Self-healing Dental Composite with Encapsulated Monomer

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Solution Overview

Problem

Dental restorative composites face issues with rapid wear and susceptibility to fracture, which limits their durability and effectiveness in dental repairs, and there is a need for materials with self-healing capabilities to autonomically resolve discontinuities.

Innovation Solution

A dental restorative composite is developed that includes microspheres encapsulating monomers and catalysts, which upon fracture, release and polymerize to heal the discontinuity, utilizing silane crosslinking agents and biocompatible crosslinking reactions at body temperature, enhancing the composite's resistance to fracture and wear.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Object-affected harmful factors

If synthetic composites are used for dental repairs, then aesthetic appearance and biocompatibility are improved, but resistance to fracture and wear resistance deteriorate

Engineering Contradiction:
Improveaesthetic appearance and biocompatibilityVSAvoidresistance to fracture and wear
Core Design Contradiction:
Object-affected harmful factorsVSStrength

Solution Approach 1:

The composite material is segmented into multiple functional components: base polymer matrix, silane crosslinking agents, and microspheres containing healing agents. This segmentation allows each component to perform its specific function while collectively improving both aesthetics and fracture resistance.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The invention uses composite materials by combining polymer matrices with silane crosslinking agents and microsphere additives. This creates a multi-phase composite system that simultaneously achieves aesthetic properties, biocompatibility, and enhanced mechanical strength through the synergistic interaction of components.

Inventive Principle:
Principle #40Composite materials

2Ease of operation

If conventional dental composites are used, then ease of application is maintained, but durability and self-repair capability are lost

Engineering Contradiction:
Improveease of applicationVSAvoiddurability and self-repair capability
Core Design Contradiction:
Ease of operationVSDuration of action of stationary object

Solution Approach 1:

The composite is prepared in advance with embedded microspheres containing healing agents and silane crosslinking agents. These components are pre-positioned within the matrix before application, allowing the material to maintain ease of application while possessing pre-configured self-healing and durability capabilities.

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The composite performs self-service through autonomous self-healing functionality. When fracture occurs, the embedded microspheres rupture and release healing agents that automatically repair the damage without external intervention, thereby extending durability while maintaining ease of initial application.

Inventive Principle:
Principle #25Self-service

3Strength

If self-healing capabilities are added to composites, then resistance to fracture and durability are improved, but device complexity increases

Engineering Contradiction:
Improveresistance to fracture and durabilityVSAvoidcomposite formulation complexity
Core Design Contradiction:
StrengthVSDevice complexity

Solution Approach 1:

The self-healing mechanism is nested within the composite structure by embedding microspheres containing healing agents inside the polymer matrix. This nested configuration allows the complex self-healing functionality to be integrated within the simpler outer composite structure, improving fracture resistance while managing formulation complexity through hierarchical organization.

Inventive Principle:
Principle #7Nested doll (Nesting)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The composite exhibits improved resistance to fracturing, increased flexural strength, and better durability, allowing for more effective and long-lasting dental repairs without external stimuli, addressing the limitations of existing composites.

Implementation Method 1

utilizing silane crosslinking agents and biocompatible crosslinking reactions at body temperature

Methodology Applied
Scientific EffectHydrolysis: Hydrolysis

Implementation Method 2

silane crosslinking agents and biocompatible crosslinking reactions

Methodology Applied
Scientific EffectCrosslinking: Chemical Bonding

Implementation Method 3

release and polymerize to heal the discontinuity

Methodology Applied
Scientific EffectPolymerization: Photopolymerisation

Data Source

PatentEP2152224B1Self-healing dental composites
Publication Date: 2022.08.17 PREMIER DENTAL PRODUCTS CO LLC

AI summary

Dental restorative composites having self-healing capabilities to repair discontinuities in the composite are provided. Dental restorative composites according to the present invention include a microsphere that encapsulates a monomer. When a fracture occurs, the microsphere is ruptured and the monomer fills the fracture. Depending on the monomer present in the microsphere, it is polymerized by a polymerization initiator or by an olefin metathesis catalyst present in the dental restorative composite. Self-healing dental restorative composites provide increased resistance to fracturing, and thus remain substantially intact for a longer period of time, preserving the remedial integrity of the dental repair or reconstruction.