R-T-B Sintered Magnet Coercivity via Mn and Al

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Solution Overview

Problem

R-T-B based sintered magnets face challenges with low Curie temperature and significant coercivity variation with temperature, requiring increased coercivity without using expensive heavy rare-earth elements like Dy and Tb, while maintaining minimal decrease in magnetization.

Innovation Solution

An R-T-B based sintered magnet composition including 12-15 at% rare-earth element, 5-8 at% boron, 0.1-1 at% Al, 0.02-0.5 at% Mn, and a transition metal T, with Fe as the main ingredient, where Mn is added to minimize deterioration in magnetic properties and increase coercivity.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If heavy rare-earth elements such as Dy and Tb are added to increase coercivity, then the coercivity of the magnet is improved, but the production cost increases significantly and resource availability becomes restricted

Engineering Contradiction:
ImprovecoercivityVSAvoidproduction cost
Core Design Contradiction:
ReliabilityVSEase of manufacture

Solution Approach 1:

The patent changes the chemical composition parameters by adding specific elements (Al, Ga, In, Sn, Ti, V, Cr, Zr, Nb, Mo, Hf, Ta, W) in controlled amounts to modify the grain boundary phase properties, thereby achieving high coercivity without relying on expensive heavy rare-earth elements

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent replaces expensive heavy rare-earth elements (Dy, Tb) with cheaper alternative elements that can achieve similar or better coercivity enhancement, making the magnet production more cost-effective and sustainable

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

2Reliability

If additive elements such as Al are increased to increase coercivity, then the coercivity is improved, but the Curie temperature and magnetization of the main phase decrease

Engineering Contradiction:
ImprovecoercivityVSAvoidCurie temperature
Core Design Contradiction:
ReliabilityVSTemperature

Solution Approach 1:

The patent applies local quality by concentrating additive elements (Al, Ga, In, Sn, Ti, V, Cr, Zr, Nb, Mo, Hf, Ta, W) in the grain boundary phase rather than allowing them to distribute throughout the main phase, thereby enhancing coercivity locally at grain boundaries while preserving the magnetic properties of the main phase

Inventive Principle:
Principle #3Local quality

Solution Approach 2:

The patent uses the grain boundary phase as an intermediary medium where additive elements are preferentially located to exert their coercivity-enhancing effect, thereby mediating between the need for high coercivity and the need to maintain high Curie temperature and magnetization in the main phase

Inventive Principle:
Principle #24Intermediary (Mediator)

3Reliability

If additive elements such as Al are increased to increase coercivity, then the coercivity is improved, but the magnetization of the main phase decreases

Engineering Contradiction:
ImprovecoercivityVSAvoidmagnetization
Core Design Contradiction:
ReliabilityVSQuantity of substance

Solution Approach 1:

The patent applies local quality by concentrating additive elements (Al, Ga, In, Sn, Ti, V, Cr, Zr, Nb, Mo, Hf, Ta, W) in the grain boundary phase rather than allowing them to distribute throughout the main phase, thereby enhancing coercivity locally at grain boundaries while preserving the magnetic properties of the main phase

Inventive Principle:
Principle #3Local quality

Solution Approach 2:

The patent uses the grain boundary phase as an intermediary medium where additive elements are preferentially located to exert their coercivity-enhancing effect, thereby mediating between the need for high coercivity and the need to maintain high Curie temperature and magnetization in the main phase

Inventive Principle:
Principle #24Intermediary (Mediator)

Data Source

PatentEP2077567B1R-t-b sintered magnet
Publication Date: 2012.08.08 PROTERIAL LTD
  • EP2077567B1 patent drawingFigure 1
  • EP2077567B1 patent drawingFigure 2~3
  • EP2077567B1 patent drawingFigure 4~5

AI summary

An R-T-B based sintered magnet according to the present invention has a composition comprising: 12 at% to 17 at% of a rare-earth element R; 5.0 at% to 8.0 at% of boron B; 0.1 at% to 1.0 at% of Al; 0.02 at% to less than 0.5 at% of Mn; and a transition metal T as the balance. The rare-earth element R is at least one element selected from the rare-earth elements, including Y (yttrium), and includes at least one of Nd and Pr. The transition element T includes Fe as its main element.