of reactive groups may accelerate hydrolysis under basic conditions

Engineering Contradiction:
Improvecoating durabilityVSAvoidpH stability
Core Design Contradiction:
StrengthVSReliability

Solution Approach 1:

The invention places different functional groups at specific locations within the polymer structure - carboxylic acid groups and ionic stabilizing groups are positioned to provide pH stability, while UV-curable groups are positioned to enable cross-linking, with each region performing its specialized function

Inventive Principle:
Principle #3Local quality

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The reactive polyurethane dispersions maintain pH stability over time, preventing pigment precipitation and ensuring the ink's jetting performance and durability, even under accelerated shelf-life conditions, while allowing for UV curing to form a durable printed image.

Implementation Method 1

one terminal capped with one or more ionic stabilizing groups... maintain pH stability over time, preventing pigment precipitation

Methodology Applied
Scientific EffectIonic stabilization:

Implementation Method 2

UV-curable polyurethane coatings can be applied in liquid form and then cured very quickly using UV radiation to produce a hard, durable cross-linked coating

Methodology Applied
Scientific EffectUV curing: Photopolymerisation

Data Source

PatentEP3507318B1Reactive polyurethane dispersions
Publication Date: 2022.11.09 HEWLETT PACKARD DEVELOPMENT COMPANY LP
  • EP3507318B1 patent drawingFigure 1
  • EP3507318B1 patent drawingFigure 2
  • EP3507318B1 patent drawing

AI summary

The present disclosure is drawn to a reactive polyurethane dispersion including a polymer strand having a polymer backbone that has two ends terminating at a first capping unit and a second capping unit. The polymer backbone can include polymerized monomers including a reactive diol and a diisocyanate. The reactive diol can be an acrylate-containing diol, a methacrylate-containing diol, a styrene-containing diol, or combination thereof. The first capping unit can be a styrene-containing monoalcohol reacted with an isocyanate group of the diisocyanate. The second capping unit can be an ionic stabilizing group.