Low-Viscosity RTV Silicone Elastomer for High PCM Loading

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Solution Overview

Problem

Existing crosslinked rubber compositions based on RTV silicone elastomers with phase-change materials (PCMs) have limited PCM content, resulting in reduced thermal energy storage and release capabilities, which are insufficient for demanding applications.

Innovation Solution

A crosslinked rubber composition using an RTV silicone elastomer with low dynamic viscosity, allowing for higher PCM content (up to 300 phr) and incorporation of thermally conductive fillers, enabling increased thermal energy storage and release, with a mass enthalpy of change of state greater than 70 J/g and thermal conductivity greater than 0.2 W.m-1K-1.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Quantity of substance

If a conventional RTV silicone elastomer with high dynamic viscosity (e.g., 15,000 mPa.s) is used to disperse PCM, then the elastomer provides sufficient structural stability, but the maximum PCM content is limited to about 43 phr (30% mass fraction), resulting in low mass enthalpy of change of state (50-70 J/g)

Engineering Contradiction:
ImprovePCM contentVSAvoidmass enthalpy of change of state
Core Design Contradiction:
Quantity of substanceVSTemperature

Solution Approach 1:

The patent changes the viscosity parameter of the RTV silicone elastomer from conventional high values (15,000 mPa.s) to very low values (≤5000 mPa.s, preferably ≤1000 mPa.s). This parameter change enables much higher PCM content (100-300 phr) to be dispersed while maintaining composition homogeneity and flexibility, thereby achieving mass enthalpy of change of state greater than 70 J/g (advantageously 80-200 J/g).

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite material system consisting of low-viscosity RTV silicone elastomer, non-encapsulated PCM (powder or liquid state), and optionally thermally conductive fillers. This composite structure allows for optimized thermal energy storage capabilities while maintaining mechanical flexibility and processability.

Inventive Principle:
Principle #40Composite materials

2Quantity of substance

If high PCM content (greater than 50 phr, especially 100-300 phr) is incorporated into the elastomer, then the mass enthalpy of change of state increases to greater than 70 J/g, but the composition may lose flexibility and become too rigid for practical applications

Engineering Contradiction:
ImprovePCM contentVSAvoidflexibility
Core Design Contradiction:
Quantity of substanceVSEase of operation

Solution Approach 1:

The patent uses very low viscosity RTV silicone elastomer (≤5000 mPa.s, preferably ≤1000 mPa.s) as the binding matrix. This low viscosity parameter enables the elastomer to effectively bind high amounts of PCM (100-300 phr) while maintaining composition homogeneity and flexibility, overcoming the rigidity issue that would normally occur with high PCM loading.

Inventive Principle:
Principle #35Parameter changes

3Stability of the object's composition

If the elastomer viscosity is reduced to enable high PCM content, then dispersibility and homogeneity improve, but the elastomer may lose structural stability and strength

Engineering Contradiction:
Improvedispersibility and homogeneityVSAvoidstructural stability
Core Design Contradiction:
Stability of the object's compositionVSStrength

Solution Approach 1:

The patent carefully selects and controls the viscosity parameter of the RTV silicone elastomer, reducing it to very low values (≤5000 mPa.s, preferably ≤1000 mPa.s) but not eliminating it completely. This optimized viscosity level provides the right balance: low enough to ensure excellent dispersibility and homogeneity of high PCM content, yet sufficient to maintain structural stability and mechanical strength of the final composition.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The composition achieves enhanced thermal energy absorption and release capabilities, suitable for demanding applications such as passive air conditioning and heating systems, with improved flexibility and temperature resistance.

Implementation Method 1

crosslinked rubber composition based on at least one 'RTV' silicone elastomer vulcanized at room temperature

Methodology Applied
Scientific EffectCrosslinking: Chemical Bonding

Implementation Method 2

crosslinked by polyaddition or polycondensation

Methodology Applied
Scientific EffectPolyaddition: Chemical Bonding

Implementation Method 3

crosslinked by polyaddition or polycondensation

Methodology Applied
Scientific EffectPolycondensation: Chemical Bonding

Implementation Method 4

PCM materials such as fatty acids, salts or paraffins, in particular, to release or absorb heat by change of state thanks to the latent heat of fusion which characterizes these PCMs

Methodology Applied
Scientific EffectPhase change: Phase Change

Implementation Method 5

release or absorb heat by change of state thanks to the latent heat of fusion which characterizes these PCMs

Methodology Applied
Scientific EffectLatent heat of fusion: Latent Heat

Implementation Method 6

pass from the liquid state to the solid state by releasing heat during their crystallization

Methodology Applied
Scientific EffectCrystallization: Crystallisation

Implementation Method 7

the composition then possibly having a thermal conductivity greater than 0.2 W.m-1K-1 and advantageously greater than 1 W.m-1K-1

Methodology Applied
Scientific EffectThermal conduction: Conduction (thermal)

Data Source

PatentEP2690141B1Silicone elastomer and MCP rubber composition, method for preparing same, flexible element and thermal control/regulation system including same
Publication Date: 2017.10.18 HUTCHINSON SA

AI summary

The present invention relates to a crosslinked rubber composition based on at least one room-temperature vulcanized "RTV" silicone elastomer and comprising at least one phase-change material (PCM), its preparation process, a flexible element comprising at least one elastomer layer capable of storing and releasing thermal energy, which is made of this composition, and a thermal control or regulation system incorporating at least one such flexible element. A composition according to the invention is such that said at least one silicone elastomer has a viscosity measured at 23°C according to ISO 3219 that is less than or equal to 5000 mPa·s. Advantageously, this silicone elastomer is of the two-component type A and B and is crosslinked by polyaddition or polycondensation, and the composition comprises the unencapsulated, micronized PCM in an amount greater than 50 parts per hundred (ppm).