R-T-B Alloy Flake Production via Rapid Strip Casting

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Solution Overview

Problem

Current methods for producing R-T-B type alloy flakes do not adequately enhance magnetic characteristics, particularly coercive force, due to issues with α-Fe production and R-rich phase dispersion, which affect the quality and efficiency of sintered magnets.

Innovation Solution

A strip casting method is employed to produce R-T-B type alloy flakes with controlled cooling rates and molten alloy supply rates, resulting in a fine R 2 T 17 phase distribution, which enhances magnetic characteristics by stabilizing coercive force and improving texture homogeneity.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Object-affected harmful factors

If a homogenization treatment at high temperature is applied for a long time to eliminate α-Fe, then α-Fe can be removed from the raw material alloy, but the production time and energy consumption increase significantly

Engineering Contradiction:
Improveα-Fe contentVSAvoidhomogenization treatment time
Core Design Contradiction:
Object-affected harmful factorsVSLoss of time

Solution Approach 1:

The invention changes the cooling rate parameter during casting from conventional slow cooling to rapid cooling (10^2 to 10^4 K/s), which fundamentally alters the solidification path and prevents α-Fe formation through kinetic control rather than thermodynamic equilibrium

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention utilizes phase transition control by rapidly cooling the molten alloy to suppress the formation of α-Fe phase during solidification, directing the phase transformation toward desired R2T14B and R-rich phases instead

Inventive Principle:
Principle #36Phase transitions

2Reliability

If the R-rich phase is not uniformly dispersed in the shaped magnet, then local failure of sintering or reduction of magnetism occurs, but achieving uniform dispersion requires precise control of raw material alloy texture

Engineering Contradiction:
Improvesintering qualityVSAvoidalloy texture control
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The invention changes the cooling rate parameter during casting to create a fine cellular dendritic structure with uniform R-rich phase distribution, achieving reliable sintering outcomes without requiring complex post-casting texture control procedures

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention performs preliminary action by establishing the desired R-rich phase dispersion pattern during the casting process itself through controlled rapid cooling, rather than requiring subsequent complex processing steps to achieve uniform distribution

Inventive Principle:
Principle #10Preliminary action

3Manufacturing precision

If α-Fe remains in the magnet after sintering, then the magnetic characteristics of the magnet are reduced, but eliminating α-Fe requires solid phase diffusion for a long time

Engineering Contradiction:
Improvemagnetic characteristicsVSAvoidsolid phase diffusion time
Core Design Contradiction:
Manufacturing precisionVSDuration of action of moving object

Solution Approach 1:

The invention prevents α-Fe phase transition during solidification by rapid cooling, eliminating the need for subsequent long-duration solid phase diffusion processes to remove unwanted α-Fe inclusions

Inventive Principle:
Principle #36Phase transitions

Solution Approach 2:

The invention skips the intermediate step of allowing α-Fe to form and then requiring lengthy diffusion treatment by directly rapidly cooling through the temperature range where α-Fe would form, rushing through the problematic phase formation zone

Inventive Principle:
Principle #21Skipping (Rushing through)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method produces alloy flakes with a high coercive force and excellent magnetic characteristics by controlling the R 2 T 17 phase distribution, leading to improved sinterability and reduced α-Fe precipitation, thus enhancing the magnetic properties of sintered magnets.

Implementation Method 1

a flake of 0.1 to 1 mm is produced through solidification upon a casting roll

Methodology Applied
Scientific EffectThermal conduction: Conduction (thermal)

Implementation Method 2

a molten alloy is cast on a copper roll of which inside is water-cooled, and a flake of 0.1 to 1 mm is produced through solidification

Methodology Applied
Scientific EffectSolidification: Freezing

Implementation Method 3

The R-rich phase expands by reacting with hydrogen in a hydrogen atmosphere and becomes a brittle hydride

Methodology Applied
Scientific EffectHydrogenation: Hydrogenation

Data Source

PatentEP1780736B1R-T-B type alloy, production method of R-T-B type alloy flake, fine powder for R-T-B type rare earth permanent magnet, and R-T-B type rare earth permanent magnet
Publication Date: 2012.12.12 RESONAC HOLDINGS CORP
  • EP1780736B1 patent drawingFigure 1~2
  • EP1780736B1 patent drawingFigure 3

AI summary

The present invention provides an R-T-B type alloy as a raw material of a rare earth-based permanent magnet having excellent magnetic characteristics. The present invention provides an R-T-B type alloy (wherein R is at least one member selected from rare earth elements including Y, T is a transition metal essentially comprising Fe, and B is boron) which is a raw material for use in a rare earth-based permanent magnet, wherein the volume percentage of the region containing an R2T17 phase having an average grain diameter of 3 µm or less in the short axis direction is from 0.5 to 10%.