Reversible Silane Surface Functionalization for Flow Cell Renewal

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Solution Overview

Problem

Current sequencing technologies, such as sequencing-by-synthesis (SBS), require a new flow cell after each use due to the irreversible attachment of silane layers, leading to high costs and waste, as there is no efficient method to renew or recycle the flow cell surfaces.

Innovation Solution

The use of reversible interactions, including host-guest complexes and copper-imine bonds, allows for the reversible immobilization of biological molecules like DNA on silane-functionalized surfaces, enabling the reuse of flow cells by dissociating the molecules under specific conditions.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of repair

If a strong base is used to remove the silane layer, then the flow cell can be renewed, but a CVD oven is required which increases device complexity and cost

Engineering Contradiction:
Improveflow cell renewalVSAvoidCVD oven requirement
Core Design Contradiction:
Ease of repairVSDevice complexity

Solution Approach 1:

The patent extracts the silane layer removal process from the complex CVD oven system by using a simple base treatment that can be performed without specialized equipment. The base selectively removes the silane layer while leaving the flow cell substrate intact, enabling renewal through a straightforward chemical treatment rather than requiring removal and re-deposition equipment.

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The patent changes the chemical parameters of the silane layer by treating it with a base solution, which alters the silane's chemical state from a stable covalently-bonded layer to a removable form. This parameter change enables the silane to be detached under mild conditions without requiring high-temperature CVD equipment, thus simplifying the renewal process.

Inventive Principle:
Principle #35Parameter changes

2Reliability

If the flow cell is disposed after each use, then sequencing quality is maintained, but cost and waste increase

Engineering Contradiction:
Improvesequencing qualityVSAvoidflow cell waste
Core Design Contradiction:
ReliabilityVSLoss of substance

Solution Approach 1:

The patent implements a recovery process where the valuable flow cell substrate is preserved and the only discarded material is the spent silane layer. By selectively removing and discarding only the consumable silane component while recovering and reusing the expensive flow cell substrate, the system maintains sequencing quality through proper surface preparation while dramatically reducing waste and cost.

Inventive Principle:
Principle #34Discarding and recovering

3Strength

If covalent attachment is used to attach DNA to the surface, then immobilization strength is improved, but reversibility is lost

Engineering Contradiction:
Improveimmobilization strengthVSAvoidreversibility
Core Design Contradiction:
StrengthVSAdaptability or versatility

Solution Approach 1:

The patent creates a dynamic system where the attachment strength can be modulated. The silane layer provides strong initial immobilization of DNA through covalent bonds, but the entire silane layer can be reversibly removed by base treatment. This dynamic approach allows the system to switch between strong attachment (during sequencing) and complete release (for renewal), providing both strength and reversibility at different operational stages.

Inventive Principle:
Principle #15Dynamics

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach enables the multiple use of flow cells, reducing waste and costs by allowing the regeneration of the flow cell surface while maintaining the integrity of the functionalized silane layer, thus facilitating cost-effective and sustainable DNA sequencing processes.

Implementation Method 1

it is known that a strong base can be used to efficiently remove the silane layer

Methodology Applied
Scientific EffectChemical reaction with base: Chemical Bonding

Data Source

PatentEP3183577B1Reversible surface functionalization
Publication Date: 2020.08.19 ILLUMINA CAMBRIDGE LTD
  • EP3183577B1 patent drawingFigure 1
  • EP3183577B1 patent drawingFigure 2
  • EP3183577B1 patent drawingFigure 3A~3B

AI summary

Some embodiments described herein relate to a substrate comprising a silane functionalized surface for reversibly immobilizing a biological molecule of interest, such as oligonucleotides, polynucleotides, or protein. Methods for immobilizing the biological molecule and the use in DNA sequencing and other diagnostic applications are also disclosed.