Salt-Forming Dye Ink Composition for Ballpoint Pen

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Solution Overview

Problem

Conventional oil-based ink compositions for ball-point pens face issues with ink stability over time, poor light resistance, and writing feel, particularly due to the instability of nigrosine-based dyes and the reactivity of surfactants with dyes leading to precipitate formation and increased viscosity.

Innovation Solution

An oil-based ink composition incorporating salt-forming dyes such as dodecyl diphenyl oxide disulfonic acid and xanthene-based basic dyes, combined with a pigment like basic carbon black, and a polyvinyl butyral resin, along with an aromatic amine, to enhance stability, light resistance, and writing feel, while maintaining a suitable viscosity and pH range.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Quantity of substance

If nigrosine-based dye is used as coloring agent, then high concentration and low cost are achieved, but ink stability over time deteriorates due to poor solubility in organic solvent

Engineering Contradiction:
Improvedye concentrationVSAvoidink stability over time
Core Design Contradiction:
Quantity of substanceVSReliability

Solution Approach 1:

The patent changes the chemical parameters of the dye system by selecting specific salt-forming dyes (triarylmethane-based, xanthene-based, or azomethine-based basic dyes) with defined solubility characteristics in organic solvents. This parameter change resolves the contradiction by achieving both high concentration (1-10 mass%) and long-term stability without precipitation.

Inventive Principle:
Principle #35Parameter changes

2Ease of operation

If surfactant is incorporated as lubricant to improve feeling of writing, then writing smoothness is enhanced, but reaction with dye occurs and precipitate is generated

Engineering Contradiction:
Improvefeeling of writingVSAvoidink stability
Core Design Contradiction:
Ease of operationVSReliability

Solution Approach 1:

The patent extracts and eliminates the surfactant component from the ink composition, resolving the contradiction by achieving writing smoothness through alternative means (ball material selection, tip design, or natural lubrication from ink additives) without introducing substances that react with the dye to form precipitates.

Inventive Principle:
Principle #2Taking out (Extraction)

3Ease of operation

If viscosity of ink is decreased to improve feeling of writing, then writing smoothness is enhanced, but lubrication state changes from fluid lubrication to boundary lubrication and wear increases

Engineering Contradiction:
Improvefeeling of writingVSAvoidwear resistance
Core Design Contradiction:
Ease of operationVSReliability

Solution Approach 1:

The patent optimizes the viscosity parameter to a specific range (100-5000 mPa·s at 20°C) that maintains fluid lubrication conditions. This parameter change ensures both improved writing smoothness and preserved wear resistance by keeping the lubrication regime in the fluid or mixed lubrication zone rather than transitioning to boundary lubrication.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The composition provides a stable, deep-colored written trace with improved light resistance and writing feel, reducing wear and maintaining lubricity even under high writing pressure, thus addressing the limitations of previous ink formulations.

Implementation Method 1

the composition further comprises a salt-forming dye of an acid dye and an aromatic ring amine

Methodology Applied
Scientific EffectSalt-forming reaction: Chemical Bonding

Implementation Method 2

a polyvinyl butyral resin in which a hydroxyl group in a molecule is 20 to 40 mol%

Methodology Applied
Scientific EffectAdhesion: Adhesive

Implementation Method 3

comprising at least a dye, a pigment, and an organic solvent

Methodology Applied
Scientific EffectDissolution: Solvation

Data Source

PatentEP2824151B1Oil-based ink composition for ballpoint pen and oil-based refill for ballpoint pen using same
Publication Date: 2018.10.10 PILOT PEN CO LTD
  • EP2824151B1 patent drawingFigure 1~2
  • EP2824151B1 patent drawingFigure 3

AI summary

[Problem to be Solved] Provided are: an oil-based ink composition for a ball-point pen having a favorable feeling of writing, the favorable deepness of a written trace, favorable light resistance, favorable ink stability over time, and favorable pigment dispersibility; and an oil-based ball-point pen refill using the oil-based ink composition. [Solution] An oil-based ink composition for a ball-point pen comprising at least a dye, a pigment, and an organic solvent, wherein the dye is at least one salt-forming dye selected from the group consisting of salt-forming dyes of alkylbenzene sulfonic acids and xanthene-based basic dyes, salt-forming dyes of alkylbenzene sulfonic acids and triarylmethane-based basic dyes, and salt-forming dyes of alkylbenzene sulfonic acids and azomethine-based basic dyes.