Renewable Base Oil Calcium Sulfonate Grease With Calcite Conversion

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Solution Overview

Problem

Existing formulations of overbased calcium sulfonate greases in renewable base oils face challenges in achieving desired consistency and performance characteristics due to the reactants reacting with vegetable oils or esters during gelation, leading to inadequate conversion of amorphous calcium carbonate to crystalline calcite, and lack of high-temperature, extreme-pressure, and anti-wear properties.

Innovation Solution

A two-step process involving promotion and conversion using renewable base oils, such as SynNova 9, to form a non-Newtonian overbased calcium sulfonate complex grease without performance additives, utilizing specific hydrocarbon mixtures with controlled branching and polarity to facilitate the conversion of amorphous calcium carbonate to crystalline calcite.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Object-affected harmful factors

If overbased calcium sulfonate is used as thickener in renewable base oils, then environment friendliness is improved, but consistency and performance characteristics deteriorate due to reactants reacting with vegetable oils or esters during gelation

Engineering Contradiction:
Improveenvironment friendlinessVSAvoidconsistency
Core Design Contradiction:
Object-affected harmful factorsVSStability of the object's composition

Solution Approach 1:

The patent uses a two-step process with an intermediary conversion step. First, overbased calcium sulfonate is prepared in a promotion step, then converted in a separate conversion step using converting agents (water, alcohols, or acids) to transform amorphous calcium carbonate to crystalline calcite. This intermediary conversion process resolves the contradiction by preventing direct reaction with renewable base oils while achieving proper gelation and consistency.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent changes the physical and chemical parameters of the system by controlling the conversion process. By adjusting parameters such as temperature (100-200°C), adding converting agents (water, alcohols, or acids), and controlling the gelation time, the patent transforms the system from a reactive state (amorphous calcium carbonate) to a stable state (crystalline calcite), thereby achieving desired consistency without harmful reactions with renewable base oils.

Inventive Principle:
Principle #35Parameter changes

2Reliability

If conventional mineral or synthetic base oils are used, then performance characteristics are improved, but environment friendliness deteriorates

Engineering Contradiction:
Improveperformance characteristicsVSAvoidenvironment friendliness
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The patent changes the base oil parameter from conventional mineral or synthetic oils to renewable base oils (vegetable oils or esters). By controlling other parameters (two-step process, converting agents, temperature), the patent maintains performance characteristics while improving environment friendliness.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent introduces an intermediary conversion step that acts as a bridge between the thickener preparation and the final grease formulation. This intermediary process ensures that the overbased calcium sulfonate is properly converted before contact with renewable base oils, thereby maintaining performance characteristics equivalent to conventional oils while using environment-friendly renewable base oils.

Inventive Principle:
Principle #24Intermediary (Mediator)

3Device complexity

If amorphous calcium carbonate is not converted to crystalline calcite, then gelation process is simplified, but high-temperature and extreme-pressure properties deteriorate

Engineering Contradiction:
Improvegelation process complexityVSAvoidhigh-temperature properties
Core Design Contradiction:
Device complexityVSTemperature

Solution Approach 1:

The patent performs preliminary conversion of amorphous calcium carbonate to crystalline calcite in a dedicated conversion step before final grease formulation. By preparing the crystalline structure in advance (preliminary action), the patent ensures high-temperature and extreme-pressure properties are achieved while maintaining a manageable gelation process.

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The resulting grease exhibits superior performance in lifespan, anti-wear, anti-friction, oxidation resistance, and high-temperature characteristics, outperforming mineral and synthetic oil-based counterparts, with reduced thickener content and improved stability under heavy loads and humid conditions.

Implementation Method 1

conversion of amorphous calcium carbonate to crystalline calcite

Methodology Applied
Scientific EffectCrystallisation: Crystallisation

Implementation Method 2

form a non-Newtonian overbased calcium sulfonate complex grease

Methodology Applied
Scientific EffectNon-Newtonian Fluids: Non-Newtonian Fluids

Implementation Method 3

utilizing specific hydrocarbon mixtures with controlled branching and polarity to facilitate the conversion

Methodology Applied
Scientific EffectSolvation: Solvation

Implementation Method 4

superior performance in lifespan, anti-wear, anti-friction, oxidation resistance, and high-temperature characteristics

Methodology Applied
Scientific EffectLubrication: Lubrication

Implementation Method 5

superior performance in lifespan, anti-wear, anti-friction, oxidation resistance, and high-temperature characteristics

Methodology Applied
Scientific EffectOxidation resistance: Oxidation

Data Source

PatentEP4139426B1High performance grease compositions with a renewable base oil
Publication Date: 2026.01.21 CHEVRON USA INC
  • EP4139426B1 patent drawingFigure 1
  • EP4139426B1 patent drawingFigure 2
  • EP4139426B1 patent drawing

AI summary

The present invention is directed to high-performance grease compositions based on renewal base oils. The compositions disclosed in this invention with or without performance additives delineate superior anti-wear, anti-friction, thermal & oxidation stability, high temperature long life, low noise, low thickener content, better dispersion in renewable base oil compared to identical grease compositions prepared with conventional mineral and synthetic base oils. The grease compositions formed from renewable base oils may be utilized in bearings and gears in automotive, industrial and marine applications.