Rubber-Metal Adhesion Layer Without Cobalt Salts or Solvents

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Solution Overview

Problem

Existing rubber-metal adhesion methods face challenges in achieving strong adhesion between rubber and metal members while minimizing environmental impact, such as the need for cobalt salts and sulfur in direct vulcanization and the use of organic solvents in indirect vulcanization.

Innovation Solution

A rubber-metal composite body is created using an adhesion layer containing a polyolefin-based resin with polar functional groups and a diene-olefin-based copolymer, where the rubber member contacts the copolymer and the metal member contacts the polar resin, enhancing adhesion through hydrogen bonding and compatibility.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Strength

If a direct vulcanization adhesion method is used with cobalt salt and sulfur, then adhesion strength is improved, but environmental burden increases and processability deteriorates

Engineering Contradiction:
Improveadhesion strengthVSAvoidenvironmental burden
Core Design Contradiction:
StrengthVSObject-affected harmful factors

Solution Approach 1:

The invention changes the chemical composition parameters of the adhesion layer by using acid-modified polyolefin resin instead of cobalt salt and sulfur, thereby maintaining adhesion strength while reducing environmental burden and improving processability

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention uses a composite adhesion layer comprising acid-modified polyolefin resin and specific copolymer materials to achieve strong adhesion without harmful substances, replacing the traditional cobalt-sulfur system

Inventive Principle:
Principle #40Composite materials

2Strength

If sulfur is used as a vulcanization system, then adhesion is achieved, but processability and heat deterioration resistance worsen

Engineering Contradiction:
ImproveadhesionVSAvoidprocessability
Core Design Contradiction:
StrengthVSEase of manufacture

Solution Approach 1:

The invention changes the vulcanization system from sulfur-based to an organic solvent-free system using acid-modified polyolefin resin, which eliminates the negative effects on processability and heat deterioration resistance while maintaining adhesion

Inventive Principle:
Principle #35Parameter changes

3Strength

If organic solvent is used in indirect vulcanization adhesion method, then adhesion is achieved, but environmental burden increases

Engineering Contradiction:
ImproveadhesionVSAvoidenvironmental burden
Core Design Contradiction:
StrengthVSObject-affected harmful factors

Solution Approach 1:

The invention extracts and eliminates organic solvents from the adhesion system by using acid-modified polyolefin resin that provides adhesion functionality without requiring harmful solvent carriers

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The invention changes the adhesion mechanism from solvent-based to a system based on acid-modified polyolefin resin that achieves adhesion through chemical modification rather than solvent mediation

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This configuration allows for strong, durable adhesion between rubber and metal members, reducing the need for cobalt salts and sulfur, and eliminating organic solvents, resulting in high-strength rubber-metal composite bodies suitable for tires and other rubber articles.

Implementation Method 1

the polyolefin-based resin having a polar functional group is an acid-modified polyolefin-based resin

Methodology Applied
Scientific EffectHydrogen bonding:

Data Source

PatentEP4067074B1Rubber-metal complex, tire, and rubber article
Publication Date: 2023.08.30 BRIDGESTONE CORP

AI summary

Provided is a rubber-metal composite body in which a rubber member and a metal member are firmly adhered to each other. The rubber-metal composite body is a rubber-metal composite body in which a rubber member and a metal member are adhered to each other via an adhesion layer, where the adhesion layer contains a polyolefin-based resin having a polar functional group, and a copolymer having a conjugated diene unit and a non-conjugated olefin unit but having no butylene unit, and the rubber member is in contact with at least the copolymer, and the metal member is in contact with at least the resin having a polar functional group.