Refractory Metal Substrates for CVD Diamond Speaker Domes

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Solution Overview

Problem

The existing methods for manufacturing diamond speaker domes using silicon substrates are costly, hazardous, and result in substrate reuse issues, thermal runaway, and impurity incorporation, while refractory metal substrates face challenges like non-uniform growth, delamination, and cracking, especially when reused for larger polycrystalline diamond discs.

Innovation Solution

A method involving a carbide forming refractory metal substrate with a carefully prepared metal carbide surface and controlled cooling to achieve delamination of polycrystalline CVD synthetic diamond components without cracking, allowing for substrate reuse and avoiding post-growth treatment steps.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If silicon substrates are used for CVD diamond growth, then diamond speaker domes can be manufactured, but the process becomes costly, hazardous, and the substrates cannot be reused

Engineering Contradiction:
Improvemanufacturing yieldVSAvoidprocess complexity and cost
Core Design Contradiction:
ReliabilityVSEase of manufacture

Solution Approach 1:

The patent replaces expensive, non-reusable silicon substrates with inexpensive, reusable refractory metal substrates. The refractory metal substrates can withstand high temperatures and mechanical stress, allowing them to be reused multiple times without degradation, thereby eliminating the need for costly acid dissolution processes and reducing manufacturing complexity

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Solution Approach 2:

The patent changes the substrate material parameters from silicon to refractory metals (tungsten, molybdenum, niobium, or tantalum), which have fundamentally different thermal and mechanical properties. This parameter change enables substrate reuse and eliminates the hazardous acid dissolution step while maintaining high manufacturing yields

Inventive Principle:
Principle #35Parameter changes

2Productivity

If silicon substrates are used in microwave activated CVD processes, then diamond growth occurs, but thermal runaway and fracture occur due to power absorption at high temperatures

Engineering Contradiction:
Improvediamond growth rateVSAvoidsubstrate stability
Core Design Contradiction:
ProductivityVSReliability

Solution Approach 1:

The patent replaces silicon substrates that suffer from thermal runaway with refractory metal substrates that can withstand high temperatures without fracturing. The refractory metals have much higher melting points and thermal stability, allowing sustained high-temperature CVD processes without substrate failure

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Solution Approach 2:

The patent changes the thermal properties of the substrate by replacing silicon with refractory metals having superior high-temperature stability. This parameter change eliminates thermal runaway while maintaining the productivity benefits of microwave activated CVD processes

Inventive Principle:
Principle #35Parameter changes

3Ease of manufacture

If refractory metal substrates are used for CVD diamond growth, then substrate reuse is possible, but non-uniform growth, delamination, and cracking occur

Engineering Contradiction:
Improvesubstrate reuse capabilityVSAvoidgrowth uniformity and defect-free quality
Core Design Contradiction:
Ease of manufactureVSManufacturing precision

Solution Approach 1:

The patent applies preliminary surface treatment to the refractory metal substrates before diamond deposition. The surfaces are mechanically polished and chemically etched to create uniform nucleation sites, ensuring uniform diamond growth and preventing delamination and cracking during subsequent processing

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The patent optimizes the surface parameters of the refractory metal substrates through mechanical and chemical treatment. This creates controlled surface roughness and chemistry that promotes uniform diamond nucleation and growth, eliminating the non-uniformity and defects associated with as-received refractory metal surfaces

Inventive Principle:
Principle #35Parameter changes

4Productivity

If silicon substrates are used, then diamond speaker domes can be manufactured, but silicon is incorporated into the diamond creating impurities

Engineering Contradiction:
Improvemanufacturing efficiencyVSAvoiddiamond purity
Core Design Contradiction:
ProductivityVSManufacturing precision

Solution Approach 1:

The patent replaces silicon substrates that contaminate the diamond with refractory metal substrates that do not incorporate into the diamond structure. The refractory metals remain as distinct substrate material, allowing production of high-purity diamond without silicon contamination

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Solution Approach 2:

The patent changes the substrate material composition from silicon to refractory metals, fundamentally altering the chemical interaction during CVD growth. This parameter change eliminates silicon incorporation into the diamond lattice, producing higher purity diamond material while maintaining manufacturing efficiency

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach enables the production of high-quality, crack-free diamond speaker domes with improved substrate reuse and reduced manufacturing costs, maintaining acoustic properties and purity by minimizing silicon incorporation and thermal stress.

Implementation Method 1

treating a non-planar surface of a carbide forming refractory metal substrate to form a metal carbide layer on said non-planar surface

Methodology Applied
Scientific EffectCarbide formation: Chemical Bonding

Implementation Method 2

growing a film of polycrystalline CVD synthetic diamond material on said non-planar surface in a CVD reactor

Methodology Applied
Scientific EffectChemical vapour deposition: Chemical Vapour Deposition

Implementation Method 3

cooling the carbide forming refractory metal substrate and the film of polycrystalline CVD synthetic diamond material at a controlled rate whereby the film of polycrystalline CVD synthetic diamond material delaminates from the metal carbide surface

Methodology Applied
Scientific EffectThermal contraction: Thermal Contraction

Data Source

PatentEP2856774B1Free-standing non-planar polycrystalline synthetic diamond components and method of fabrication
Publication Date: 2016.11.30 ELEMENT SIX TECH LTD
  • EP2856774B1 patent drawingFigure 1~2
  • EP2856774B1 patent drawingFigure 3~4
  • EP2856774B1 patent drawingFigure 5

AI summary

A free-standing non-planar polycrystalline CVD synthetic diamond component which comprises a nucleation face and a growth face, the nucleation face comprising smaller grains than the growth face, the nucleation face having a surface roughness Ra no more than 50 nm, wherein the free-standing non-planar polycrystalline CVD synthetic diamond component has a longest linear dimension when projected onto a plane of no less than 5 mm and is substantially crack free over at least a central region thereof, wherein the central region is at least 70% of a total area of the free-standing non-planar polycrystalline CVD synthetic diamond component, wherein the central region has no cracks which intersect both external major faces of the free-standing non-planar polycrystalline CVD synthetic diamond component and extend greater than 2 mm in length.