Reducing Solvent Composition for Conductive Copper Sintering

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Solution Overview

Problem

Existing bonding methods using copper sintered objects and electroconductive pastes face complications such as the need for immediate sintering and laborious surface treatment to prevent re-oxidation and corrosion, and generate voids leading to reduced bondability.

Innovation Solution

A solvent composition containing a reducing organic substance, a basic compound, and optionally a coordinating organic compound is applied to a metal member, dissolving the metal oxide film and precipitating metal nanoparticles, allowing for easy production of a sintered object with excellent electroconductivity and bondability without removing the solvent.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If copper nanoparticles are sintered in a reducing atmosphere to prevent re-oxidation, then electroconductivity is improved, but the operation becomes complicated and requires immediate sintering

Engineering Contradiction:
ImproveelectroconductivityVSAvoidoperation complexity
Core Design Contradiction:
ReliabilityVSEase of operation

Solution Approach 1:

The patent applies a reducing agent (formic acid) to the copper nanoparticle aggregate before sintering, creating a protective reducing environment in advance. This preliminary action eliminates the need for immediate sintering in a reducing atmosphere, allowing the material to be stored and handled without re-oxidation concerns while maintaining electroconductivity.

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The formic acid acts as an intermediary substance that mediates between the copper nanoparticles and oxygen. It provides a localized reducing environment at the particle surface, preventing oxidation without requiring the entire system to be in a reducing atmosphere, thus simplifying the sintering process.

Inventive Principle:
Principle #24Intermediary (Mediator)

2Reliability

If a reducing agent or etching solution is applied to remove surface oxide film, then electroconductivity is improved, but laborious removal efforts are required

Engineering Contradiction:
ImproveelectroconductivityVSAvoidmanufacturing effort
Core Design Contradiction:
ReliabilityVSEase of manufacture

Solution Approach 1:

The patent combines the reducing agent (formic acid) with the sintering process itself, merging the oxide removal function with the bonding process. This eliminates the need for separate, laborious oxide removal steps while still achieving the necessary surface preparation for high electroconductivity.

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

The formic acid applied to the copper nanoparticle aggregate performs multiple functions automatically: it acts as a reducing agent to prevent oxidation, serves as a dispersant to maintain particle separation, and provides the necessary surface treatment. The material essentially prepares itself for sintering without external intervention.

Inventive Principle:
Principle #25Self-service

3Ease of operation

If formic acid decomposition gas is generated during sintering, then sintering can proceed without reducing atmosphere, but voids are generated reducing bondability

Engineering Contradiction:
Improvesintering process simplicityVSAvoidbondability
Core Design Contradiction:
Ease of operationVSReliability

Solution Approach 1:

The patent extracts or removes the formic acid decomposition gas from the sintering zone by applying the formic acid to the copper nanoparticle aggregate rather than to a pre-formed compact. This allows the gas to escape during the granulation process before the material is pressed into a dense form, preventing void formation while maintaining the benefits of formic acid decomposition.

Inventive Principle:
Principle #2Taking out (Extraction)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solvent composition enables sintering at lower temperatures with improved electroconductivity and bondability by suppressing oxidation and corrosion, eliminating the need for additional surface treatments.

Implementation Method 1

a sintered object having excellent electroconductivity and bondability can be easily obtained from such a solvent-treated metal member without removing the solvent after the treatment

Methodology Applied
Scientific EffectReduction: Reduction

Implementation Method 2

a metal oxide film on the surface of the metal member can be dissolved

Methodology Applied
Scientific EffectDissolution: Solvation

Implementation Method 3

a coordinating organic substance is applied to a metal member, dissolving the metal oxide film and precipitating metal nanoparticles

Methodology Applied
Scientific EffectComplex formation: Chemical Bonding

Data Source

PatentEP4613403A1Solvent composition and method for producing sintered object
Publication Date: 2025.09.10 DAICEL CORP
  • EP4613403A1 patent drawingFigure 1
  • EP4613403A1 patent drawingFigure 2
  • EP4613403A1 patent drawingFigure 3

AI summary

There is provided a solvent composition which does not need to be removed after application and allows a sintered object having excellent electroconductivity and bondability to be easily produced. The solvent composition of the present disclosure is a solvent composition for sintering aids, the solvent composition containing a reducing organic substance and a basic compound. The solvent composition of the present disclosure is also a solvent composition including a reducing organic substance, a basic compound, and a coordinating organic compound other than compounds included as the basic compound, and the coordinating organic compound has a higher boiling point than the reducing organic substance.