Renewable Hydrocarbon Coprocessing for Cold Flow and Aromatic Reduction

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Solution Overview

Problem

Existing processes struggle to efficiently produce liquid hydrocarbons from renewable sources that meet fuel specifications by addressing issues of high n-paraffin and aromatic content, which affect cold flow properties and environmental impact.

Innovation Solution

A process combining hydrotreated n-paraffin-rich and hydropyrolyzed aromatic-rich liquids, followed by hydrogenation and hydroisomerization, to reduce n-paraffin and aromatic content, improving cold flow properties and meeting fuel specifications.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If renewable feedstocks are hydrotreated to remove oxygen, sulphur, and nitrogen, then the fuel quality is improved, but the n-paraffin content becomes too high which deteriorates cold flow properties

Engineering Contradiction:
Improvefuel qualityVSAvoidcold flow properties
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The process segments the treatment of different renewable feedstocks into separate streams: one stream (hydrotreated vegetable oils/animal fats) produces n-paraffin-rich liquid, while another stream (hydropyrolyzed biomass) produces aromatic-rich liquid. These segmented streams are then combined and reprocessed together to achieve synergistic effects that neither stream can achieve alone.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The patent merges two differently processed renewable liquid streams - the n-paraffin-rich liquid from hydrotreating and the aromatic-rich liquid from hydropyrolysis - into a combined feedstock. This merging allows the subsequent hydroisomerization step to simultaneously reduce n-paraffin content (improving cold flow) and manage aromatic content, resolving the cold flow property deterioration issue.

Inventive Principle:
Principle #5Merging (Combining)

2Use of energy by moving object

If hydropyrolyzed aromatic-rich liquid is produced from biomass, then the aromatic content increases which improves energy density, but the environmental impact worsens due to higher aromatic emissions

Engineering Contradiction:
Improveenergy densityVSAvoidaromatic emissions
Core Design Contradiction:
Use of energy by moving objectVSObject-generated harmful factors

Solution Approach 1:

The patent combines aromatic-rich liquid from hydropyrolysis with n-paraffin-rich liquid from hydrotreating to create a balanced mixed feedstock. The subsequent hydroisomerization process in the merged stream reduces aromatic content by approximately 50% while maintaining the energy density benefits, thus lowering aromatic emissions without sacrificing energy content.

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

The process converts the potentially harmful high aromatic content into a benefit by using it as a feedstock for hydroisomerization. The aromatic-rich liquid serves as a valuable carbon source that, when processed through the combined treatment, yields reduced aromatic emissions while maintaining fuel quality and energy density.

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

3Object-affected harmful factors

If n-paraffin content is reduced through hydroisomerization, then cold flow properties are improved, but the process complexity increases due to additional catalytic steps

Engineering Contradiction:
Improvecold flow propertiesVSAvoidprocess complexity
Core Design Contradiction:
Object-affected harmful factorsVSDevice complexity

Solution Approach 1:

The patent merges multiple functions into a single integrated hydroisomerization step that processes the combined renewable liquid feedstock. This single catalytic process simultaneously achieves n-paraffin conversion (improving cold flow), aromatic content reduction (lowering emissions), and fuel quality enhancement, thereby reducing overall process complexity compared to treating separate streams through multiple different processes.

Inventive Principle:
Principle #5Merging (Combining)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process synergistically enhances cold flow properties and reduces aromatic content, producing a liquid hydrocarbon suitable for fuels and chemicals, with improved environmental performance.

Implementation Method 1

subjecting the combined liquid to a hydrogenation catalyst and conditions sufficient to cause a hydrodearomatization reaction

Methodology Applied
Scientific EffectHydrodearomatization: Hydrogenation

Implementation Method 2

subjecting the dearomatized liquid to a hydroisomerization catalyst and conditions sufficient to cause a hydroisomerization reaction

Methodology Applied
Scientific EffectHydroisomerization: Catalysis

Implementation Method 3

The renewable feedstocks are therefore hydrotreated to remove oxygen, sulphur, and nitrogen

Methodology Applied
Scientific EffectHydrotreating: Hydrogenation

Implementation Method 4

providing a second liquid produced by hydropyrolyzing a second renewable source selected from the group consisting of lignin, lignocellulosic material, cellulosic material, hemicellulosic material, waste plastic, municipal waste, and combinations thereof

Methodology Applied
Scientific EffectHydropyrolysis: Pyrolysis

Data Source

PatentEP4444823B1Process for producing a liquid hydrocarbon from renewable sources
Publication Date: 2026.02.11 SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ BV
  • EP4444823B1 patent drawingFigure 1

AI summary

A process for producing a liquid hydrocarbon from renewable sources includes combining first and second liquids, where the first liquid is produced by hydrotreating a first renewable source and the second liquid is produced by hydropyrolyzing a second renewable source. The first liquid has a n-paraffin content greater than or equal to 50 wt.%, while the second liquid has an aromatic content greater than or equal to 5 wt.%. The combined liquid has a first n-paraffin content and a first aromatic content before being subjected to a hydrogenation catalyst and conditions sufficient to cause a hydrodearomatization reaction, and a hydroisomerization catalyst and conditions sufficient to cause a hydroisomerization reaction. The resulting liquid hydrocarbon has a second n-paraffin content that is less than the first n-paraffin content and a second aromatic content that is less than the first aromatic content.