Reactor for Syngas Production via CO2 Conversion

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Solution Overview

Problem

Existing reactors for synthesis gas production face issues such as soot formation, energy inefficiency, and economic inefficiency due to multi-stage processes, which lead to carburization and destruction of steel surfaces, and require expensive purification and complex reactor construction.

Innovation Solution

A pressure- and temperature-resistant reactor with at least two fluid-tight supply lines for CO2 and H2 reactant fluids, recuperative countercurrent heat exchange zones, and a reaction zone with a catalyst bed, designed to minimize soot formation and optimize energy use, allowing for single-stage processing and recycling of waste gases.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If high temperature and pressure are used to drive the endothermic CO2 and H2 conversion reaction, then synthesis gas production efficiency is improved, but soot formation increases leading to carburization and destruction of steel surfaces

Engineering Contradiction:
Improvesynthesis gas production efficiencyVSAvoidsoot formation
Core Design Contradiction:
ProductivityVSObject-generated harmful factors

Solution Approach 1:

A water vapor injection system is introduced as an intermediary substance into the reaction zone. The water vapor acts as a mediator that suppresses soot formation and carburization of the steel surface while allowing the endothermic reaction to proceed at high temperature and pressure conditions, thus resolving the contradiction between productivity and harmful factor generation

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent changes the chemical composition parameters of the reaction mixture by introducing water vapor. This parameter change modifies the reaction environment to suppress soot formation and protect the steel surface, enabling the system to operate at optimal temperature and pressure for synthesis gas production without the harmful side effects

Inventive Principle:
Principle #35Parameter changes

2Productivity

If multi-stage processes with repeated catalyst passage are used to achieve highest yield, then synthesis gas production yield is improved, but process complexity and energy consumption increase

Engineering Contradiction:
Improvesynthesis gas production yieldVSAvoidprocess complexity
Core Design Contradiction:
ProductivityVSDevice complexity

Solution Approach 1:

The patent merges multiple functional zones (heating zone, reaction zone, heat exchange zones) into a single integrated reactor system. This combining of functions allows the process to achieve high yield in a single pass through optimized reaction conditions and heat recovery, eliminating the need for complex multi-stage processes with repeated catalyst passage

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

The patent implements continuous heat exchange and reaction in a single-stage process. The countercurrent heat exchange zones maintain continuous heat transfer to the reactants, ensuring optimal reaction conditions are maintained throughout the single pass through the catalyst, thereby achieving high yield without repeated processing stages

Inventive Principle:
Principle #20Continuity of useful action

3Reliability

If steel reactors are used to withstand high temperature and pressure, then reactor durability is improved, but soot formation on surfaces leads to carburization and destruction of the steel

Engineering Contradiction:
Improvereactor durabilityVSAvoidsteel surface lifespan
Core Design Contradiction:
ReliabilityVSDuration of action of stationary object

Solution Approach 1:

Water vapor is introduced as an intermediary protective substance into the reaction zone. It acts as a mediator that suppresses soot formation and prevents carburization of the steel surface, thereby protecting the reactor material from degradation while maintaining the high temperature and pressure conditions necessary for reaction durability

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent creates a protective atmosphere in the reaction zone by introducing water vapor. This inert-like environment suppresses the formation of soot and prevents direct contact between carbon-containing species and the steel surface, thereby preventing carburization and extending the lifespan of the reactor material

Inventive Principle:
Principle #39Inert atmosphere (Inert environment)

4Productivity

If recycling of waste gases is implemented to increase utilization, then economic efficiency is improved, but soot formation in the reactor increases

Engineering Contradiction:
Improvecarbon-containing species utilizationVSAvoidsoot formation
Core Design Contradiction:
ProductivityVSObject-generated harmful factors

Solution Approach 1:

Water vapor is introduced as an intermediary substance into the reaction zone where waste gases are recycled. It acts as a mediator that suppresses soot formation while allowing the recycling process to proceed, thus enabling high utilization of carbon-containing species without the harmful side effect of increased soot formation

Inventive Principle:
Principle #24Intermediary (Mediator)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The reactor achieves efficient synthesis gas production with reduced soot formation, optimized energy use, and improved economic efficiency by minimizing reactor complexity and enabling the use of different starting materials and reactions, while maintaining stability up to 50 bar pressure and 1100°C temperature.

Implementation Method 1

at least one reaction zone with at least one catalyst in a catalyst bed

Methodology Applied
Scientific EffectCatalysis: Catalysis

Implementation Method 2

at least two recuperative countercurrent heat exchange zones, partial areas of the at least two feed lines being arranged in both countercurrent heat exchange zones

Methodology Applied
Scientific EffectHeat exchange: Heat Exchanger

Implementation Method 3

at least one heating zone, wherein at least a partial area of the at least second supply line for the second educt fluid is arranged in the heating zone

Methodology Applied
Scientific EffectHeating: Heating

Data Source

PatentEP3678767B1Conversion reactor and management of method
Publication Date: 2023.06.07 KARLSRUHER INST FUR TECH
  • EP3678767B1 patent drawingFigure 1
  • EP3678767B1 patent drawingFigure 2
  • EP3678767B1 patent drawingFigure 3A~3B

AI summary

The invention relates to a pressure- and temperature-resistant reactor for preparing syngas in a reverse CO conversion, in which gases containing CO2 are converted under high pressure with the aid of hydrogen into a syngas mixture (CO and H2), and relates to a method for preparing a syngas mixture using said reactor.