Superabsorbent Polymer Surface Crosslinking for Rewetting Resistance

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Solution Overview

Problem

Superabsorbent polymers used in hygiene products face issues with rewetting and urine leakage phenomena due to pressure, which existing methods have not effectively addressed.

Innovation Solution

A superabsorbent polymer is developed by crosslinking an acrylic acid-based monomer with a sodium polycarboxylate surfactant and epoxy crosslinking agents of different equivalent weights, followed by surface modification, to enhance absorption properties and prevent rewetting.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Quantity of substance

If conventional superabsorbent polymers are used to achieve high absorbency, then water absorption capacity is improved, but rewetting and urine leakage phenomena occur under pressure

Engineering Contradiction:
Improvewater absorption capacityVSAvoidrewetting resistance
Core Design Contradiction:
Quantity of substanceVSReliability

Solution Approach 1:

The patent applies local quality by creating a surface crosslinked layer on the superabsorbent polymer particles. This surface layer has different properties (higher crosslinking density, lower water solubility) compared to the interior, providing pressure resistance and preventing rewetting while maintaining high absorption capacity in the core region.

Inventive Principle:
Principle #3Local quality

Solution Approach 2:

The patent uses composite materials by combining the base superabsorbent polymer (acrylic acid-based) with epoxy crosslinking agents and surfactants. The resulting composite structure integrates the high absorption capability of the polymer with the mechanical strength and pressure resistance of the crosslinked network.

Inventive Principle:
Principle #40Composite materials

2Reliability

If the superabsorbent polymer is highly crosslinked to suppress rewetting, then reliability under pressure is improved, but liquid permeability deteriorates

Engineering Contradiction:
Improverewetting resistanceVSAvoidliquid permeability
Core Design Contradiction:
ReliabilityVSObject-generated harmful factors

Solution Approach 1:

The surface crosslinked layer provides the necessary crosslinking density for rewetting resistance, while the interior maintains appropriate porosity and crosslinking for liquid permeability. This spatial differentiation of properties resolves the contradiction between reliability and permeability.

Inventive Principle:
Principle #3Local quality

Solution Approach 2:

The patent utilizes porous materials by maintaining a porous internal structure with controlled crosslinking density. The pores allow liquid penetration and absorption while the surface crosslinked layer prevents excessive water release under pressure, balancing permeability and rewetting resistance.

Inventive Principle:
Principle #31Porous materials

3Quantity of substance

If the superabsorbent polymer absorbs large amounts of liquid, then water retention capacity is improved, but urine leakage occurs under user weight pressure

Engineering Contradiction:
Improvewater retention capacityVSAvoidurine leakage
Core Design Contradiction:
Quantity of substanceVSObject-affected harmful factors

Solution Approach 1:

The surface crosslinked layer acts as a protective barrier prepared in advance to prevent urine leakage. This pre-formed protective layer resists the compressive force of user weight, preventing the absorbed urine from leaking out, thus cushioning against the harmful effect before it occurs.

Inventive Principle:
Principle #11Beforehand cushioning (Prior cushioning)

Solution Approach 2:

The composite structure of the crosslinked superabsorbent polymer with epoxy agents and surfactants creates a material that simultaneously achieves high water retention and pressure resistance, preventing urine leakage while maintaining absorption capacity.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The resulting superabsorbent polymer exhibits improved water retention, liquid permeability, and reduced rewetting and urine leakage, maintaining a dry state even under pressure.

Implementation Method 1

an acrylic acid-based monomer having acidic groups which are at least partially neutralized and an internal crosslinking agent are crosslinked

Methodology Applied
Scientific EffectCrosslinking: Chemical Bonding

Implementation Method 2

A superabsorbent polymer (SAP) is a synthetic polymeric material capable of absorbing moisture from 500 to 1000 times its own weight

Methodology Applied
Scientific EffectAbsorption: Absorption (physical)

Implementation Method 3

heating the base resin in the presence of a surface crosslinking agent to carry out surface modification of the base resin

Methodology Applied
Scientific EffectSurface crosslinking: Chemical Bonding

Implementation Method 4

heating the base resin in the presence of a surface crosslinking agent

Methodology Applied
Scientific EffectHeating: Heating

Implementation Method 5

an acrylic acid-based monomer having acidic groups which are at least partially neutralized and an internal crosslinking agent are crosslinked in the presence of a sodium polycarboxylate surfactant

Methodology Applied
Scientific EffectSurfactant action: Surfactant

Data Source

PatentUS12071523B2Superabsorbent polymer and preparation method for the same
Publication Date: 2024.08.27 LG CHEM LTD

AI summary

A method of preparing a superabsorbent polymer includes preparing a base resin in which an acrylic acid-based monomer having acidic groups which are at least partially neutralized and an internal crosslinking agent are crosslinked in the presence of a sodium polycarboxylate surfactant; and heating the base resin in the presence of a surface crosslinking agent to carry out surface modification of the base resin, wherein the internal crosslinking agent includes a first epoxy crosslinking agent having an epoxy equivalent weight of 100 g/eq or more to less than 130 g/eq, and a second epoxy crosslinking agent having an epoxy equivalent weight of 130 g/eq or more. The superabsorbent polymer provides improved rewetting property and liquid permeability.