Sacrificial Mould for Shrinkage Control in Pre-ceramic Composite Manufacturing

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Solution Overview

Problem

Current methods for manufacturing thermostructural composite articles from preceramic prepreg materials face significant challenges due to dimensional shrinkage during the ceramization process, which complicates the production of complex shapes and is costly, especially when using steel moulds that deform and corrode over time.

Innovation Solution

A method utilizing a sacrificial mould produced by lamination with the component, employing conventional prepregs like carbon fibre or basalt fibre to maintain shape during pyrolysis, avoiding shrinkage and deformation, and allowing for the use of preceramic polymers like poly-dimethylsiloxane without additives, which reduces costs and maintains thermomechanical integrity.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If steel moulds are used to maintain form during ceramization, then dimensional stability is improved, but manufacturing cost increases and the moulds suffer from deformation and corrosion

Engineering Contradiction:
Improvedimensional stabilityVSAvoidmanufacturing cost
Core Design Contradiction:
Manufacturing precisionVSEase of manufacture

Solution Approach 1:

The patent employs a disposable paper mould instead of expensive steel moulds. The paper mould is discarded after a single use, eliminating the high manufacturing costs and maintenance issues of steel moulds. This disposable approach resolves the contradiction by providing adequate dimensional stability for one-use applications without the excessive cost and durability problems of reusable steel moulds.

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Solution Approach 2:

The paper mould acts as an intermediary between the preceramic prepreg and the final ceramic component. It provides the necessary form and dimensional stability during ceramization, then is easily removed after serving its purpose. This intermediary role allows the use of low-cost materials while achieving the required manufacturing precision.

Inventive Principle:
Principle #24Intermediary (Mediator)

2Manufacturing precision

If preceramic polymers with additives are used to reduce shrinkage, then dimensional stability is improved, but material cost increases

Engineering Contradiction:
Improvedimensional stabilityVSAvoidmaterial cost
Core Design Contradiction:
Manufacturing precisionVSQuantity of substance

Solution Approach 1:

The paper mould provides preliminary counter-action to the shrinkage of preceramic polymers during ceramization. By being pressed against the prepreg, it mechanically opposes the dimensional reduction, compensating for the natural shrinkage tendency without requiring expensive shrinkage-reducing additives in the polymer itself.

Inventive Principle:
Principle #9Preliminary anti-action

Solution Approach 2:

The paper mould creates a negative copy or impression of the desired final component shape. The prepreg is formed to match the mould's geometry, and after ceramization, the component retains this shape. This copying approach allows accurate shape reproduction without modifying the preceramic polymer composition with costly additives.

Inventive Principle:
Principle #26Copying

3Ease of manufacture

If conventional prepregs are used without sacrificial mould, then production cost is reduced, but dimensional shrinkage of 50% occurs during ceramization

Engineering Contradiction:
Improveproduction costVSAvoiddimensional stability
Core Design Contradiction:
Ease of manufactureVSManufacturing precision

Solution Approach 1:

The sacrificial paper mould serves as an intermediary that temporarily provides dimensional stability during ceramization. It is pressed against the conventional prepreg to prevent shrinkage, then removed after the ceramic component is formed. This allows the use of inexpensive conventional prepregs while achieving the required dimensional accuracy.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The paper mould is applied to the prepreg before ceramization to preliminarily establish the desired shape and prevent shrinkage. This preliminary action of constraining the prepreg in the correct geometry allows conventional materials to produce precise components without requiring expensive shrinkage-resistant materials.

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This method enables the production of articles with complex shapes without shrinkage or deformation, maintaining the desired geometry and thermomechanical properties up to high temperatures, while reducing production costs and avoiding the limitations of traditional steel moulds.

Implementation Method 1

Preceramic polymers are polymers that can be converted into ceramic by means of a pyrolysis heat treatment at a temperature generally ranging from 600 to 1300°C

Methodology Applied
Scientific EffectPyrolysis: Pyrolysis

Implementation Method 2

a sacrificial mould, produced by lamination on another mould, together with the component to be manufactured

Methodology Applied
Scientific EffectMechanical constraint: Mechanical Force

Data Source

PatentEP3233481B1A method to manufacture an article of a fiber made reinforced thermostructural composite
Publication Date: 2019.01.30 ENTE PER LE NUOVE TECH LENERGIA E LAMBIENTE (ENEA)

AI summary

A method to manufacture an article made of a thermostructural composite starting from a preceramic prepreg and comprising the steps of: - preparing a prepreg multilayer material, in which at least one layer of preceramic prepreg is arranged between at least two layers of conventional prepreg; - cross-linking, during which the conventional prepreg and the preceramic prepreg are cross-linked; - ceramization, during which said prepreg multilayer material resulting from the cross-linking step undergoes a temperature that is greater than the one of the cross-linking step and is such as to cause the ceramization of said preceramic prepreg; - removal, during which said layers of conventional prepreg are removed.