Reducing Fluorescence in Recycled Pulp via Sequential Oxidation

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Solution Overview

Problem

Fluorescent whitening agents in recycled paper pulp cause operational issues in de-inked pulp and paper mills, affect product quality, and pose potential health hazards, necessitating an efficient method to reduce or remove them, especially for food-grade applications.

Innovation Solution

A process involving the simultaneous or subsequent addition of chlorine dioxide and sodium hypochlorite to pulp slurry, with chlorine dioxide added first, effectively reduces fluorescence, using specific chemical amounts and timing to achieve near-zero fluorescence without significant brightness increase.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Illumination intensity

If fluorescent whitening agents are added to enhance brightness, then apparent brightness is improved, but operational problems occur in de-inked pulp mills and product quality is impaired

Engineering Contradiction:
Improveapparent brightnessVSAvoidoperational reliability
Core Design Contradiction:
Illumination intensityVSReliability

Solution Approach 1:

The patent removes fluorescent whitening agents from recycled pulp through chemical treatment with chlorine dioxide and sodium hypochlorite, extracting the harmful fluorescent compounds while preserving the pulp fibers for further processing

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The patent changes the chemical parameters of the pulp by introducing specific oxidizing agents (chlorine dioxide and sodium hypochlorite) in controlled amounts and sequences, transforming the fluorescent compounds into non-fluorescent degradation products

Inventive Principle:
Principle #35Parameter changes

2Illumination intensity

If fluorescent whitening agents are used to enhance brightness, then apparent brightness is improved, but color and brightness control is affected

Engineering Contradiction:
Improveapparent brightnessVSAvoidcolor and brightness control
Core Design Contradiction:
Illumination intensityVSManufacturing precision

Solution Approach 1:

The patent extracts fluorescent whitening agents from the pulp using sequential chemical treatment, removing the substances that interfere with color and brightness control measurements and processing

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The patent implements UV-based on-line color sensors with control loops that can accurately measure and control color and brightness parameters after fluorescent agents are removed, enabling precise manufacturing control

Inventive Principle:
Principle #23Feedback

3Illumination intensity

If fluorescent whitening agents are added to improve brightness, then apparent brightness is improved, but health hazards are created through leaching

Engineering Contradiction:
Improveapparent brightnessVSAvoidhealth hazard from leaching
Core Design Contradiction:
Illumination intensityVSObject-affected harmful factors

Solution Approach 1:

The patent extracts fluorescent whitening agents from recycled pulp through chemical oxidation with chlorine dioxide and sodium hypochlorite, removing the leachable compounds that pose health hazards in food-grade applications

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The patent uses strong oxidizing agents (chlorine dioxide and sodium hypochlorite) to rapidly degrade fluorescent whitening agents into non-hazardous compounds, eliminating health risks associated with leaching

Inventive Principle:
Principle #38Strong oxidants (Accelerated oxidation)

4Object-generated harmful factors

If chlorine dioxide is used to reduce fluorescence, then fluorescence is reduced, but residual chlorine dioxide hazards remain

Engineering Contradiction:
ImprovefluorescenceVSAvoidresidual chlorine dioxide hazard
Core Design Contradiction:
Object-generated harmful factorsVSObject-affected harmful factors

Solution Approach 1:

The patent introduces sodium hypochlorite as an intermediary substance that reacts with and neutralizes residual chlorine dioxide, converting it into less hazardous compounds while maintaining fluorescence reduction benefits

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent converts the potentially harmful residual chlorine dioxide into beneficial or neutral substances through reaction with sodium hypochlorite, transforming a hazard into a safe end state

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process achieves significant reduction or elimination of fluorescence, reducing chemical usage and preventing residual chlorine dioxide-related hazards, while maintaining pulp quality and safety for food-grade applications.

Implementation Method 1

contacting the pulp, which contains fluorescent agents, with a combination of chlorine dioxide (CIO2) and sodium hypochlorite (or a derivative of sodium hypochlorite) in amounts sufficient to reduce the fluorescence of the pulp

Methodology Applied
Scientific EffectOxidation: Oxidation

Data Source

PatentEP2798121B1Process for reducing fluorescence in pulp
Publication Date: 2016.10.12 NALCO CO
  • EP2798121B1 patent drawingFigure 1~2
  • EP2798121B1 patent drawingFigure 3~4
  • EP2798121B1 patent drawingFigure 5~6

AI summary

The invention is directed to a method for reducing fluorescence in recycled pulp, wherein the method includes: contacting a pulp slurry containing fluorescent agents with chlorine dioxide; and contacting the pulp slurry with a sodium hypochlorite component, in an amount sufficient to reduce the fluorescence of the pulp; wherein the pulp is contacted with sodium hypochlorite component simultaneous with or after contact with chlorine dioxide.