Rubber Cord Coating Composition for Aged Tire Adhesion

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Solution Overview

Problem

Existing rubber coating mixtures for metallic reinforcements, particularly those using resorcinol-based systems, face challenges in maintaining adhesion properties after aging, which affects the durability of reinforced rubber products.

Innovation Solution

A sulfur-curable rubber coating mixture comprising a novolak resin with alkyl urethane units, produced by reacting a phenol compound and a carbamate resin, combined with a sulfenimide accelerator, such as N-tert-butyl-2-benzothiazolesulfenimide, to enhance adhesion and reduce the need for hazardous sulfenamide accelerators.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If resorcinol-based adhesion systems are used in rubber coating mixtures, then initial adhesion to metallic reinforcements is achieved, but adhesion properties deteriorate after aging under oxygen exposure

Engineering Contradiction:
Improveadhesion properties after agingVSAvoiddurability of reinforced rubber products
Core Design Contradiction:
ReliabilityVSDuration of action of stationary object

Solution Approach 1:

The patent changes the chemical composition parameters of the adhesion system by replacing resorcinol-based systems with novolak resins containing alkyl urethane units. This parameter change maintains initial adhesion while improving resistance to oxygen aging, thereby resolving the contradiction between initial adhesion and aged adhesion properties.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent uses composite material approach by combining novolak resins with alkyl urethane units and sulfenimide accelerators in a specific formulation. This composite adhesion system provides both initial bonding capability and long-term stability under aging conditions, resolving the contradiction between initial adhesion and durability after aging.

Inventive Principle:
Principle #40Composite materials

2Productivity

If sulfenamide accelerators are used to achieve sufficient vulcanization, then crosslinking speed is improved, but health and environmental hazards increase

Engineering Contradiction:
Improvevulcanization speedVSAvoidhazardous substances
Core Design Contradiction:
ProductivityVSObject-generated harmful factors

Solution Approach 1:

The patent replaces hazardous sulfenamide accelerators with sulfenimide accelerators that decompose more completely and produce fewer harmful byproducts. This substitution maintains vulcanization effectiveness while eliminating the health and environmental hazards associated with sulfenamide accelerators.

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Solution Approach 2:

The patent converts the potential harm of accelerator residues into a benefit by selecting sulfenimide accelerators that decompose more completely during vulcanization, leaving minimal harmful residues. This transforms the accelerator selection from a source of contamination to a solution that reduces environmental and health hazards.

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The combination achieves improved adhesion to metallic reinforcements even after aging, enhancing the durability of rubber products by maintaining strong reinforcement-rubber bonds under oxygen exposure.

Implementation Method 1

sulfur-crosslinkable rubber coating mixture

Methodology Applied
Scientific EffectSulfur crosslinking: Chemical Bonding

Implementation Method 2

During the vulcanization process, a resin is formed from the methylene donor and the methylene acceptor

Methodology Applied
Scientific EffectVulcanization: Chemical Bonding

Implementation Method 3

which interacts adhesively with the surface of the reinforcement

Methodology Applied
Scientific EffectAdhesion: Adhesive

Implementation Method 4

a second network based on methylene donor and methylene acceptor forms, which interacts adhesively with the surface of the reinforcement

Methodology Applied
Scientific EffectChemical bonding: Chemical Bonding

Implementation Method 5

During the vulcanization process, a resin is formed from the methylene donor and the methylene acceptor

Methodology Applied
Scientific EffectResin formation: Chemical Bonding

Implementation Method 6

a second network based on methylene donor and methylene acceptor forms

Methodology Applied
Scientific EffectPolymerization: Chemical Bonding

Data Source

PatentEP4399242B1Sulfur crosslinkable rubber composition and pneumatic tire
Publication Date: 2025.10.08 CONTINENTAL REIFEN DEUTSCHLAND GMBH

AI summary

The invention relates to a sulfur-crosslinkable rubber-coating mixture for metal tyre cords, the mixture containing - 0.25 to 5 phr (parts by weight per 100 parts by weight of all the rubbers in the mixture) of at least one novolac resin that includes alkyl urethane units and is produced by reacting a phenol compound, an aldehyde and a carbamate resin, the carbamate resin being produced by reacting alkyl urethane with an aldehyde, and - 0.5 to 3 phr of at least one sulfenimide accelerator. The invention further relates to a pneumatic vehicle tyre that includes at least one sulfur-crosslinked rubber-coating mixture of this kind.